80 1001 Shetter, Rick NCAR Photolysis Frequency SOLVE 1 1 2000 03 08 2000 07 19 0 Time (# of seconds after midnight) 19 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 J[O3 -> O2 + O(1D)](1/sec) J[NO2 -> NO + O(3P)](1/sec) J[H2O2 -> 2 OH](1/sec) J[HNO2 -> OH + NO](1/sec) J[HNO3 -> OH + NO2](1/sec) J[CH2O -> H + HCO](1/sec) J[CH2O -> H2 + CO](1/sec) J[CH3COCH3](1/sec) J[CH3OOH -> CH3O + OH](1/sec) J[CH3ONO2 -> CH3O+NO2](1/sec) J[PAN + hv -> products](1/sec) J[ClONO2 + hv -> Cl + NO3](1/sec) J[ClONO2 + hv -> ClO + NO2](1/sec) J[BrONO2 + hv -> Br + NO3](1/sec) J[BrONO2 + hv -> BrO + NO2](1/sec) J[CH3CH2ONO2 + hv -> Products](1/sec) J[BrCl + hv --> Br + Cl](1/sec) J[HOCl + hv --> HO + Cl](1/sec) J[HOBr + hv --> HO + Br](1/sec) 0 41 o The quantities reported in this file are the total photolysis frequencies (or photolysis rate coefficients, or J-values) of 19 photolysis reactions, calculated by combining direct measurements of the solar actinic flux with tabulated data for the molecular absorption cross section and dissociation quantum yield of each reaction. o The instruments used to measure the total solar actinic flux are the NCAR Scanning Actinic Flux Spectroradiometers (SAFS). o The time reported for each record is the start of the 20 seconds scan. The individual reactions have different sampling intervals and different midpoints around which these intervals are centered. o All data points taken are included, i.e. no outlier screening or smoothing has been applied to these data. o For each reaction, a Limit of Detection (LOD) was computed as the average j-value + twice the standard deviation during a dark data period (after sunset and before sunrise). In the final processing, j-values below the LOD were artificially set equal to the LOD for that reaction. o A preliminary estimate of the instrumental uncertainty of the spectroradiometer technique is approximately 10% (dependent on spectral range and molecular data). o A list of Quantum Yield and Cross Section data used in the computation of each Photolysis Reaction follows. Also reported is the LOD estimated for that reaction. REACTION XSxQY LOD J[O3 -> O2 + O(1D)] (xs:WMO85+Molina/qy:Talukdar98) 1.23E-008 J[NO2 -> NO + O(3P)] (xs:JPL94/qy:Gardiner) 2.58E-007 J[H2O2 -> 2 OH] (xs:JPL97/qy:1) 5.55E-010 J[HNO2 -> OH + NO] (xs:JPL97/qy:1) 6.13E-008 J[HNO3 -> OH + NO2] (xs:Burkholder93/qy:1) 9.22E-011 J[CH2O -> H + HCO] (xs:NCAR/qy:Madronich91) 3.28E-009 J[CH2O -> H2 + CO] (xs:NCAR/qy:Madronich91) 3.22E-009 J[CH3COCH3] (xs:Martinez91/qy:McKeen97) 4.39E-010 J[CH3OOH -> CH3O + OH] (xs:IUPAC97/qy:1) 4.48E-010 J[CH3ONO2 -> CH3O+NO2] (xs:Talukdar97/qy:1) 1.12E-010 J[PAN + hv -> products] (xs:Talukdar95/qy:1) 5.12E-011 J[ClONO2 + hv -> Cl + NO3] (xs:JPL97/qy:JPL97) 1.65E-009 J[ClONO2 + hv -> ClO + NO2] (xs:JPL97/qy:JPL97) 6.80E-010 J[BrONO2 + hv -> Br + NO3] (xs:JPL97/qy:JPL97) 1.44E-008 J[BrONO2 + hv -> BrO + NO2] (xs:JPL97/qy:JPL97) 3.52E-008 J[CH3CH2ONO2 + hv -> Products] (xs:Talukdar97/qy:1) 1.71E-010 J[BrCl + hv --> Br + Cl] (xs:Maric et al./qy:1) 2.46E-007 J[HOCl + hv --> HO + Cl] (xs:Burkholder/qy:1) 1.50E-008 J[HOBr + hv --> HO + Br] (xs:Ingham et al./qy:1) 7.54E-008 o For any question. please contact the Principal Investigator Rick Shetter (shetter@ucar.edu) or the ARIM data manager Luca Cinquini (luca@ucar.edu). 29600 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 29620 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 29660 1.251e-006 2.732e-003 1.233e-006 5.900e-004 5.993e-008 5.122e-006 1.130e-005 4.757e-008 1.105e-006 7.854e-008 9.019e-008 1.009e-005 1.265e-006 1.142e-004 2.797e-004 1.342e-007 3.667e-003 6.000e-005 7.129e-004 29680 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 29700 1.212e-006 2.680e-003 1.205e-006 5.791e-004 5.806e-008 4.941e-006 1.103e-005 4.572e-008 1.080e-006 7.599e-008 8.780e-008 9.876e-006 1.233e-006 1.113e-004 2.725e-004 1.299e-007 3.548e-003 5.881e-005 6.928e-004 29720 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 9999.0 29740 1.276e-006 2.623e-003 1.208e-006 5.711e-004 5.887e-008 4.984e-006 1.103e-005 4.675e-008 1.081e-006 7.713e-008 8.838e-008 9.737e-006 1.238e-006 1.090e-004 2.669e-004 1.317e-007 3.439e-003 5.854e-005 6.775e-004 29760 1.313e-006 2.615e-003 1.206e-006 5.693e-004 5.915e-008 4.974e-006 1.099e-005 4.733e-008 1.078e-006 7.753e-008 8.841e-008 9.710e-006 1.237e-006 1.086e-004 2.658e-004 1.323e-007 3.425e-003 5.835e-005 6.743e-004 29780 1.324e-006 2.655e-003 1.221e-006 5.778e-004 5.980e-008 5.032e-006 1.118e-005 4.777e-008 1.092e-006 7.838e-008 8.943e-008 9.838e-006 1.252e-006 1.097e-004 2.686e-004 1.338e-007 3.450e-003 5.913e-005 6.810e-004 29800 1.315e-006 2.643e-003 1.220e-006 5.770e-004 5.978e-008 5.044e-006 1.115e-005 4.774e-008 1.091e-006 7.835e-008 8.936e-008 9.815e-006 1.251e-006 1.095e-004 2.682e-004 1.338e-007 3.441e-003 5.909e-005 6.796e-004 29820 1.346e-006 2.645e-003 1.233e-006 5.786e-004 6.046e-008 5.081e-006 1.124e-005 4.842e-008 1.102e-006 7.924e-008 9.030e-008 9.846e-006 1.264e-006 1.096e-004 2.682e-004 1.352e-007 3.425e-003 5.952e-005 6.793e-004 29840 1.318e-006 2.607e-003 1.215e-006 5.695e-004 5.970e-008 5.012e-006 1.107e-005 4.777e-008 1.086e-006 7.829e-008 8.910e-008 9.707e-006 1.246e-006 1.081e-004 2.645e-004 1.336e-007 3.381e-003 5.861e-005 6.697e-004 29860 1.322e-006 2.602e-003 1.214e-006 5.685e-004 5.960e-008 4.988e-006 1.101e-005 4.769e-008 1.084e-006 7.815e-008 8.897e-008 9.688e-006 1.245e-006 1.077e-004 2.637e-004 1.334e-007 3.366e-003 5.853e-005 6.674e-004 29880 1.312e-006 2.602e-003 1.215e-006 5.699e-004 5.963e-008 5.026e-006 1.108e-005 4.764e-008 1.086e-006 7.818e-008 8.910e-008 9.700e-006 1.247e-006 1.079e-004 2.641e-004 1.334e-007 3.371e-003 5.865e-005 6.685e-004 29900 1.324e-006 2.614e-003 1.217e-006 5.715e-004 5.968e-008 5.017e-006 1.110e-005 4.775e-008 1.088e-006 7.822e-008 8.915e-008 9.725e-006 1.248e-006 1.082e-004 2.650e-004 1.335e-007 3.384e-003 5.876e-005 6.708e-004 29920 1.354e-006 2.682e-003 1.253e-006 5.871e-004 6.142e-008 5.185e-006 1.143e-005 4.911e-008 1.120e-006 8.049e-008 9.170e-008 9.986e-006 1.284e-006 1.108e-004 2.713e-004 1.374e-007 3.449e-003 6.047e-005 6.856e-004 29940 1.348e-006 2.670e-003 1.249e-006 5.851e-004 6.125e-008 5.176e-006 1.142e-005 4.898e-008 1.117e-006 8.024e-008 9.138e-008 9.940e-006 1.281e-006 1.102e-004 2.697e-004 1.369e-007 3.421e-003 6.031e-005 6.812e-004 29960 1.343e-006 2.658e-003 1.243e-006 5.829e-004 6.095e-008 5.130e-006 1.129e-005 4.885e-008 1.112e-006 7.982e-008 9.082e-008 9.892e-006 1.274e-006 1.097e-004 2.685e-004 1.362e-007 3.403e-003 6.005e-005 6.781e-004 29980 1.351e-006 2.646e-003 1.250e-006 5.806e-004 6.131e-008 5.195e-006 1.142e-005 4.912e-008 1.116e-006 8.030e-008 9.134e-008 9.869e-006 1.280e-006 1.091e-004 2.670e-004 1.370e-007 3.368e-003 6.013e-005 6.732e-004 30000 1.363e-006 2.632e-003 1.248e-006 5.783e-004 6.147e-008 5.173e-006 1.131e-005 4.939e-008 1.114e-006 8.055e-008 9.135e-008 9.828e-006 1.280e-006 1.084e-004 2.653e-004 1.374e-007 3.338e-003 5.998e-005 6.685e-004 30020 1.365e-006 2.620e-003 1.247e-006 5.763e-004 6.148e-008 5.186e-006 1.136e-005 4.940e-008 1.114e-006 8.057e-008 9.132e-008 9.797e-006 1.279e-006 1.079e-004 2.642e-004 1.374e-007 3.315e-003 5.991e-005 6.654e-004 30040 1.382e-006 2.616e-003 1.252e-006 5.772e-004 6.189e-008 5.207e-006 1.138e-005 4.989e-008 1.118e-006 8.110e-008 9.168e-008 9.790e-006 1.285e-006 1.077e-004 2.636e-004 1.383e-007 3.298e-003 6.004e-005 6.633e-004 30060 1.374e-006 2.607e-003 1.253e-006 5.750e-004 6.188e-008 5.218e-006 1.137e-005 4.982e-008 1.118e-006 8.106e-008 9.166e-008 9.767e-006 1.285e-006 1.074e-004 2.630e-004 1.383e-007 3.288e-003 6.002e-005 6.621e-004 30080 1.423e-006 2.631e-003 1.275e-006 5.795e-004 6.335e-008 5.351e-006 1.160e-005 5.127e-008 1.136e-006 8.299e-008 9.331e-008 9.873e-006 1.308e-006 1.084e-004 2.655e-004 1.414e-007 3.307e-003 6.084e-005 6.669e-004 30100 1.434e-006 2.613e-003 1.290e-006 5.812e-004 6.424e-008 5.409e-006 1.170e-005 5.199e-008 1.149e-006 8.421e-008 9.456e-008 9.857e-006 1.325e-006 1.077e-004 2.637e-004 1.435e-007 3.249e-003 6.136e-005 6.628e-004 30120 1.429e-006 2.658e-003 1.287e-006 5.875e-004 6.387e-008 5.375e-006 1.171e-005 5.167e-008 1.148e-006 8.367e-008 9.412e-008 9.974e-006 1.320e-006 1.096e-004 2.683e-004 1.426e-007 3.336e-003 6.150e-005 6.737e-004 30140 1.479e-006 2.671e-003 1.318e-006 5.947e-004 6.565e-008 5.515e-006 1.196e-005 5.324e-008 1.174e-006 8.603e-008 9.651e-008 1.008e-005 1.353e-006 1.091e-004 2.671e-004 1.466e-007 3.263e-003 6.268e-005 6.673e-004 30160 1.341e-006 2.244e-003 1.193e-006 5.062e-004 5.963e-008 5.038e-006 1.083e-005 4.838e-008 1.055e-006 7.817e-008 8.751e-008 8.638e-006 1.223e-006 9.278e-005 2.272e-004 1.331e-007 2.704e-003 5.550e-005 5.680e-004 30180 1.168e-006 2.037e-003 1.047e-006 4.483e-004 5.219e-008 4.409e-006 9.544e-006 4.236e-008 9.244e-007 6.837e-008 7.662e-008 7.776e-006 1.071e-006 8.590e-005 2.103e-004 1.165e-007 2.614e-003 4.880e-005 5.280e-004 30200 1.213e-006 2.211e-003 1.084e-006 4.912e-004 5.403e-008 4.572e-006 9.849e-006 4.394e-008 9.669e-007 7.073e-008 7.918e-008 8.291e-006 1.112e-006 9.024e-005 2.209e-004 1.205e-007 2.717e-003 5.169e-005 5.548e-004 30220 1.148e-006 2.143e-003 1.039e-006 4.740e-004 5.173e-008 4.411e-006 9.407e-006 4.206e-008 9.286e-007 6.767e-008 7.569e-008 7.993e-006 1.066e-006 8.737e-005 2.139e-004 1.153e-007 2.647e-003 4.966e-005 5.374e-004 30240 1.162e-006 2.124e-003 1.017e-006 4.702e-004 5.071e-008 4.247e-006 9.289e-006 4.169e-008 9.124e-007 6.630e-008 7.407e-008 7.914e-006 1.044e-006 8.719e-005 2.135e-004 1.129e-007 2.675e-003 4.892e-005 5.398e-004 30260 1.118e-006 2.077e-003 1.005e-006 4.591e-004 4.996e-008 4.216e-006 9.135e-006 4.078e-008 8.992e-007 6.532e-008 7.300e-008 7.746e-006 1.030e-006 8.519e-005 2.086e-004 1.113e-007 2.594e-003 4.811e-005 5.252e-004 30280 1.109e-006 2.070e-003 9.830e-007 4.546e-004 4.885e-008 4.135e-006 8.949e-006 4.002e-008 8.812e-007 6.383e-008 7.142e-008 7.680e-006 1.008e-006 8.485e-005 2.077e-004 1.088e-007 2.604e-003 4.728e-005 5.233e-004 30300 1.149e-006 2.318e-003 1.048e-006 5.071e-004 5.096e-008 4.328e-006 9.597e-006 4.141e-008 9.457e-007 6.639e-008 7.551e-008 8.489e-006 1.071e-006 9.393e-005 2.300e-004 1.134e-007 2.914e-003 5.142e-005 5.792e-004 30320 1.197e-006 2.276e-003 1.074e-006 5.019e-004 5.307e-008 4.486e-006 9.807e-006 4.327e-008 9.640e-007 6.934e-008 7.798e-008 8.438e-006 1.101e-006 9.263e-005 2.268e-004 1.182e-007 2.827e-003 5.191e-005 5.704e-004 30340 1.091e-006 2.072e-003 9.720e-007 4.534e-004 4.832e-008 4.082e-006 8.867e-006 3.934e-008 8.712e-007 6.322e-008 7.085e-008 7.682e-006 9.980e-007 8.554e-005 2.094e-004 1.077e-007 2.664e-003 4.686e-005 5.297e-004 30360 1.101e-006 2.133e-003 9.938e-007 4.663e-004 4.919e-008 4.172e-006 9.062e-006 4.005e-008 8.925e-007 6.428e-008 7.215e-008 7.881e-006 1.019e-006 8.797e-005 2.154e-004 1.096e-007 2.748e-003 4.810e-005 5.464e-004 30380 1.091e-006 2.124e-003 9.912e-007 4.632e-004 4.895e-008 4.159e-006 9.036e-006 3.981e-008 8.891e-007 6.394e-008 7.187e-008 7.849e-006 1.015e-006 8.780e-005 2.150e-004 1.090e-007 2.750e-003 4.787e-005 5.453e-004 30400 1.100e-006 2.143e-003 9.918e-007 4.659e-004 4.905e-008 4.163e-006 9.051e-006 3.999e-008 8.905e-007 6.407e-008 7.192e-008 7.902e-006 1.017e-006 8.891e-005 2.177e-004 1.092e-007 2.811e-003 4.800e-005 5.539e-004 30420 1.102e-006 2.180e-003 9.969e-007 4.720e-004 4.918e-008 4.180e-006 9.095e-006 4.011e-008 8.962e-007 6.421e-008 7.220e-008 8.011e-006 1.022e-006 9.054e-005 2.217e-004 1.095e-007 2.877e-003 4.842e-005 5.644e-004 30440 1.091e-006 2.153e-003 9.901e-007 4.672e-004 4.891e-008 4.145e-006 9.020e-006 3.982e-008 8.898e-007 6.387e-008 7.171e-008 7.921e-006 1.015e-006 8.936e-005 2.188e-004 1.089e-007 2.835e-003 4.801e-005 5.574e-004 30460 1.107e-006 2.161e-003 9.926e-007 4.687e-004 4.911e-008 4.164e-006 9.056e-006 4.007e-008 8.917e-007 6.413e-008 7.196e-008 7.946e-006 1.018e-006 8.942e-005 2.189e-004 1.093e-007 2.825e-003 4.813e-005 5.562e-004 30480 1.110e-006 2.134e-003 9.868e-007 4.631e-004 4.901e-008 4.143e-006 8.990e-006 4.008e-008 8.857e-007 6.403e-008 7.166e-008 7.865e-006 1.012e-006 8.855e-005 2.168e-004 1.091e-007 2.801e-003 4.772e-005 5.516e-004 30500 1.087e-006 2.133e-003 9.865e-007 4.637e-004 4.880e-008 4.146e-006 9.005e-006 3.971e-008 8.856e-007 6.376e-008 7.155e-008 7.861e-006 1.011e-006 8.836e-005 2.163e-004 1.087e-007 2.789e-003 4.774e-005 5.499e-004 30520 1.090e-006 2.169e-003 9.884e-007 4.686e-004 4.887e-008 4.156e-006 9.032e-006 3.980e-008 8.885e-007 6.384e-008 7.168e-008 7.963e-006 1.014e-006 9.037e-005 2.213e-004 1.088e-007 2.892e-003 4.801e-005 5.648e-004 30540 1.106e-006 2.241e-003 9.996e-007 4.805e-004 4.934e-008 4.186e-006 9.137e-006 4.019e-008 9.001e-007 6.442e-008 7.241e-008 8.188e-006 1.025e-006 9.498e-005 2.325e-004 1.099e-007 3.148e-003 4.880e-005 6.033e-004 30560 1.343e-006 2.711e-003 1.214e-006 5.853e-004 5.988e-008 5.082e-006 1.110e-005 4.887e-008 1.096e-006 7.810e-008 8.764e-008 9.894e-006 1.245e-006 1.126e-004 2.756e-004 1.332e-007 3.594e-003 5.940e-005 7.017e-004 30580 1.354e-006 2.779e-003 1.229e-006 5.964e-004 6.032e-008 5.136e-006 1.123e-005 4.915e-008 1.111e-006 7.858e-008 8.845e-008 1.011e-005 1.259e-006 1.156e-004 2.829e-004 1.341e-007 3.736e-003 6.037e-005 7.211e-004 30600 1.685e-006 3.770e-003 1.595e-006 8.213e-004 7.612e-008 6.436e-006 1.468e-005 6.183e-008 1.460e-006 9.875e-008 1.132e-007 1.355e-005 1.628e-006 1.527e-004 3.738e-004 1.690e-007 4.838e-003 8.054e-005 9.501e-004 30620 1.678e-006 3.279e-003 1.531e-006 7.198e-004 7.522e-008 6.467e-006 1.405e-005 6.284e-008 1.382e-006 9.777e-008 1.094e-007 1.207e-005 1.565e-006 1.351e-004 3.307e-004 1.667e-007 4.182e-003 7.442e-005 8.372e-004 30640 1.507e-006 2.950e-003 1.373e-006 6.455e-004 6.758e-008 5.829e-006 1.263e-005 5.713e-008 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