44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 01 27 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 32803.63 3.8 999999.9 999999.9 32838.63 0.2 999999.9 999999.9 32873.63 -0.6 999999.9 999999.9 32908.63 11.3 999999.9 999999.9 32943.63 6.1 999999.9 999999.9 32978.63 12.6 999999.9 999999.9 33013.63 -11.9 999999.9 999999.9 33048.63 2.0 999999.9 999999.9 33083.63 2.9 999999.9 999999.9 33118.63 7.1 999999.9 999999.9 33153.63 5.2 999999.9 999999.9 33188.63 8.4 999999.9 999999.9 33223.63 43.8 999999.9 999999.9 33258.63 89.5 999999.9 999999.9 33293.63 91.8 999999.9 999999.9 33328.63 103.2 999999.9 999999.9 33363.63 147.8 999999.9 101.3 33398.63 155.8 999999.9 71.6 33433.63 171.1 999999.9 -29.4 33468.63 250.1 101.6 999999.9 33503.63 281.0 125.4 999999.9 33538.63 306.6 999999.9 999999.9 33573.63 333.1 999999.9 999999.9 33608.63 323.6 999999.9 999999.9 33643.63 314.5 999999.9 999999.9 33678.63 455.9 188.8 999999.9 33713.63 498.6 184.6 999999.9 33748.63 554.3 999999.9 999999.9 33783.63 541.8 999999.9 487.6 33818.63 567.1 999999.9 578.6 33853.63 478.8 999999.9 446.2 33888.63 373.5 86.3 999999.9 33923.63 332.6 77.9 999999.9 33958.63 325.8 999999.9 999999.9 33993.63 642.8 999999.9 999999.9 34028.63 649.0 999999.9 999999.9 34063.63 717.1 999999.9 999999.9 34098.63 683.1 265.4 999999.9 34133.63 756.8 256.5 999999.9 34168.63 687.0 999999.9 999999.9 34203.63 769.3 999999.9 24.2 34238.63 774.1 999999.9 11.6 34273.63 892.7 999999.9 999999.9 34308.63 849.0 317.3 999999.9 34343.63 971.2 331.6 999999.9 34378.63 964.8 999999.9 999999.9 34413.63 960.0 999999.9 999999.9 34448.63 954.5 999999.9 999999.9 34483.63 966.9 999999.9 999999.9 34518.63 1073.5 999999.9 999999.9 34553.63 1147.3 999999.9 999999.9 34588.63 1105.4 999999.9 999999.9 34623.63 1223.6 999999.9 999999.9 34658.63 1103.9 999999.9 999999.9 34693.63 1108.2 999999.9 999999.9 34728.63 1112.6 999999.9 999999.9 34763.63 1122.1 392.0 999999.9 34798.63 1118.3 371.8 999999.9 34833.63 1095.3 999999.9 999999.9 34868.63 1132.4 999999.9 -0.9 34903.63 1172.1 999999.9 35.7 34938.63 1177.1 999999.9 999999.9 34973.63 1179.4 407.1 999999.9 35008.63 1204.8 374.3 999999.9 35043.63 1236.7 999999.9 999999.9 35078.63 1211.7 999999.9 999999.9 35113.63 1226.7 999999.9 999999.9 35148.63 1222.5 999999.9 999999.9 35183.63 1240.0 400.6 999999.9 35218.63 1342.0 388.2 999999.9 35253.63 1276.9 999999.9 999999.9 35288.63 1313.7 999999.9 106.4 35323.63 1338.8 999999.9 99.1 35358.63 1410.5 999999.9 999999.9 35393.63 1375.2 411.2 999999.9 35428.63 1345.4 413.0 999999.9 35463.63 1430.7 999999.9 999999.9 35498.63 1503.4 999999.9 999999.9 35533.63 1488.3 999999.9 999999.9 35568.63 1454.0 999999.9 999999.9 35603.63 1495.7 409.7 999999.9 35638.63 1414.3 415.5 999999.9 35673.63 1436.0 999999.9 999999.9 35708.63 1456.5 999999.9 164.6 35743.63 1435.7 999999.9 184.0 35778.63 1400.1 999999.9 999999.9 35813.63 1477.0 406.2 999999.9 35848.63 1388.3 407.6 999999.9 35883.63 1475.0 999999.9 999999.9 35918.63 1468.1 999999.9 999999.9 35953.63 1436.0 999999.9 999999.9 35988.63 1426.2 999999.9 999999.9 36023.63 1707.5 999999.9 999999.9 36058.63 1735.1 999999.9 999999.9 36093.63 1700.6 999999.9 999999.9 36128.63 1657.9 999999.9 999999.9 36163.63 1564.8 999999.9 999999.9 36198.63 1602.1 999999.9 999999.9 36233.63 1526.2 999999.9 999999.9 36268.63 1485.3 388.3 999999.9 36303.63 1439.2 372.2 999999.9 36338.63 1436.1 999999.9 999999.9 36373.63 1461.4 999999.9 492.3 36408.63 1389.2 999999.9 335.0 36443.63 1331.7 999999.9 999999.9 36478.63 1400.2 326.1 999999.9 36513.63 1411.6 325.4 999999.9 36548.63 1388.2 999999.9 999999.9 36583.63 1271.3 999999.9 999999.9 36618.63 1328.2 999999.9 999999.9 36653.63 1328.1 999999.9 999999.9 36688.63 1379.3 320.9 999999.9 36723.63 1345.2 310.6 999999.9 36758.63 1258.6 999999.9 999999.9 36793.63 1020.1 999999.9 351.3 36828.63 969.4 999999.9 271.6 36863.63 970.4 999999.9 999999.9 36898.63 886.3 140.5 999999.9 36933.63 913.2 145.3 999999.9 36968.63 759.9 999999.9 999999.9 37003.63 714.8 999999.9 999999.9 37038.63 716.3 999999.9 999999.9 37073.63 708.6 999999.9 999999.9 37108.63 672.6 100.7 999999.9 37143.63 661.2 86.3 999999.9 37178.63 629.5 999999.9 999999.9 37213.63 593.8 999999.9 781.0 37248.63 575.8 999999.9 793.0 37283.63 370.6 999999.9 999999.9 37318.63 303.5 4.2 999999.9 37353.63 435.8 34.1 999999.9 37388.63 484.0 999999.9 999999.9 37423.63 309.1 999999.9 999999.9 37458.63 259.4 999999.9 999999.9 37493.63 253.3 999999.9 999999.9 37528.63 238.8 999999.9 999999.9 37563.63 221.7 999999.9 999999.9 37598.63 221.4 999999.9 999999.9 37633.63 213.7 999999.9 999999.9 37668.63 217.4 999999.9 999999.9 37703.63 220.8 999999.9 999999.9 37738.63 219.2 999999.9 999999.9 37773.63 206.0 11.1 999999.9 37808.63 211.0 15.8 999999.9 37843.63 223.5 999999.9 999999.9 37878.63 236.9 999999.9 659.4 37913.63 182.7 999999.9 598.7 37948.63 174.3 999999.9 999999.9 37983.63 167.2 -8.2 999999.9 38018.63 164.3 -0.1 999999.9 38053.63 166.9 999999.9 999999.9 38088.63 190.6 999999.9 999999.9 38123.63 159.0 999999.9 999999.9 38158.63 159.5 999999.9 999999.9 38193.63 183.3 11.6 999999.9 38228.63 161.5 4.9 999999.9 38263.63 217.1 999999.9 999999.9 38298.63 168.5 999999.9 686.0 38333.63 149.9 999999.9 609.6 38368.63 163.4 999999.9 999999.9 38403.63 137.6 -7.0 999999.9 38438.63 133.9 7.0 999999.9 38473.63 135.4 999999.9 999999.9 38508.63 126.1 999999.9 999999.9 38543.63 133.5 999999.9 999999.9 38578.63 125.9 999999.9 999999.9 38613.63 136.2 3.0 999999.9 38648.63 151.2 3.3 999999.9 38683.63 183.0 999999.9 999999.9 38718.63 163.9 999999.9 815.9 38753.63 188.5 999999.9 778.3 38788.63 202.7 999999.9 999999.9 38823.63 149.4 5.3 999999.9 38858.63 129.6 -6.7 999999.9 38893.63 146.4 999999.9 999999.9 38928.63 110.1 999999.9 999999.9 38963.63 130.9 999999.9 999999.9 38998.63 188.1 999999.9 999999.9 39033.63 144.0 999999.9 999999.9 39068.63 125.5 999999.9 999999.9 39103.63 126.6 999999.9 999999.9 39138.63 110.4 999999.9 999999.9 39173.63 112.3 999999.9 999999.9 39208.63 112.7 999999.9 999999.9 39243.63 96.1 999999.9 999999.9 39278.63 101.9 9.0 999999.9 39313.63 93.8 5.2 999999.9 39348.63 84.9 999999.9 999999.9 39383.63 112.5 999999.9 654.6 39418.63 106.7 999999.9 583.4 39453.63 96.4 999999.9 999999.9 39488.63 98.8 -1.5 999999.9 39523.63 74.4 -7.8 999999.9 39558.63 67.0 999999.9 999999.9 39593.63 101.4 999999.9 999999.9 39628.63 89.9 999999.9 999999.9 39663.63 78.4 999999.9 999999.9 39698.63 62.2 -0.0 999999.9 39733.63 81.7 -0.1 999999.9 39768.63 77.8 999999.9 999999.9 39803.63 93.0 999999.9 614.6 39838.63 105.4 999999.9 554.7 39873.63 88.0 999999.9 999999.9 39908.63 98.6 -3.5 999999.9 39943.63 103.6 -0.4 999999.9 39978.63 80.3 999999.9 999999.9 40013.63 83.4 999999.9 999999.9 40048.63 72.4 999999.9 999999.9 40083.63 69.8 999999.9 999999.9 40118.63 85.9 -1.3 999999.9 40153.63 93.6 -6.5 999999.9 40188.63 81.2 999999.9 999999.9 40223.63 90.4 999999.9 645.6 40258.63 85.0 999999.9 651.6 40293.63 70.6 999999.9 999999.9 40328.63 70.8 -17.5 999999.9 40363.63 64.7 -6.4 999999.9 40398.63 70.4 999999.9 999999.9 40433.63 73.5 999999.9 999999.9 40468.63 72.2 999999.9 999999.9 40503.63 67.0 999999.9 999999.9 40538.63 78.6 999999.9 999999.9 40573.63 68.9 999999.9 999999.9 40608.63 85.8 999999.9 999999.9 40643.63 81.2 999999.9 999999.9 40678.63 78.8 999999.9 999999.9 40713.63 83.5 999999.9 999999.9 40748.63 63.0 999999.9 999999.9 40783.63 68.1 6.8 999999.9 40818.63 58.7 -2.6 999999.9 40853.63 69.3 999999.9 999999.9 40888.63 82.8 999999.9 570.8 40923.63 82.5 999999.9 485.6 40958.63 68.6 999999.9 999999.9 40993.63 74.8 -5.2 999999.9 41028.63 84.1 -4.3 999999.9 41063.63 80.6 999999.9 999999.9 41098.63 92.7 999999.9 999999.9 41133.63 93.5 999999.9 999999.9 41168.63 77.3 999999.9 999999.9 41203.63 83.9 1.5 999999.9 41238.63 80.5 -8.2 999999.9 41273.63 97.6 999999.9 999999.9 41308.63 90.8 999999.9 683.1 41343.63 89.1 999999.9 659.2 41378.63 87.5 999999.9 999999.9 41413.63 74.7 999999.9 999999.9 41448.63 66.2 -13.2 999999.9 41483.63 106.3 999999.9 999999.9 41518.63 86.5 999999.9 999999.9 41553.63 88.9 999999.9 999999.9 41588.63 75.7 999999.9 999999.9 41623.63 84.8 -9.8 999999.9 41658.63 72.0 -23.2 999999.9 41693.63 67.5 999999.9 999999.9 41728.63 86.6 999999.9 660.3 41763.63 68.9 999999.9 446.7 41798.63 89.0 999999.9 999999.9 41833.63 59.2 2.3 999999.9 41868.63 54.9 -7.6 999999.9 41903.63 64.6 999999.9 999999.9 41938.63 51.5 999999.9 999999.9 41973.63 59.9 999999.9 999999.9 42008.63 73.8 999999.9 999999.9 42043.63 75.4 999999.9 999999.9 42078.63 76.8 999999.9 999999.9 42113.63 96.3 999999.9 999999.9 42148.63 116.1 999999.9 999999.9 42183.63 81.6 999999.9 999999.9 42218.63 79.5 999999.9 999999.9 42253.63 61.1 999999.9 999999.9 42288.63 58.7 999999.9 999999.9 42323.63 82.1 -0.9 999999.9 42358.63 91.8 999999.9 999999.9 42393.63 81.4 999999.9 576.4 42428.63 72.8 999999.9 545.8 42463.63 72.6 999999.9 999999.9 42498.63 84.9 -12.2 999999.9 42533.63 86.9 -20.5 999999.9 42568.63 97.9 999999.9 999999.9 42603.63 110.7 999999.9 999999.9 42638.63 97.1 999999.9 999999.9 42673.63 99.9 999999.9 999999.9 42708.63 90.9 15.9 999999.9 42743.63 91.9 3.8 999999.9 42778.63 91.0 999999.9 999999.9 42813.63 93.8 999999.9 702.9 42848.63 69.8 999999.9 692.0 42883.63 69.0 999999.9 999999.9 42918.63 71.0 -6.5 999999.9 42953.63 79.4 -8.0 999999.9 42988.63 92.9 999999.9 999999.9 43023.63 57.0 999999.9 999999.9 43058.63 68.9 999999.9 999999.9 43093.63 48.6 999999.9 999999.9 43128.63 43.0 8.5 999999.9 43163.63 17.6 8.3 999999.9 43198.63 22.3 999999.9 999999.9 43233.63 30.9 999999.9 226.2 43268.63 29.9 999999.9 204.2 43303.63 29.5 999999.9 999999.9 43338.63 22.8 -4.6 999999.9 43373.63 20.3 4.0 999999.9 43408.63 34.8 999999.9 999999.9 43443.63 32.7 999999.9 999999.9 43478.63 34.3 999999.9 999999.9 43513.63 28.8 999999.9 999999.9 43548.63 15.7 999999.9 999999.9 43583.63 40.7 999999.9 999999.9 43618.63 37.9 999999.9 999999.9 43653.63 25.3 999999.9 999999.9 43688.63 37.0 999999.9 999999.9 43723.63 40.4 999999.9 999999.9 43758.63 27.5 999999.9 999999.9 43793.63 29.0 16.3 999999.9 43828.63 28.5 14.4 999999.9 43863.63 29.9 999999.9 999999.9 43898.63 30.7 999999.9 156.7 43933.63 27.8 999999.9 180.9 43968.63 9.1 999999.9 103.3 44003.63 13.9 6.1 999999.9 44038.63 9.1 5.6 999999.9 44073.63 18.5 999999.9 999999.9 44108.63 25.9 999999.9 999999.9 44143.63 18.3 999999.9 999999.9 44178.63 12.4 999999.9 999999.9 44213.63 7.1 13.2 999999.9 44248.63 9.0 16.7 999999.9 44283.63 24.2 999999.9 999999.9 44318.63 19.4 999999.9 82.7 44353.63 18.3 999999.9 159.2 44388.63 10.9 999999.9 80.1 44423.63 16.1 3.5 999999.9 44458.63 16.4 9.9 999999.9 44493.63 35.0 999999.9 999999.9 44528.63 12.3 999999.9 999999.9 44563.63 23.7 999999.9 999999.9 44598.63 14.8 999999.9 999999.9 44633.63 36.6 5.8 999999.9 44668.63 71.8 16.3 999999.9 44703.63 76.9 999999.9 999999.9 44738.63 74.2 999999.9 671.6 44773.63 71.8 999999.9 612.3 44808.63 89.5 999999.9 999999.9 44843.63 55.1 6.5 999999.9 44878.63 72.5 -8.7 999999.9 44913.63 90.1 999999.9 999999.9 44948.63 117.7 999999.9 999999.9 44983.63 126.4 999999.9 999999.9 45018.63 127.1 999999.9 999999.9 45053.63 110.6 999999.9 999999.9 45088.63 105.9 999999.9 999999.9 45123.63 127.5 999999.9 999999.9 45158.63 125.6 999999.9 999999.9 45193.63 107.0 999999.9 999999.9 45228.63 101.0 999999.9 999999.9 45263.63 98.8 999999.9 999999.9 45298.63 101.5 12.0 999999.9 45333.63 102.5 -2.1 999999.9 45368.63 115.2 999999.9 999999.9 45403.63 116.7 999999.9 680.8 45438.63 116.0 999999.9 724.6 45473.63 128.3 999999.9 999999.9 45508.63 125.7 -4.1 999999.9 45543.63 124.8 -1.5 999999.9 45578.63 132.5 999999.9 999999.9 45613.63 144.0 999999.9 999999.9 45648.63 136.6 999999.9 999999.9 45683.63 140.3 999999.9 999999.9 45718.63 119.1 9.1 999999.9 45753.63 151.1 -11.6 999999.9 45788.63 161.1 999999.9 999999.9 45823.63 142.6 999999.9 742.8 45858.63 126.2 999999.9 585.9 45893.63 137.8 999999.9 999999.9 45928.63 126.7 -5.1 999999.9 45963.63 147.6 -12.8 999999.9 45998.63 205.5 999999.9 999999.9 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