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Harvard Integrated Cavity Output Spectroscopy (ICOS)

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PI

The Harvard CRDS/ICOS instrument is an absorption spectrometer that uses the relatively new and highly sensitive techniques of integrated cavity output spectroscopy (ICOS) and cavity ringdown spectroscopy (CRDS) with a high-finesse optical cavity and a cw quantum cascade laser (QCL) source. The primary spectroscopic technique employed is ICOS, in which intra-cavity absorption is measured from the steady-state output of the cavity. Light from a high power, tunable, single mode, solid-state laser source is coupled into a cavity consisting of two concave, highly reflective mirrors (R ≈ 0.9999), through which air continuously flows. The laser is scanned over a spectral region of 1–2 cm-1 containing an absorption feature, and the cavity output is detected by an LN2-cooled HgCdTe detector. The resultant output approximates an absorption spectrum with an effective pathlength of > 5 km, far greater than that of standard multipass Herriott or White cells.

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