Inferring regional sources and sinks of atmospheric CO2 from GOSAT XCO2 data

Deng, F., D. B. A. Jones, D. Henze, N. Bousserez, K. Bowman, J. B. Fisher, R. Nassar, C. O'Dell, D. Wunch, P. Wennberg, E. Kort, S. C. Wofsy, T. Blumenstock, N. M. Deutscher, D. W. T. Griffith, F. Hase, P. Heikkinen, V. Sherlock, K. Strong, R. Sussmann, and T. Warneke (2014), Inferring regional sources and sinks of atmospheric CO2 from GOSAT XCO2 data, Atmos. Chem. Phys., 14, 3703-3727, doi:10.5194/acp-14-3703-2014.

We have examined the utility of retrieved columnaveraged, dry-air mole fractions of CO2 (XCO2 ) from the Greenhouse Gases Observing Satellite (GOSAT) for quantifying monthly, regional flux estimates of CO2 , using the GEOS-Chem four-dimensional variational (4D-Var) data assimilation system. We focused on assessing the potential impact of biases in the GOSAT CO2 data on the regional flux estimates. Using different screening and bias correction approaches, we selected three different subsets of the GOSAT XCO2 data for the 4D-Var inversion analyses, and found that the inferred global fluxes were consistent across the three XCO2 inversions. However, the GOSAT observational coverage was a challenge for the regional flux estimates. In the northern extratropics, the inversions were more sensitive to North American fluxes than to European and Asian fluxes due to the lack of observations over Eurasia in winter and over eastern and southern Asia in summer. The regional flux estimates were also sensitive to the treatment of the residual bias in the GOSAT XCO2 data. The largest differences obtained were for temperate North America and temperate South America, for which the largest spread between the inversions was 1.02 and 0.96 Pg C, respectively. In the case of temperate North America, one inversion suggested a strong source, whereas the second and third XCO2 inversions produced a weak and strong sink, respectively. Despite the discrepancies in the regional flux estimates between the three XCO2 inversions, the a posteriori CO2 distributions were in good agreement (with a mean difference between the three inversions of typically less than 0.5 ppm) with independent data from the Total Carbon Column Observing Network (TCCON), the surface flask network, and from the HIAPER Pole-to-Pole Observations (HIPPO) aircraft campaign. The discrepancy in the regional flux estimates from the different inversions, despite the agreement of the global flux estimates

PDF of Publication: 
Download from publisher's website.