TransCom N2O model inter-comparison – Part 2: Atmospheric inversion estimates of N2O emissions

Thompson, R.L., K. Ishijima, E. Saikawa, M. Corazza, U. Karstens, P.K. Patra, P. Bergamaschi, F. Chevallier, E. Dlugokencky, R.G. Prinn, R. Weiss, S. O’Doherty, P.J. Fraser, L.P. Steele, P.B. Krummel, A. Vermeulen, Y. Tohjima, A. Jordan, L. Haszpra, M. Steinbacher, S. Van der Laan, T. Aalto, F. Meinhardt, M.E. Popa, J. Moncrieff, and P. Bousquet (2014), TransCom N2O model inter-comparison – Part 2: Atmospheric inversion estimates of N2O emissions, Atmos. Chem. Phys., 14, 6177-6194, doi:10.5194/acp-14-6177-2014.
Abstract

This study examines N2O emission estimates from five different atmospheric inversion frameworks based on chemistry transport models (CTMs). The five frameworks differ in the choice of CTM, meteorological data, prior uncertainties and inversion method but use the same prior emissions and observation data set. The posterior modelled atmospheric N2O mole fractions are compared to observations to assess the performance of the inversions and to help diagnose problems in the modelled transport. Additionally, the mean emissions for 2006 to 2008 are compared in terms of the spatial distribution and seasonality. Overall, there is a good agreement among the inversions for the mean global total emission, which ranges from 16.1 to 18.7 TgN yr 1 and is consistent with previous estimates. Ocean emissions represent between 31 and 38% of the global total com- pared to widely varying previous estimates of 24 to 38 %. Emissions from the northern mid- to high latitudes are likely to be more important, with a consistent shift in emissions from the tropics and subtropics to the mid- to high latitudes in the Northern Hemisphere; the emission ratio for 0–30

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