44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 03 07 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 24908.25 4.0 999999.9 999999.9 24943.25 -18.3 999999.9 999999.9 24978.25 5.2 999999.9 999999.9 25013.25 5.0 999999.9 999999.9 25048.25 12.0 999999.9 999999.9 25083.25 15.0 999999.9 999999.9 25118.25 1.0 999999.9 999999.9 25153.25 -13.2 999999.9 999999.9 25188.25 -11.5 999999.9 999999.9 25223.25 12.9 999999.9 999999.9 25258.25 -0.3 999999.9 999999.9 25293.25 2.5 999999.9 999999.9 25328.25 -5.0 999999.9 999999.9 25363.25 18.7 999999.9 999999.9 25398.25 22.3 999999.9 999999.9 25433.25 12.9 999999.9 999999.9 25468.25 21.1 999999.9 999999.9 25503.25 23.6 999999.9 999999.9 25538.25 42.2 999999.9 999999.9 25573.25 49.1 999999.9 999999.9 25608.25 42.0 999999.9 999999.9 25643.25 73.4 999999.9 999999.9 25678.25 71.2 999999.9 999999.9 25713.25 84.4 999999.9 999999.9 25748.25 83.7 999999.9 999999.9 25783.25 115.8 999999.9 999999.9 25818.25 174.6 999999.9 999999.9 25853.25 187.8 999999.9 999999.9 25888.25 189.9 999999.9 473.3 25923.25 159.7 999999.9 500.3 25958.25 145.1 999999.9 573.4 25993.25 186.4 61.2 999999.9 26028.25 232.2 67.9 999999.9 26063.25 415.1 999999.9 999999.9 26098.25 437.1 999999.9 999999.9 26133.25 402.0 999999.9 999999.9 26168.25 394.8 999999.9 999999.9 26203.25 416.6 116.5 999999.9 26238.25 450.4 114.5 999999.9 26273.25 496.1 132.5 999999.9 26308.25 484.6 999999.9 513.6 26343.25 509.8 999999.9 446.1 26378.25 535.1 999999.9 512.3 26413.25 579.6 125.3 999999.9 26448.25 654.8 146.3 999999.9 26483.25 751.8 999999.9 999999.9 26518.25 695.1 999999.9 999999.9 26553.25 731.3 999999.9 999999.9 26588.25 735.3 999999.9 999999.9 26623.25 800.5 999999.9 999999.9 26658.25 791.7 999999.9 999999.9 26693.25 807.2 999999.9 999999.9 26728.25 810.9 999999.9 999999.9 26763.25 834.7 999999.9 999999.9 26798.25 849.7 999999.9 999999.9 26833.25 861.6 999999.9 999999.9 26868.25 845.4 210.7 999999.9 26903.25 859.4 224.5 999999.9 26938.25 923.7 218.2 999999.9 26973.25 878.1 999999.9 346.5 27008.25 843.7 999999.9 380.4 27043.25 824.6 999999.9 999999.9 27078.25 845.6 193.5 999999.9 27113.25 841.4 215.2 999999.9 27148.25 875.3 999999.9 999999.9 27183.25 931.2 999999.9 999999.9 27218.25 943.2 999999.9 999999.9 27253.25 896.0 999999.9 999999.9 27288.25 857.5 221.1 999999.9 27323.25 901.5 221.5 999999.9 27358.25 941.1 225.7 999999.9 27393.25 903.1 999999.9 408.8 27428.25 876.3 999999.9 371.3 27463.25 890.1 999999.9 999999.9 27498.25 925.2 211.4 999999.9 27533.25 913.1 220.7 999999.9 27568.25 994.2 999999.9 999999.9 27603.25 973.6 999999.9 999999.9 27638.25 994.4 999999.9 999999.9 27673.25 905.0 999999.9 999999.9 27708.25 955.8 230.6 999999.9 27743.25 905.8 203.8 999999.9 27778.25 947.7 210.2 999999.9 27813.25 950.8 999999.9 364.1 27848.25 927.7 999999.9 395.1 27883.25 870.6 999999.9 999999.9 27918.25 942.6 200.8 999999.9 27953.25 925.7 239.4 999999.9 27988.25 979.5 999999.9 999999.9 28023.25 992.2 999999.9 999999.9 28058.25 956.8 999999.9 999999.9 28093.25 967.7 999999.9 999999.9 28128.25 1033.3 999999.9 999999.9 28163.25 984.2 999999.9 999999.9 28198.25 1026.3 999999.9 999999.9 28233.25 1026.1 999999.9 999999.9 28268.25 983.2 999999.9 999999.9 28303.25 1004.6 999999.9 999999.9 28338.25 978.8 999999.9 999999.9 28373.25 1040.3 259.8 999999.9 28408.25 969.5 211.9 999999.9 28443.25 940.5 231.7 999999.9 28478.25 946.5 999999.9 390.1 28513.25 955.9 999999.9 460.3 28548.25 942.3 999999.9 999999.9 28583.25 966.0 191.7 999999.9 28618.25 1014.6 222.0 999999.9 28653.25 1031.4 999999.9 999999.9 28688.25 1006.8 999999.9 999999.9 28723.25 977.4 999999.9 999999.9 28758.25 985.9 999999.9 999999.9 28793.25 982.9 245.2 999999.9 28828.25 1011.9 239.3 999999.9 28863.25 995.6 240.3 999999.9 28898.25 936.7 999999.9 403.6 28933.25 967.1 999999.9 460.9 28968.25 975.5 999999.9 999999.9 29003.25 1014.9 239.4 999999.9 29038.25 974.3 265.6 999999.9 29073.25 1052.0 999999.9 999999.9 29108.25 1025.9 999999.9 999999.9 29143.25 1021.9 999999.9 999999.9 29178.25 999.8 999999.9 999999.9 29213.25 984.6 269.0 999999.9 29248.25 998.4 259.8 999999.9 29283.25 939.4 281.0 999999.9 29318.25 921.4 999999.9 312.2 29353.25 926.4 999999.9 357.6 29388.25 947.4 999999.9 999999.9 29423.25 981.5 238.2 999999.9 29458.25 998.7 251.5 999999.9 29493.25 1070.9 999999.9 999999.9 29528.25 1062.0 999999.9 999999.9 29563.25 1075.5 999999.9 999999.9 29598.25 1002.1 999999.9 999999.9 29633.25 1132.2 999999.9 999999.9 29668.25 1104.0 999999.9 999999.9 29703.25 1053.5 999999.9 999999.9 29738.25 1103.5 999999.9 999999.9 29773.25 1074.4 999999.9 999999.9 29808.25 1025.3 999999.9 999999.9 29843.25 1074.3 999999.9 999999.9 29878.25 1012.5 301.4 999999.9 29913.25 1060.9 293.6 999999.9 29948.25 1037.5 250.9 999999.9 29983.25 1005.3 999999.9 409.4 30018.25 970.7 999999.9 471.3 30053.25 944.4 999999.9 999999.9 30088.25 924.3 206.6 999999.9 30123.25 957.3 220.9 999999.9 30158.25 958.9 999999.9 999999.9 30193.25 942.3 999999.9 999999.9 30228.25 1005.8 999999.9 999999.9 30263.25 986.9 999999.9 999999.9 30298.25 1001.4 274.1 999999.9 30333.25 961.6 253.3 999999.9 30368.25 1002.6 259.5 999999.9 30403.25 968.6 999999.9 394.0 30438.25 902.1 999999.9 438.6 30473.25 914.0 999999.9 999999.9 30508.25 946.3 231.9 999999.9 30543.25 1026.7 239.1 999999.9 30578.25 1217.5 999999.9 999999.9 30613.25 1210.2 999999.9 999999.9 30648.25 1095.5 999999.9 999999.9 30683.25 1060.9 999999.9 999999.9 30718.25 1074.7 305.7 999999.9 30753.25 1128.9 331.6 999999.9 30788.25 1118.8 323.4 999999.9 30823.25 1116.9 999999.9 204.7 30858.25 1114.5 999999.9 227.8 30893.25 1087.3 999999.9 999999.9 30928.25 1094.9 296.6 999999.9 30963.25 1092.7 287.9 999999.9 30998.25 1181.1 999999.9 999999.9 31033.25 1169.8 999999.9 999999.9 31068.25 1239.7 999999.9 999999.9 31103.25 1162.9 999999.9 999999.9 31138.25 1212.6 999999.9 999999.9 31173.25 1157.7 999999.9 999999.9 31208.25 1203.1 999999.9 999999.9 31243.25 1173.9 999999.9 999999.9 31278.25 1165.7 999999.9 999999.9 31313.25 1123.6 999999.9 999999.9 31348.25 1096.7 999999.9 999999.9 31383.25 1090.8 297.2 999999.9 31418.25 1070.5 274.0 999999.9 31453.25 1122.1 284.8 999999.9 31488.25 1070.5 999999.9 304.4 31523.25 1075.8 999999.9 378.4 31558.25 1031.3 999999.9 999999.9 31593.25 1014.5 236.2 999999.9 31628.25 976.9 242.6 999999.9 31663.25 1031.1 999999.9 999999.9 31698.25 1054.8 999999.9 999999.9 31733.25 1012.4 999999.9 999999.9 31768.25 989.9 999999.9 999999.9 31803.25 989.6 256.9 999999.9 31838.25 967.3 220.0 999999.9 31873.25 947.0 237.3 999999.9 31908.25 918.1 999999.9 392.3 31943.25 892.8 999999.9 429.8 31978.25 899.6 999999.9 999999.9 32013.25 938.1 210.6 999999.9 32048.25 925.0 215.2 999999.9 32083.25 959.7 999999.9 999999.9 32118.25 974.4 999999.9 999999.9 32153.25 923.8 999999.9 999999.9 32188.25 889.3 999999.9 999999.9 32223.25 930.3 215.8 999999.9 32258.25 992.8 249.2 999999.9 32293.25 1041.8 234.8 999999.9 32328.25 976.7 999999.9 455.1 32363.25 921.4 999999.9 435.4 32398.25 913.8 999999.9 999999.9 32433.25 978.2 225.6 999999.9 32468.25 954.3 201.5 999999.9 32503.25 979.7 999999.9 999999.9 32538.25 994.2 999999.9 999999.9 32573.25 927.2 999999.9 999999.9 32608.25 916.8 999999.9 999999.9 32643.25 905.5 999999.9 999999.9 32678.25 900.2 999999.9 999999.9 32713.25 896.8 999999.9 999999.9 32748.25 942.6 999999.9 999999.9 32783.25 928.2 999999.9 999999.9 32818.25 1037.5 999999.9 999999.9 32853.25 1061.9 999999.9 999999.9 32888.25 1050.0 256.0 999999.9 32923.25 1066.0 266.6 999999.9 32958.25 1052.3 255.5 999999.9 32993.25 1014.0 999999.9 374.3 33028.25 1027.6 999999.9 316.2 33063.25 1027.3 999999.9 999999.9 33098.25 998.4 260.7 999999.9 33133.25 942.2 230.6 999999.9 33168.25 1035.8 999999.9 999999.9 33203.25 974.8 999999.9 999999.9 33238.25 913.2 999999.9 999999.9 33273.25 815.5 999999.9 999999.9 33308.25 897.9 207.0 999999.9 33343.25 943.2 212.3 999999.9 33378.25 989.2 225.4 999999.9 33413.25 967.7 999999.9 460.2 33448.25 1027.2 999999.9 324.7 33483.25 1028.4 999999.9 999999.9 33518.25 1039.0 250.7 999999.9 33553.25 1032.4 270.3 999999.9 33588.25 1096.4 999999.9 999999.9 33623.25 1133.0 999999.9 999999.9 33658.25 1128.6 999999.9 999999.9 33693.25 1088.3 999999.9 999999.9 33728.25 1073.1 302.8 999999.9 33763.25 1096.1 299.6 999999.9 33798.25 1103.6 297.2 999999.9 33833.25 1103.6 999999.9 195.0 33868.25 1116.0 999999.9 235.9 33903.25 1066.5 999999.9 999999.9 33938.25 1112.4 293.9 999999.9 33973.25 1134.2 275.9 999999.9 34008.25 1121.6 999999.9 999999.9 34043.25 1084.0 999999.9 999999.9 34078.25 1137.9 999999.9 999999.9 34113.25 1095.8 999999.9 999999.9 34148.25 1138.0 999999.9 999999.9 34183.25 1137.2 999999.9 999999.9 34218.25 1133.3 999999.9 999999.9 34253.25 1172.6 999999.9 999999.9 34288.25 1158.7 999999.9 999999.9 34323.25 1084.0 999999.9 999999.9 34358.25 1123.0 999999.9 999999.9 34393.25 1072.5 304.4 999999.9 34428.25 1030.2 278.4 999999.9 34463.25 1049.7 263.0 999999.9 34498.25 1033.7 999999.9 373.8 34533.25 1061.6 999999.9 390.8 34568.25 1084.9 999999.9 999999.9 34603.25 1077.5 257.1 999999.9 34638.25 1081.8 288.3 999999.9 34673.25 1068.0 999999.9 999999.9 34708.25 1141.3 999999.9 999999.9 34743.25 1083.6 999999.9 999999.9 34778.25 1079.3 999999.9 999999.9 34813.25 1044.1 267.5 999999.9 34848.25 1042.1 238.2 999999.9 34883.25 976.6 272.4 999999.9 34918.25 1001.7 999999.9 284.9 34953.25 1001.1 999999.9 362.8 34988.25 1056.1 999999.9 999999.9 35023.25 958.5 243.9 999999.9 35058.25 972.3 246.8 999999.9 35093.25 1061.7 999999.9 999999.9 35128.25 1042.1 999999.9 999999.9 35163.25 1029.8 999999.9 999999.9 35198.25 1076.0 999999.9 999999.9 35233.25 1117.2 282.3 999999.9 35268.25 1075.6 280.5 999999.9 35303.25 1066.6 280.8 999999.9 35338.25 975.0 999999.9 411.0 35373.25 914.8 999999.9 420.5 35408.25 927.0 999999.9 999999.9 35443.25 965.5 235.5 999999.9 35478.25 986.6 240.8 999999.9 35513.25 992.7 999999.9 999999.9 35548.25 1049.8 999999.9 999999.9 35583.25 1054.6 999999.9 999999.9 35618.25 1058.0 999999.9 999999.9 35653.25 1112.8 999999.9 999999.9 35688.25 1002.4 999999.9 999999.9 35723.25 982.2 999999.9 999999.9 35758.25 1015.7 999999.9 999999.9 35793.25 944.1 999999.9 999999.9 35828.25 987.7 999999.9 999999.9 35863.25 960.2 999999.9 999999.9 35898.25 933.4 306.2 999999.9 35933.25 964.5 258.9 999999.9 35968.25 1039.0 258.8 999999.9 36003.25 1081.8 999999.9 359.8 36038.25 988.8 999999.9 383.5 36073.25 1049.0 999999.9 999999.9 36108.25 1101.7 269.5 999999.9 36143.25 1082.2 278.1 999999.9 36178.25 1109.2 999999.9 999999.9 36213.25 1094.3 999999.9 999999.9 36248.25 1129.5 999999.9 999999.9 36283.25 1044.4 999999.9 999999.9 36318.25 1118.1 319.4 999999.9 36353.25 1045.9 314.2 999999.9 36388.25 1072.3 319.2 999999.9 36423.25 1093.0 999999.9 239.0 36458.25 1036.6 999999.9 307.1 36493.25 1046.8 999999.9 999999.9 36528.25 1099.6 282.0 999999.9 36563.25 1101.6 293.7 999999.9 36598.25 1121.7 999999.9 999999.9 36633.25 1114.7 999999.9 999999.9 36668.25 1163.0 999999.9 999999.9 36703.25 1180.1 999999.9 999999.9 36738.25 1115.1 332.3 999999.9 36773.25 1127.8 311.7 999999.9 36808.25 1137.8 345.8 999999.9 36843.25 1108.5 999999.9 197.7 36878.25 1060.9 999999.9 311.6 36913.25 1035.9 999999.9 999999.9 36948.25 1074.9 275.0 999999.9 36983.25 1049.4 315.7 999999.9 37018.25 1100.9 999999.9 999999.9 37053.25 1119.4 999999.9 999999.9 37088.25 1113.1 999999.9 999999.9 37123.25 1137.3 999999.9 999999.9 37158.25 1197.4 999999.9 999999.9 37193.25 1155.2 999999.9 999999.9 37228.25 1228.3 999999.9 999999.9 37263.25 1231.0 999999.9 999999.9 37298.25 1169.3 999999.9 999999.9 37333.25 1134.0 999999.9 999999.9 37368.25 1124.9 999999.9 999999.9 37403.25 1115.3 320.3 999999.9 37438.25 1167.8 312.1 999999.9 37473.25 1081.0 330.0 999999.9 37508.25 1087.4 999999.9 194.0 37543.25 1096.0 999999.9 281.5 37578.25 1080.5 999999.9 999999.9 37613.25 1076.6 292.5 999999.9 37648.25 1131.7 323.4 999999.9 37683.25 1110.9 999999.9 999999.9 37718.25 1137.8 999999.9 999999.9 37753.25 1143.6 999999.9 999999.9 37788.25 1094.6 999999.9 999999.9 37823.25 1106.5 308.5 999999.9 37858.25 1120.4 310.9 999999.9 37893.25 1077.1 331.2 999999.9 37928.25 1067.9 999999.9 208.8 37963.25 1058.7 999999.9 239.9 37998.25 1124.5 999999.9 999999.9 38033.25 1094.4 324.9 999999.9 38068.25 1078.1 324.0 999999.9 38103.25 1133.3 999999.9 999999.9 38138.25 1082.2 999999.9 999999.9 38173.25 1063.0 999999.9 999999.9 38208.25 1035.5 999999.9 999999.9 38243.25 1024.6 334.4 999999.9 38278.25 1054.9 311.6 999999.9 38313.25 991.9 316.4 999999.9 38348.25 1042.5 999999.9 435.2 38383.25 1028.9 999999.9 463.2 38418.25 999.9 999999.9 999999.9 38453.25 1038.8 277.3 999999.9 38488.25 998.9 258.3 999999.9 38523.25 985.1 999999.9 999999.9 38558.25 1022.7 999999.9 999999.9 38593.25 976.7 999999.9 999999.9 38628.25 1059.6 999999.9 999999.9 38663.25 1121.1 999999.9 999999.9 38698.25 1074.1 999999.9 999999.9 38733.25 1105.4 999999.9 999999.9 38768.25 1106.5 999999.9 999999.9 38803.25 1088.5 999999.9 999999.9 38838.25 1071.8 999999.9 999999.9 38873.25 1019.0 999999.9 999999.9 38908.25 1057.4 295.4 999999.9 38943.25 1043.8 314.2 999999.9 38978.25 1032.3 306.2 999999.9 39013.25 1071.4 999999.9 273.9 39048.25 1060.8 999999.9 300.4 39083.25 1090.9 999999.9 999999.9 39118.25 1035.9 338.9 999999.9 39153.25 1022.6 321.4 999999.9 39188.25 1086.4 999999.9 999999.9 39223.25 1098.0 999999.9 999999.9 39258.25 1079.6 999999.9 999999.9 39293.25 1109.9 999999.9 999999.9 39328.25 1100.4 353.4 999999.9 39363.25 1109.7 365.6 999999.9 39398.25 1052.6 363.1 999999.9 39433.25 1041.2 999999.9 236.0 39468.25 1023.4 999999.9 286.8 39503.25 977.2 999999.9 999999.9 39538.25 993.2 289.3 999999.9 39573.25 980.6 302.5 999999.9 39608.25 1020.1 999999.9 999999.9 39643.25 984.0 999999.9 999999.9 39678.25 967.2 999999.9 999999.9 39713.25 900.1 999999.9 999999.9 39748.25 899.3 290.5 999999.9 39783.25 904.0 277.7 999999.9 39818.25 840.4 243.3 999999.9 39853.25 797.1 999999.9 656.2 39888.25 784.5 999999.9 809.6 39923.25 784.5 999999.9 999999.9 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