25 1001 K.K. Perkins (kathy@huarp.harvard.edu), E.J. Lanzendorf, and J.G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 Harvard NO2 SOLVE 1 1 2000 03 07 2001 07 27 0 Elapsed time (sec) from 0 GMT on flight day 1 1.0 999999.9 NO2 Volume Mixing Ratio (pptv) 8 FINAL DATA Estimated Accuracy (2 sigma): +/- 20 percent Estimated Zero Offset error (2 sigma): + 35 /- 10 ppt NO2 measurements during deep vortex flights with high ClO concentrations suggest a systematic offset of ~10 to 15 ppt ppt. We recommend accounting for this offset in the analysis of SOLVE data. For more information on flight-specific errors or instrument specifics, please contact the investigators. 2 ********** FINAL DATA ********** Time NO2 25445.25 2.1 25465.25 26.9 25480.25 43.8 25490.25 52.7 25500.25 49.1 25515.25 23.0 25651.25 30.2 25666.25 40.9 25686.25 30.8 25701.25 41.8 25711.25 21.5 25721.25 36.2 25736.25 38.6 25756.25 47.7 25771.25 55.5 25841.25 34.9 25851.25 35.8 25861.25 33.9 25876.25 41.4 25896.25 35.1 25911.25 19.8 25921.25 31.2 26062.25 12.9 26077.25 11.8 26097.25 12.3 26112.25 17.9 26122.25 14.2 26132.25 15.8 26147.25 24.5 26167.25 24.2 26182.25 12.6 26192.25 16.5 26202.25 9.3 26217.25 11.6 26237.25 30.6 26252.25 17.0 26262.25 28.3 26272.25 25.6 26287.25 16.2 26307.25 18.7 26322.25 17.6 26332.25 14.3 26342.25 18.1 26473.25 12.8 26488.25 14.2 26508.25 14.4 26523.25 3.9 26533.25 10.6 26543.25 7.2 26558.25 12.0 26578.25 16.0 26593.25 14.8 26603.25 22.3 26613.25 16.9 26628.25 14.1 26648.25 15.4 26663.25 18.5 26673.25 17.1 26683.25 8.4 26698.25 23.3 26718.25 21.5 26733.25 9.8 26743.25 20.2 26753.25 29.4 26768.25 13.5 26788.25 21.7 26803.25 16.7 26813.25 14.3 26823.25 19.9 26838.25 14.5 26858.25 19.5 26873.25 25.7 26883.25 26.0 26893.25 15.6 26908.25 17.3 26928.25 9.7 26943.25 12.7 26953.25 8.9 26963.25 6.4 26978.25 20.1 26998.25 15.0 27013.25 16.4 27023.25 16.7 27033.25 12.3 27048.25 15.8 27068.25 27.5 27083.25 16.2 27093.25 15.4 27103.25 22.3 27118.25 18.3 27138.25 19.0 27153.25 18.3 27163.25 10.9 27173.25 17.4 27188.25 13.8 27208.25 17.6 27223.25 16.9 27233.25 16.1 27243.25 18.2 27258.25 22.2 27278.25 20.6 27293.25 15.4 27303.25 13.1 27313.25 16.2 27328.25 14.7 27348.25 8.6 27363.25 17.4 27373.25 21.2 27383.25 16.8 27398.25 22.0 27418.25 14.6 27433.25 17.5 27443.25 18.7 27453.25 15.3 27468.25 12.9 27488.25 12.3 27503.25 12.2 27513.25 18.0 27523.25 8.5 27538.25 12.6 27558.25 9.1 27573.25 17.9 27583.25 6.9 27593.25 13.9 27608.25 6.9 27628.25 17.3 27643.25 8.4 27653.25 11.2 27663.25 13.6 27678.25 24.8 27698.25 15.7 27713.25 27.3 27723.25 16.6 27733.25 27.3 27748.25 20.9 27768.25 21.0 27783.25 18.1 27793.25 27.0 27803.25 24.5 27818.25 26.6 27838.25 15.7 27853.25 8.2 27863.25 22.2 27873.25 15.1 27888.25 11.3 27908.25 24.9 27923.25 19.5 27933.25 22.2 27943.25 8.2 27958.25 13.0 27978.25 16.6 27993.25 9.4 28003.25 16.1 28013.25 13.9 28028.25 8.2 28048.25 14.2 28063.25 21.4 28073.25 22.3 28083.25 13.2 28098.25 18.6 28118.25 9.8 28133.25 12.9 28143.25 28.7 28153.25 15.3 28168.25 16.1 28188.25 20.6 28203.25 12.4 28213.25 11.3 28223.25 17.7 28238.25 22.8 28258.25 24.1 28273.25 23.0 28283.25 23.1 28293.25 19.0 28308.25 20.9 28328.25 11.3 28343.25 12.1 28353.25 16.1 28364.25 19.0 28378.25 8.8 28514.25 13.7 28529.25 14.6 28549.25 15.5 28564.25 12.9 28574.25 19.0 28584.25 11.6 28599.25 21.6 28619.25 9.7 28634.25 7.5 28644.25 7.3 28654.25 8.9 28669.25 13.0 28689.25 7.0 28704.25 13.8 28714.25 18.7 28724.25 11.1 28739.25 10.8 28759.25 10.2 28774.25 15.1 28784.25 18.2 28794.25 18.1 28809.25 22.9 28829.25 16.1 28844.25 13.7 28854.25 18.3 28864.25 17.4 28879.25 15.8 28899.25 17.9 28914.25 23.4 28924.25 21.3 28934.25 14.8 28949.25 18.9 28969.25 14.2 28984.25 10.8 28994.25 11.1 29004.25 15.4 29019.25 17.2 29039.25 16.9 29054.25 20.8 29064.25 17.7 29074.25 16.6 29089.25 22.4 29109.25 10.0 29124.25 17.7 29134.25 12.9 29144.25 14.6 29159.25 21.7 29179.25 18.5 29194.25 5.3 29204.25 18.7 29214.25 15.0 29229.25 14.1 29249.25 11.1 29264.25 14.0 29274.25 8.1 29284.25 12.7 29299.25 8.6 29319.25 14.0 29334.25 11.8 29344.25 20.6 29354.25 11.0 29369.25 15.1 29389.25 6.8 29404.25 13.2 29414.25 8.6 29424.25 15.4 29439.25 21.6 29459.25 9.1 29474.25 18.7 29484.25 18.9 29494.25 21.2 29509.25 15.3 29530.25 13.5 29544.25 10.7 29554.25 14.0 29564.25 11.1 29579.25 12.6 29599.25 19.0 29614.25 7.8 29624.25 20.1 29634.25 3.1 29649.25 13.0 29669.25 6.2 29684.25 23.4 29694.25 22.9 29704.25 7.2 29719.25 12.5 29739.25 19.8 29754.25 18.8 29764.25 12.6 29774.25 11.2 29789.25 15.7 29809.25 10.2 29824.25 13.1 29834.25 15.5 29844.25 12.8 29859.25 9.2 29879.25 15.5 29894.25 22.0 29904.25 17.7 29914.25 10.2 29929.25 15.5 29949.25 24.8 29964.25 16.6 29974.25 12.2 29984.25 18.9 29999.25 10.4 30019.25 10.1 30034.25 21.4 30044.25 15.7 30054.25 16.4 30069.25 10.8 30089.25 14.5 30104.25 30.9 30114.25 12.3 30124.25 20.0 30139.25 17.0 30159.25 22.1 30174.25 11.4 30184.25 15.9 30194.25 15.5 30209.25 12.6 30229.25 18.6 30244.25 19.6 30254.25 17.4 30264.25 14.8 30279.25 22.1 30299.25 22.6 30314.25 14.4 30324.25 26.1 30334.25 9.8 30349.25 25.3 30369.25 16.0 30384.25 13.7 30394.25 16.3 30404.25 8.5 30419.25 23.2 30439.25 17.7 30454.25 23.7 30464.25 22.0 30474.25 21.8 30489.25 17.7 30509.25 14.3 30524.25 20.1 30534.25 14.6 30544.25 11.9 30559.25 21.0 30579.25 10.9 30594.25 8.4 30604.25 13.9 30614.25 8.9 30629.25 12.9 30765.25 14.9 30780.25 22.8 30800.25 27.2 30815.25 18.6 30825.25 16.8 30835.25 20.8 30851.25 17.8 30870.25 5.6 30885.25 13.9 30895.25 18.2 30905.25 19.3 30920.25 21.6 30940.25 17.2 30955.25 19.9 30965.25 16.3 30975.25 24.4 30990.25 22.5 31010.25 11.0 31025.25 15.5 31035.25 18.7 31045.25 21.5 31060.25 19.6 31095.25 11.9 31105.25 24.7 31115.25 14.5 31130.25 19.4 31150.25 19.5 31165.25 23.4 31175.25 15.7 31185.25 9.3 31200.25 9.2 31220.25 23.6 31235.25 21.0 31245.25 24.9 31255.25 15.3 31270.25 5.8 31290.25 12.3 31305.25 17.0 31315.25 15.8 31325.25 1.9 31340.25 10.2 31360.25 16.7 31375.25 18.4 31385.25 17.5 31395.25 13.0 31410.25 12.1 31430.25 14.1 31445.25 9.9 31455.25 7.6 31465.25 18.4 31480.25 16.8 31500.25 11.4 31515.25 15.0 31525.25 13.0 31535.25 13.2 31550.25 17.6 31570.25 19.2 31585.25 11.7 31595.25 13.8 31605.25 14.6 31620.25 18.0 31640.25 14.4 31655.25 12.4 31665.25 19.9 31675.25 9.9 31690.25 16.7 31710.25 17.7 31725.25 18.4 31735.25 12.2 31745.25 9.4 31760.25 13.6 31780.25 15.9 31795.25 6.3 31805.25 15.7 31815.25 14.7 31830.25 10.5 31850.25 15.8 31866.25 10.6 31876.25 18.9 31885.25 19.4 31900.25 12.5 31920.25 20.5 31935.25 21.3 31945.25 19.0 31955.25 15.9 31970.25 16.7 31990.25 12.6 32005.25 19.6 32016.25 16.5 32025.25 17.6 32040.25 20.5 32060.25 18.8 32075.25 14.1 32085.25 17.3 32095.25 19.4 32110.25 21.4 32130.25 17.6 32145.25 16.9 32155.25 29.1 32165.25 17.6 32180.25 18.8 32200.25 10.6 32215.25 16.3 32225.25 17.2 32235.25 16.1 32250.25 13.4 32270.25 18.7 32285.25 11.0 32295.25 6.9 32305.25 11.6 32320.25 19.1 32340.25 16.0 32355.25 15.9 32365.25 24.6 32375.25 18.0 32390.25 23.3 32410.25 22.7 32425.25 15.3 32435.25 18.3 32445.25 18.2 32460.25 18.6 32480.25 22.7 32495.25 23.6 32505.25 26.2 32515.25 17.1 32530.25 32.8 32550.25 18.6 32565.25 19.4 32575.25 19.8 32585.25 20.3 32600.25 27.9 32620.25 30.1 32635.25 25.0 32645.25 17.1 32655.25 24.9 32670.25 22.7 32806.25 18.1 32821.25 17.9 32841.25 24.9 32856.25 17.5 32866.25 17.8 32876.25 22.1 32891.25 26.9 32911.25 15.8 32926.25 16.8 32936.25 20.8 32946.25 8.5 32961.25 12.2 32981.25 15.8 32996.25 11.3 33006.25 13.3 33016.25 13.7 33031.25 16.2 33051.25 8.7 33066.25 17.2 33076.25 11.2 33086.25 9.7 33101.25 9.7 33121.25 11.4 33136.25 7.2 33146.25 10.2 33156.25 7.2 33171.25 19.7 33192.25 17.3 33206.25 17.9 33216.25 18.0 33226.25 15.6 33241.25 16.5 33261.25 17.6 33276.25 20.7 33286.25 20.0 33296.25 19.0 33311.25 20.9 33331.25 17.1 33346.25 10.7 33356.25 16.7 33366.25 19.3 33381.25 13.1 33401.25 23.3 33416.25 13.2 33426.25 15.2 33436.25 20.4 33451.25 11.9 33471.25 26.0 33487.25 14.2 33496.25 12.0 33506.25 14.6 33522.25 19.5 33542.25 7.7 33556.25 15.4 33567.25 15.6 33576.25 14.0 33591.25 8.9 33612.25 13.5 33627.25 10.1 33637.25 9.9 33647.25 6.6 33661.25 16.9 33681.25 11.1 33696.25 5.7 33707.25 -2.3 33717.25 6.8 33732.25 7.2 33752.25 7.5 33767.25 9.0 33777.25 10.2 33787.25 21.5 33802.25 10.3 33822.25 8.7 33837.25 12.3 33847.25 7.5 33857.25 13.4 33872.25 6.9 33892.25 6.5 33906.25 6.2 33917.25 5.8 33927.25 19.2 33942.25 7.9 33962.25 10.2 33977.25 8.7 33987.25 11.2 33997.25 11.0 34012.25 5.9 34032.25 10.8 34047.25 13.2 34057.25 10.4 34067.25 11.4 34082.25 10.3 34102.25 8.4 34117.25 10.5 34127.25 12.7 34137.25 12.4 34152.25 19.5 34172.25 13.1 34187.25 14.0 34197.25 13.8 34208.25 7.4 34222.25 13.5 34242.25 11.1 34257.25 9.6 34267.25 14.9 34277.25 8.5 34292.25 15.4 34312.25 15.7 34327.25 5.3 34337.25 13.6 34348.25 12.4 34362.25 12.6 34382.25 12.5 34397.25 12.3 34407.25 12.6 34417.25 15.5 34432.25 17.4 34452.25 0.6 34467.25 12.5 34477.25 17.0 34487.25 9.9 34502.25 12.1 34522.25 14.5 34537.25 15.0 34547.25 24.4 34557.25 21.9 34572.25 18.4 34592.25 19.8 34607.25 19.9 34617.25 16.0 34627.25 16.7 34642.25 15.6 34662.25 14.3 34677.25 17.4 34687.25 16.1 34697.25 11.0 34712.25 12.7 34732.25 18.0 34747.25 15.7 34757.25 10.9 34767.25 17.5 34782.25 19.6 34802.25 13.2 34817.25 19.0 34827.25 11.3 34837.25 18.7 34852.25 15.9 34872.25 19.5 34887.25 17.7 34897.25 13.6 34907.25 14.7 34922.25 15.7 35058.25 17.9 35073.25 8.9 35093.25 21.5 35108.25 13.4 35118.25 17.6 35128.25 18.1 35143.25 13.6 35163.25 20.2 35178.25 19.7 35188.25 11.5 35198.25 20.6 35213.25 16.3 35233.25 21.6 35248.25 15.6 35258.25 14.8 35268.25 17.4 35283.25 12.9 35303.25 26.5 35318.25 20.3 35328.25 13.3 35338.25 17.2 35353.25 14.8 35374.25 22.1 35388.25 17.1 35398.25 19.4 35408.25 7.8 35423.25 18.6 35443.25 21.8 35458.25 19.8 35468.25 19.0 35478.25 19.3 35493.25 10.3 35514.25 11.8 35529.25 16.5 35538.25 18.4 35548.25 14.8 35563.25 12.3 35583.25 11.4 35598.25 12.0 35608.25 7.1 35618.25 14.0 35633.25 20.7 35653.25 7.8 35668.25 12.8 35678.25 20.8 35688.25 14.2 35703.25 15.6 35723.25 15.0 35738.25 21.8 35748.25 20.8 35758.25 10.1 35773.25 17.8 35793.25 22.9 35808.25 15.9 35818.25 14.2 35828.25 25.7 35843.25 22.8 35863.25 23.8 35878.25 11.0 35888.25 18.0 35898.25 11.9 35913.25 14.9 35933.25 18.8 35948.25 48.5 35963.25 19.3 35983.25 20.9 36003.25 14.8 36018.25 12.8 36028.25 19.3 36038.25 12.3 36053.25 11.6 36073.25 7.1 36088.25 9.7 36098.25 15.1 36108.25 10.4 36123.25 13.8 36143.25 17.5 36158.25 13.1 36168.25 15.8 36178.25 14.1 36193.25 17.0 36213.25 15.1 36228.25 8.0 36238.25 18.2 36248.25 20.5 36263.25 10.0 36283.25 13.0 36298.25 14.6 36308.25 7.1 36318.25 12.9 36333.25 9.0 36353.25 15.4 36368.25 20.1 36378.25 6.9 36388.25 21.7 36403.25 12.3 36423.25 14.5 36438.25 6.3 36448.25 14.8 36458.25 12.4 36473.25 11.8 36493.25 9.0 36508.25 7.1 36518.25 9.4 36543.25 14.5 36563.25 15.1 36578.25 14.4 36588.25 13.9 36598.25 22.0 36613.25 12.3 36633.25 18.4 36648.25 16.6 36658.25 11.5 36668.25 10.3 36684.25 28.3 36703.25 11.8 36718.25 19.3 36728.25 18.1 36738.25 12.2 36753.25 12.3 36773.25 18.9 36788.25 13.4 36798.25 16.4 36808.25 19.8 36823.25 12.0 36843.25 12.9 36858.25 22.4 36868.25 16.6 36878.25 13.6 36893.25 10.6 36913.25 8.1 36928.25 16.0 36938.25 14.1 36948.25 18.2 36963.25 13.3 37099.25 17.1 37114.25 14.6 37134.25 9.8 37149.25 16.0 37159.25 25.1 37169.25 15.7 37184.25 13.8 37204.25 15.9 37219.25 20.0 37229.25 19.2 37239.25 17.6 37254.25 12.5 37274.25 14.9 37289.25 12.3 37299.25 16.8 37309.25 12.1 37324.25 19.4 37344.25 17.1 37359.25 21.4 37369.25 16.9 37379.25 18.7 37394.25 13.3 37414.25 17.3 37429.25 17.8 37439.25 19.9 37449.25 15.3 37464.25 16.0 37484.25 19.8 37499.25 11.3 37509.25 16.4 37519.25 13.5 37534.25 26.2 37554.25 17.9 37569.25 11.9 37579.25 15.4 37589.25 20.9 37604.25 13.8 37624.25 8.4 37639.25 9.1 37649.25 10.7 37659.25 18.8 37674.25 12.6 37694.25 15.4 37709.25 20.0 37719.25 19.2 37729.25 25.3 37744.25 11.3 37764.25 13.6 37779.25 16.1 37789.25 17.1 37799.25 15.7 37814.25 12.5 37834.25 20.5 37850.25 18.7 37860.25 20.8 37869.25 17.8 37884.25 17.2 37904.25 15.4 37919.25 17.0 37929.25 14.5 37939.25 15.4 37954.25 16.3 37974.25 17.9 37989.25 13.6 37999.25 19.7 38009.25 10.4 38024.25 22.1 38044.25 19.1 38059.25 23.4 38069.25 17.0 38079.25 18.1 38094.25 25.1 38114.25 16.7 38129.25 21.9 38139.25 20.5 38149.25 13.8 38164.25 17.9 38184.25 12.9 38199.25 21.0 38209.25 15.8 38219.25 17.4 38234.25 14.8 38254.25 13.2 38269.25 11.4 38279.25 15.4 38289.25 17.6 38304.25 13.2 38324.25 13.7 38339.25 18.2 38349.25 8.9 38359.25 17.9 38374.25 26.4 38394.25 13.5 38409.25 16.4 38419.25 15.2 38429.25 10.5 38444.25 12.8 38464.25 11.6 38479.25 20.6 38489.25 17.6 38499.25 18.3 38514.25 19.4 38534.25 23.5 38549.25 19.7 38559.25 24.6 38569.25 18.9 38584.25 27.2 38604.25 22.7 38619.25 18.2 38629.25 21.3 38639.25 22.2 38654.25 15.8 38674.25 14.0 38689.25 12.9 38699.25 18.1 38709.25 6.2 38724.25 13.0 38744.25 11.6 38759.25 22.8 38769.25 19.5 38779.25 13.8 38794.25 14.7 38814.25 25.4 38829.25 20.3 38839.25 16.4 38849.25 18.0 38864.25 21.6 38884.25 17.9 38899.25 21.6 38909.25 14.9 38919.25 12.7 38934.25 20.8 38954.25 25.5 38969.25 22.7 38979.25 19.9 38989.25 16.8 39004.25 16.3 39025.25 16.8 39039.25 15.1 39049.25 13.9 39059.25 12.7 39074.25 13.7 39094.25 8.4 39109.25 14.4 39119.25 14.9 39129.25 8.8 39144.25 18.4 39164.25 12.3 39179.25 11.5 39189.25 9.8 39199.25 13.0 39214.25 17.9 39350.25 7.4 39365.25 10.7 39385.25 13.1 39400.25 14.4 39410.25 14.6 39420.25 17.8 39435.25 17.8 39455.25 23.3 39470.25 18.4 39480.25 22.1 39490.25 12.9 39505.25 17.1 39525.25 19.2 39540.25 16.4 39550.25 24.8 39560.25 17.7 39575.25 20.0 39595.25 16.0 39610.25 19.5 39620.25 15.4 39630.25 22.2 39645.25 15.6 39665.25 19.8 39680.25 18.0 39690.25 21.7 39700.25 18.2 39715.25 18.1 39735.25 16.9 39750.25 19.1 39760.25 20.6 39770.25 22.8 39785.25 20.4 39805.25 12.4 39820.25 22.7 39830.25 16.3 39840.25 23.0 39855.25 16.4 39875.25 24.5 39890.25 24.4 39900.25 18.5 39910.25 27.2 39925.25 19.6 39945.25 20.2 39960.25 12.9 39970.25 29.7 39980.25 14.8 39995.25 21.4 40015.25 17.7 40030.25 24.5 40040.25 18.1 40050.25 12.6 40065.25 23.6 40085.25 18.1 40100.25 19.4 40110.25 21.1 40120.25 28.1 40135.25 16.6 40155.25 21.2 40170.25 16.5 40180.25 17.2 40191.25 31.3 40205.25 20.5 40225.25 19.2 40240.25 18.5 40250.25 8.6 40260.25 21.4 40275.25 20.0 40295.25 11.1 40310.25 20.2 40320.25 14.5 40330.25 13.1 40345.25 19.2 40365.25 15.9 40380.25 19.1 40390.25 13.0 40400.25 17.5 40415.25 16.4 40435.25 19.0 40450.25 20.3 40460.25 18.6 40470.25 11.1 40485.25 21.3 40505.25 20.4 40520.25 25.1 40530.25 21.5 40540.25 22.9 40555.25 28.8 40575.25 23.0 40590.25 12.9 40600.25 14.2 40610.25 17.7 40625.25 16.6 40645.25 10.7 40660.25 18.1 40670.25 14.6 40680.25 14.1 40695.25 19.5 40715.25 18.1 40730.25 16.6 40740.25 19.2 40750.25 13.0 40765.25 11.0 40785.25 11.2 40800.25 26.2 40810.25 21.1 40820.25 22.2 40835.25 16.4 40855.25 17.6 40870.25 19.0 40880.25 20.5 40890.25 21.8 40905.25 23.3 40925.25 24.3 40940.25 20.4 40950.25 18.6 40960.25 28.8 40975.25 18.2 40995.25 16.4 41010.25 14.0 41020.25 20.9 41030.25 15.5 41045.25 17.8 41065.25 13.4 41080.25 19.4 41090.25 23.0 41100.25 17.6 41115.25 17.4 41135.25 13.2 41150.25 20.4 41160.25 17.8 41170.25 25.0 41185.25 13.5 41205.25 19.6 41220.25 28.5 41230.25 17.2 41240.25 15.5 41255.25 18.7 41391.25 22.2 41406.25 16.3 41426.25 17.1 41441.25 18.1 41451.25 15.0 41461.25 21.1 41476.25 20.8 41496.25 15.9 41511.25 18.0 41521.25 13.3 41531.25 11.7 41546.25 11.6 41566.25 11.4 41581.25 12.1 41591.25 10.0 41601.25 14.4 41616.25 14.0 41636.25 13.1 41651.25 7.5 41661.25 11.9 41671.25 12.7 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