ALIAS (Aircraft Laser Infrared Absorption Spectrometer) measures total water, total water isotopes, carbon monoxide, and carbon dioxide isotope ratios. No other instrument provides real-time measurements of carbon dioxide isotope ratios which are clear identifiers of atmospheric transport (18O/17O/16O for stratospheric intrusion, 13C/12C for anthropogenic signals). ALIAS easily adapts to changing mission priorities and can be configured to measure HCl, CH4, SO2, and N2O by simply replacing a semiconductor laser. These measurements contribute to Atmospheric Composition Focus Area research by providing key data on how convective processes affect stratospheric composition, the development of cirrus particles and their affect on Earth's radiative balance, and health of the ozone layer through measurement of chlorine partitioning.

ATHOS uses laser-induced fluorescence (LIF) to measure OH and HO2 simultaneously. OH is both excited and detected with the A2Σ+ (v’=0) → X2π (v”=0) transition near 308 nm. HO2 is reacted with reagent NO to form OH and is then detected with LIF. The laser is tuned on and off the OH wavelength to determine the fluorescence and background signals. ATHOS can detect OH and HO2 in clear air and light clouds from Earth's surface to the lower stratosphere. The ambient air is slowed from the aircraft speed of 240 m/s to 8-40 m/s in an aerodynamic nacelle. It is then pulled by a vacuum pump through a small inlet, up a sampling tube, and into two low-pressure detection cells - the first for OH and the second for HO2. Detection occurs in each cell at the intersection of the airflow, the laser beam, and the detector field-of-view.

This is a stratospheric lidar which is configured to fly on the NASA DC-8. It is a zenith viewing instrument, which makes vertical profile measurements of ozone, aerosols and temperature. Stratospheric ozone can be measured at solar zenith angles greater than ~30 degrees, while temperature and aerosols require SZA > 90 degrees. The SNR is maximized under dark coonditions. The measurement of Near-field water vapor measurements is being investigated and could be readily implemented. The instrument utilizes a XeCl excimer laser and a Nd-YAG laser to make DIAL, Raman DIAL, and backscatter measurements. A zenith viewing 16" telescope receives the lidar returns.

The Airborne Laser Infrared Absorption Spectrometer (ALIAS-II) is a very high resolution scanning tunable diode laser spectrometer which makes direct, simultaneous measurements of selectable combinations of HCl, NO2, CO, CO2, CH4, and N2O at sub-part-per-billion levels over a 3-30 second integration time. The measurement technique is based upon using tunable lead-salt and/or quantum cascade lasers operating from 3.4 to 8 microns wavelength scanning over absorption lines at 10 Hz recording second harmonic spectra. The instrument features an open-cradle multipass Herriott absorption cell with 15.24-cm diameter spherical zerodur mirrors coated with gold on chrome. The separation between the mirrors is adjustable allowing for a relatively small cell (0.75-m to 1.5-m) to contain an optical path length up to 120-m, depending on the spacing of the mirrors. Lasers and detectors are contained in a lightweight aluminum liquid nitrogen Dewar which can achieve a 28-hour hold time with only a 2 liter charge of liquid nitrogen. The instrument features custom laser current drives, signal chains, InSb detectors and preamps, 16-bit signal averager, analog signal conditioner, and digital I/O which are controlled by an onboard Pentium processor. Data is written to a ruggedized 2-Gb hard disk every 30 seconds and simultaneously transmitted via telemetry to ground station computers which provide backup storage of the data. The instrument weighs 36 kg and requires <56 watts for operation. Additional power up to 250 watts is available for structural heaters and current draw varies with atmospheric conditions.