48 1001 ELKINS, JAMES; HURST, DALE; ROMASHKIN, PAVEL; DUTTON, GEOFF U.S. DEPT OF COMMERCE, NOAA / CMDL / HALOCARBONS AND OTHER ATMOSPHERIC TRACE SPECIES GROUP ACATS SOLVE 1 1 2000 01 14 2000 12 21 0 ELAPSED TIME IN SECONDS FROM 00:00:00 GMT ON SAMPLE DATE 8 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 Mean Age of Air (years) Mean Age Error (1-sd) (years) Total Br (ppt) Total Organic Br (ppt) Total Inorganic Br (ppt) Total Cl (ppb) Total Organic Cl (ppb) Total Inorganic Cl (ppb) 25 The mean age (Age) of each sampled air mass was determined from the corresponding ACATS measurement of SF6 and the documented tropospheric trend of SF6 [Geller et al., 1997] using a variation of the mean age formula in Volk et al. [1997]. We use dG = -0.8 to account for a SF6 calibration scale change. This term no longer represents only a delay from the surface to the tropopause. The mean age error reported is solely based on the SF6 measurement precision and is thus useful in comparing ACATS ages from different flights. Absolute accuracy of the SF6 measurement and any systematic errors in the method used to calculate mean ages are not included. Organic chlorine (CCly) was calculated from ACATS in-situ measurements of CFC-11, CFC-12, CFC-113, CH3CCl3, and CCl4. Contributions to CCly from CH3Cl and HCFC-22 (measured by WAS) were calculated from their correlations with tracers measured by ACATS. Organic bromine (CBry) was calculated from ACATS in-situ measurements of halon-1211. Contributions to CBry from CH3Br, halon-2402, halon-1301, CH2Br2, and CH2BrCl (measured by WAS) were calculated from their correlations with tracers measured by ACATS using the formula in Wamsley et al. [1997]. The total chlorine (TotalCl) and total bromine (TotalBr) content of each sampled air mass was calculated from the documented tropospheric trends of chlorinated and brominated trace gases (e.g., Montzka et al. [1996]) and weighted with a mean age spectrum calculated by Hall & Plumb [1994]. Inorganic chlorine (Cly) and inorganic bromine (Bry) were calculated as TotalCl-CCly and TotalBr-CBry, respectively. Data submitted only for air masses with potential temperature greater than 380 K. 1 GMTs Age AgeERR TotalBr CBry Bry TotalCl CCly Cly 45305 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 45375 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 45445 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 45515 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 45585 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 45655 1.70 0.55 19.381 14.927 4.455 3.411 2.957 0.454 45725 1.09 0.53 19.489 9999.000 9999.000 3.393 9999.000 9999.000 45865 1.55 0.54 19.407 9999.000 9999.000 3.407 9999.000 9999.000 45935 9999.00 9999.00 9999.000 14.921 9999.000 9999.000 2.972 9999.000 46005 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 46075 9999.00 9999.00 9999.000 14.023 9999.000 9999.000 2.906 9999.000 46145 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 46215 9999.00 9999.00 9999.000 13.935 9999.000 9999.000 2.897 9999.000 46285 2.58 0.53 19.201 9999.000 9999.000 3.434 9999.000 9999.000 46425 2.66 0.53 19.180 9999.000 9999.000 3.436 9999.000 9999.000 46495 3.23 0.50 19.015 7.955 11.060 3.447 2.273 1.175 46565 3.07 0.49 19.065 9999.000 9999.000 3.444 9999.000 9999.000 46705 3.03 0.49 19.077 9999.000 9999.000 3.443 9999.000 9999.000 46775 2.86 0.49 19.124 6.603 12.521 3.440 2.099 1.341 46845 3.15 0.50 19.040 9999.000 9999.000 3.446 9999.000 9999.000 46985 3.40 0.50 18.963 9999.000 9999.000 3.450 9999.000 9999.000 47055 3.65 0.51 18.884 5.512 13.372 3.454 1.951 1.503 47125 3.44 0.50 18.950 9999.000 9999.000 3.451 9999.000 9999.000 47195 3.52 0.50 18.924 5.348 13.576 3.452 1.928 1.524 47265 3.91 0.51 18.803 9999.000 9999.000 3.458 9999.000 9999.000 47335 3.74 0.51 18.857 5.344 13.513 3.455 1.939 1.517 47405 3.99 0.51 18.776 9999.000 9999.000 3.458 9999.000 9999.000 47545 4.08 0.47 18.748 9999.000 9999.000 3.459 9999.000 9999.000 47615 3.99 0.51 18.776 4.576 14.199 3.458 1.826 1.632 47685 3.65 0.51 18.884 9999.000 9999.000 3.454 9999.000 9999.000 47755 3.91 0.51 18.803 5.004 13.799 3.458 1.884 1.573 47825 3.82 0.51 18.830 9999.000 9999.000 3.456 9999.000 9999.000 47895 4.03 0.51 18.762 4.749 14.013 3.459 1.849 1.610 47965 3.82 0.51 18.830 9999.000 9999.000 3.456 9999.000 9999.000 48105 4.03 0.47 18.762 9999.000 9999.000 3.459 9999.000 9999.000 48175 4.29 0.48 18.680 3.602 15.079 3.461 1.651 1.810 48245 4.12 0.47 18.735 9999.000 9999.000 3.460 9999.000 9999.000 48315 4.25 0.48 18.694 3.668 15.025 3.461 1.675 1.786 48385 4.12 0.47 18.735 9999.000 9999.000 3.460 9999.000 9999.000 48455 4.29 0.48 18.680 3.599 15.081 3.461 1.675 1.787 48525 4.25 0.48 18.694 9999.000 9999.000 3.461 9999.000 9999.000 48665 4.34 0.48 18.667 9999.000 9999.000 3.462 9999.000 9999.000 48735 3.99 0.51 18.776 3.584 15.192 3.458 1.660 1.798 48805 4.38 0.48 18.653 9999.000 9999.000 3.462 9999.000 9999.000 48875 4.21 0.48 18.708 3.496 15.211 3.461 1.651 1.809 48945 3.69 0.51 18.870 9999.000 9999.000 3.455 9999.000 9999.000 49015 3.86 0.51 18.816 4.447 14.369 3.457 1.802 1.655 49085 3.65 0.51 18.884 9999.000 9999.000 3.454 9999.000 9999.000 49225 3.65 0.51 18.884 9999.000 9999.000 3.454 9999.000 9999.000 49295 3.82 0.51 18.830 4.853 13.976 3.456 1.871 1.585 49365 4.03 0.51 18.762 9999.000 9999.000 3.459 9999.000 9999.000 49505 3.91 0.51 18.803 9999.000 9999.000 3.458 9999.000 9999.000 49575 3.99 0.51 18.776 4.442 14.333 3.458 1.806 1.653 49645 3.69 0.51 18.870 9999.000 9999.000 3.455 9999.000 9999.000 49785 3.52 0.50 18.924 9999.000 9999.000 3.452 9999.000 9999.000 49855 3.69 0.51 18.870 4.188 14.682 3.455 1.765 1.690 49925 3.69 0.51 18.870 9999.000 9999.000 3.455 9999.000 9999.000 49995 3.57 0.50 18.910 5.303 13.607 3.453 1.930 1.523 50065 3.61 0.51 18.897 9999.000 9999.000 3.454 9999.000 9999.000 50135 3.57 0.50 18.910 5.748 13.163 3.453 1.986 1.467 50205 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 50345 3.48 0.50 18.937 9999.000 9999.000 3.452 9999.000 9999.000 50415 3.40 0.50 18.963 5.737 13.226 3.450 1.989 1.461 50485 3.03 0.49 19.077 9999.000 9999.000 3.443 9999.000 9999.000 50625 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 50695 3.40 0.50 18.963 7.272 11.691 3.450 2.180 1.270 50765 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 50905 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 50975 3.36 0.50 18.976 6.898 12.078 3.450 2.118 1.332 51045 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 51115 3.61 0.51 18.897 6.749 12.148 3.454 2.098 1.356 51185 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 51255 3.36 0.50 18.976 6.828 12.149 3.450 2.110 1.340 51325 3.40 0.50 18.963 9999.000 9999.000 3.450 9999.000 9999.000 51465 3.57 0.50 18.910 9999.000 9999.000 3.453 9999.000 9999.000 51535 3.40 0.50 18.963 6.456 12.507 3.450 2.040 1.411 51605 3.61 0.51 18.897 9999.000 9999.000 3.454 9999.000 9999.000 51675 3.32 0.50 18.989 6.981 12.009 3.449 2.137 1.312 51745 3.48 0.50 18.937 9999.000 9999.000 3.452 9999.000 9999.000 51815 3.36 0.50 18.976 6.851 12.126 3.450 2.135 1.314 51885 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 52025 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 52095 3.40 0.50 18.963 6.840 12.123 3.450 2.108 1.342 52165 3.40 0.50 18.963 9999.000 9999.000 3.450 9999.000 9999.000 52305 3.40 0.50 18.963 9999.000 9999.000 3.450 9999.000 9999.000 52375 3.27 0.50 19.002 6.986 12.016 3.448 2.187 1.261 52445 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 52585 2.86 0.49 19.124 9999.000 9999.000 3.440 9999.000 9999.000 52655 2.90 0.49 19.113 7.478 11.635 3.441 2.247 1.194 52725 3.44 0.50 18.950 9999.000 9999.000 3.451 9999.000 9999.000 52795 3.36 0.50 18.976 7.541 11.435 3.450 2.239 1.210 52865 3.23 0.50 19.015 9999.000 9999.000 3.447 9999.000 9999.000 52935 3.15 0.50 19.040 7.458 11.582 3.446 2.245 1.201 53005 3.15 0.50 19.040 9999.000 9999.000 3.446 9999.000 9999.000 53145 2.94 0.49 19.101 9999.000 9999.000 3.442 9999.000 9999.000 53215 2.94 0.49 19.101 7.973 11.128 3.442 2.293 1.149 53285 2.90 0.49 19.113 9999.000 9999.000 3.441 9999.000 9999.000 53355 3.19 0.50 19.027 8.276 10.752 3.447 2.342 1.105 53425 2.94 0.49 19.101 9999.000 9999.000 3.442 9999.000 9999.000 53495 2.86 0.49 19.124 8.201 10.923 3.440 2.308 1.132 53565 3.23 0.50 19.015 9999.000 9999.000 3.447 9999.000 9999.000 53705 3.11 0.50 19.052 9999.000 9999.000 3.445 9999.000 9999.000 53775 2.99 0.49 19.089 8.179 10.910 3.443 2.312 1.131 53845 3.11 0.50 19.052 9999.000 9999.000 3.445 9999.000 9999.000 53985 3.03 0.49 19.077 9999.000 9999.000 3.443 9999.000 9999.000 54055 2.90 0.49 19.113 7.921 11.191 3.441 2.288 1.153 54125 2.86 0.49 19.124 9999.000 9999.000 3.440 9999.000 9999.000 54265 3.11 0.50 19.052 9999.000 9999.000 3.445 9999.000 9999.000 54335 2.74 0.53 19.158 7.550 11.609 3.437 2.250 1.187 54405 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 54475 3.07 0.49 19.065 7.277 11.788 3.444 2.215 1.229 54545 2.86 0.49 19.124 9999.000 9999.000 3.440 9999.000 9999.000 54615 3.15 0.50 19.040 7.240 11.800 3.446 2.216 1.230 54685 3.44 0.50 18.950 9999.000 9999.000 3.451 9999.000 9999.000 54825 3.40 0.50 18.963 9999.000 9999.000 3.450 9999.000 9999.000 54895 3.74 0.51 18.857 6.927 11.930 3.455 2.166 1.289 54965 3.11 0.50 19.052 9999.000 9999.000 3.445 9999.000 9999.000 55105 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 55175 2.78 0.53 19.147 7.967 11.180 3.438 2.285 1.153 55245 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 55385 3.07 0.49 19.065 9999.000 9999.000 3.444 9999.000 9999.000 55455 3.44 0.50 18.950 7.792 11.158 3.451 2.268 1.183 55525 3.11 0.50 19.052 9999.000 9999.000 3.445 9999.000 9999.000 55595 3.11 0.50 19.052 8.036 11.017 3.445 2.290 1.155 55665 3.23 0.50 19.015 9999.000 9999.000 3.447 9999.000 9999.000 55735 3.11 0.50 19.052 8.192 10.860 3.445 2.314 1.131 55805 3.44 0.50 18.950 9999.000 9999.000 3.451 9999.000 9999.000 55945 2.66 0.53 19.180 9999.000 9999.000 3.436 9999.000 9999.000 56015 3.03 0.49 19.077 7.611 11.466 3.443 2.234 1.210 56085 3.03 0.49 19.077 9999.000 9999.000 3.443 9999.000 9999.000 56155 2.74 0.53 19.158 8.576 10.583 3.437 2.365 1.073 56225 2.62 0.53 19.191 9999.000 9999.000 3.435 9999.000 9999.000 56295 2.78 0.53 19.147 8.721 10.426 3.438 2.384 1.055 56365 2.99 0.49 19.089 9999.000 9999.000 3.443 9999.000 9999.000 56505 2.66 0.53 19.180 9999.000 9999.000 3.436 9999.000 9999.000 56575 2.58 0.53 19.201 8.749 10.452 3.434 2.378 1.056 56645 2.86 0.49 19.124 9999.000 9999.000 3.440 9999.000 9999.000 56715 2.74 0.53 19.158 8.451 10.707 3.437 2.343 1.095 56785 2.82 0.49 19.136 9999.000 9999.000 3.439 9999.000 9999.000 56855 3.19 0.50 19.027 9.070 9.958 3.447 2.416 1.031 56925 3.03 0.49 19.077 9999.000 9999.000 3.443 9999.000 9999.000 57065 2.94 0.49 19.101 9999.000 9999.000 3.442 9999.000 9999.000 57135 2.78 0.53 19.147 9.407 9.741 3.438 2.441 0.997 57205 2.82 0.49 19.136 9999.000 9999.000 3.439 9999.000 9999.000 57275 2.90 0.49 19.113 9.364 9.749 3.441 2.452 0.989 57345 2.78 0.53 19.147 9999.000 9999.000 3.438 9999.000 9999.000 57415 2.94 0.49 19.101 9.551 9.550 3.442 2.471 0.970 57485 3.03 0.49 19.077 9999.000 9999.000 3.443 9999.000 9999.000 57625 2.62 0.53 19.191 9999.000 9999.000 3.435 9999.000 9999.000 57695 3.40 0.50 18.963 9.751 9.212 3.450 2.500 0.950 57765 2.86 0.49 19.124 9999.000 9999.000 3.440 9999.000 9999.000 57905 3.19 0.50 19.027 9999.000 9999.000 3.447 9999.000 9999.000 57975 2.86 0.49 19.124 9.495 9.630 3.440 2.459 0.981 58045 2.94 0.49 19.101 9999.000 9999.000 3.442 9999.000 9999.000 58185 2.54 0.52 19.211 9999.000 9999.000 3.433 9999.000 9999.000 58255 3.07 0.49 19.065 9.446 9.619 3.444 2.449 0.996 58325 2.94 0.49 19.101 9999.000 9999.000 3.442 9999.000 9999.000 58395 2.94 0.49 19.101 9.725 9.376 3.442 2.498 0.944 58465 2.58 0.53 19.201 9999.000 9999.000 3.434 9999.000 9999.000 58535 2.46 0.52 19.231 10.742 8.489 3.431 2.600 0.831 58605 2.58 0.53 19.201 9999.000 9999.000 3.434 9999.000 9999.000 58745 2.86 0.49 19.124 9999.000 9999.000 3.440 9999.000 9999.000 58815 2.66 0.53 19.180 10.362 8.818 3.436 2.548 0.888 58885 2.58 0.53 19.201 9999.000 9999.000 3.434 9999.000 9999.000 58955 2.90 0.49 19.113 10.134 8.979 3.441 2.534 0.907 59025 3.07 0.49 19.065 9999.000 9999.000 3.444 9999.000 9999.000 59095 2.94 0.49 19.101 9.925 9.176 3.442 2.498 0.944 59165 2.82 0.53 19.136 9999.000 9999.000 3.439 9999.000 9999.000 59305 2.82 0.49 19.136 9999.000 9999.000 3.439 9999.000 9999.000 59375 2.82 0.53 19.136 10.077 9.059 3.439 2.525 0.914 59445 3.07 0.49 19.065 9999.000 9999.000 3.444 9999.000 9999.000 59515 2.42 0.52 19.241 10.256 8.984 3.430 2.551 0.879 59585 2.50 0.52 19.221 9999.000 9999.000 3.432 9999.000 9999.000 59655 2.70 0.53 19.169 10.506 8.664 3.437 2.566 0.870 59725 2.66 0.53 19.180 9999.000 9999.000 3.436 9999.000 9999.000 59865 2.54 0.52 19.211 9999.000 9999.000 3.433 9999.000 9999.000 59935 2.38 0.52 19.250 10.359 8.891 3.429 2.556 0.873 60005 2.54 0.52 19.211 9999.000 9999.000 3.433 9999.000 9999.000 60075 2.90 0.49 19.113 10.224 8.889 3.441 2.533 0.908 60145 3.19 0.50 19.027 9999.000 9999.000 3.447 9999.000 9999.000 60215 2.86 0.49 19.124 10.359 8.765 3.440 2.542 0.898 60285 2.90 0.49 19.113 9999.000 9999.000 3.441 9999.000 9999.000 60425 2.42 0.52 19.241 9999.000 9999.000 3.430 9999.000 9999.000 60495 2.82 0.53 19.136 9.931 9.205 3.439 2.491 0.949 60565 2.26 0.52 19.277 9999.000 9999.000 3.426 9999.000 9999.000 60705 3.48 0.50 18.937 9999.000 9999.000 3.452 9999.000 9999.000 60775 3.11 0.50 19.052 8.605 10.447 3.445 2.327 1.118 60845 3.40 0.50 18.963 9999.000 9999.000 3.450 9999.000 9999.000 60985 3.95 0.51 18.789 9999.000 9999.000 3.458 9999.000 9999.000 61055 4.12 0.47 18.735 4.547 14.188 3.460 1.771 1.689 61125 3.74 0.51 18.857 9999.000 9999.000 3.455 9999.000 9999.000 61195 3.86 0.51 18.816 4.994 13.823 3.457 1.858 1.599 61265 4.03 0.51 18.762 9999.000 9999.000 3.459 9999.000 9999.000 61335 3.95 0.51 18.789 4.968 13.821 3.458 1.837 1.621 61405 3.91 0.51 18.803 9999.000 9999.000 3.458 9999.000 9999.000 61545 3.69 0.51 18.870 9999.000 9999.000 3.455 9999.000 9999.000 61615 3.78 0.51 18.843 4.928 13.915 3.456 1.841 1.615 61685 3.91 0.51 18.803 9999.000 9999.000 3.458 9999.000 9999.000 61825 3.74 0.51 18.857 9999.000 9999.000 3.455 9999.000 9999.000 61895 3.91 0.51 18.803 4.818 13.984 3.458 1.815 1.642 61965 4.03 0.51 18.762 9999.000 9999.000 3.459 9999.000 9999.000 62105 3.99 0.51 18.776 9999.000 9999.000 3.458 9999.000 9999.000 62175 4.25 0.48 18.694 3.959 14.735 3.461 1.671 1.790 62245 3.57 0.50 18.910 9999.000 9999.000 3.453 9999.000 9999.000 62315 3.78 0.51 18.843 4.419 14.425 3.456 1.762 1.694 62385 3.86 0.51 18.816 9999.000 9999.000 3.457 9999.000 9999.000 62455 4.34 0.48 18.667 4.513 14.154 3.462 1.758 1.703 62525 4.12 0.47 18.735 9999.000 9999.000 3.460 9999.000 9999.000 62665 3.99 0.51 18.776 9999.000 9999.000 3.458 9999.000 9999.000 62735 3.82 0.51 18.830 4.814 14.016 3.456 1.809 1.648 62805 3.99 0.51 18.776 9999.000 9999.000 3.458 9999.000 9999.000 62875 3.86 0.51 18.816 4.424 14.392 3.457 1.767 1.690 62945 3.95 0.51 18.789 9999.000 9999.000 3.458 9999.000 9999.000 63015 3.61 0.51 18.897 4.423 14.474 3.454 1.763 1.691 63085 3.95 0.51 18.789 9999.000 9999.000 3.458 9999.000 9999.000 63225 3.91 0.51 18.803 9999.000 9999.000 3.458 9999.000 9999.000 63295 3.78 0.51 18.843 5.330 13.513 3.456 1.917 1.539 63365 3.69 0.51 18.870 9999.000 9999.000 3.455 9999.000 9999.000 63505 4.12 0.47 18.735 9999.000 9999.000 3.460 9999.000 9999.000 63575 3.91 0.51 18.803 5.425 13.378 3.458 1.911 1.547 63645 3.61 0.51 18.897 9999.000 9999.000 3.454 9999.000 9999.000 63785 3.95 0.51 18.789 9999.000 9999.000 3.458 9999.000 9999.000 63855 3.82 0.51 18.830 5.271 13.559 3.456 1.915 1.541 63925 3.86 0.51 18.816 9999.000 9999.000 3.457 9999.000 9999.000 63995 3.74 0.51 18.857 6.155 12.702 3.455 2.023 1.433 64065 3.32 0.50 18.989 9999.000 9999.000 3.449 9999.000 9999.000 64135 3.82 0.51 18.830 6.329 12.501 3.456 2.036 1.420 64205 3.78 0.51 18.843 9999.000 9999.000 3.456 9999.000 9999.000 64345 3.27 0.50 19.002 9999.000 9999.000 3.448 9999.000 9999.000 64415 3.65 0.51 18.884 5.950 12.933 3.454 1.990 1.464 64485 3.65 0.51 18.884 9999.000 9999.000 3.454 9999.000 9999.000 64555 3.82 0.51 18.830 5.762 13.068 3.456 1.953 1.503 64625 3.86 0.51 18.816 9999.000 9999.000 3.457 9999.000 9999.000 64695 3.57 0.50 18.910 5.462 13.448 3.453 1.905 1.548 64765 3.65 0.51 18.884 9999.000 9999.000 3.454 9999.000 9999.000 64905 4.16 0.47 18.721 9999.000 9999.000 3.460 9999.000 9999.000 64975 4.60 0.48 18.585 2.976 15.609 3.463 1.474 1.989 65045 4.34 0.48 18.667 9999.000 9999.000 3.462 9999.000 9999.000 65185 3.99 0.51 18.776 9999.000 9999.000 3.458 9999.000 9999.000 65255 4.12 0.47 18.735 2.962 15.773 3.460 1.455 2.005 65325 3.95 0.51 18.789 9999.000 9999.000 3.458 9999.000 9999.000 65465 4.21 0.48 18.708 9999.000 9999.000 3.461 9999.000 9999.000 65535 3.95 0.51 18.789 3.658 15.131 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