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An operational data product available for both the Suomi National Polar-orbiting Partnership (S-NPP) and National Oceanic and Atmospheric Administration-20 (NOAA20) platforms provides high-spatial-resolution infrared (IR) absorption band radiances for Visible Infrared Imaging Radiometer Suite (VIIRS) based on a VIIRS and Crosstrack Infrared Sounder (CrIS) data fusion method. This study investigates the use of these IR radiances, centered at 4.5, 6.7, 7.3, 9.7, 13.3, 13.6, 13.9, and 14.2 µm, to construct atmospheric moisture products (e.g., total precipitable water and upper tropospheric humidity) and to evaluate their accuracy. Total precipitable water (TPW) and upper tropospheric humidity (UTH) retrieved from hyperspectral sounder CrIS measurements are provided at the associated VIIRS sensor’s high spatial resolution (750 m) and are compared subsequently to collocated operational Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) and S-NPP VIIRS moisture products. This study suggests that the use of VIIRS IR absorption band radiances will provide continuity with Aqua MODIS moisture products.