44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 01 14 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 45139.75 999999.9 999999.9 999999.9 45174.75 999999.9 999999.9 999999.9 45209.75 999999.9 999999.9 999999.9 45244.75 999999.9 999999.9 999999.9 45279.75 999999.9 999999.9 999999.9 45314.75 -8.4 999999.9 999999.9 45349.75 -10.3 999999.9 999999.9 45384.75 0.8 999999.9 999999.9 45419.75 12.4 999999.9 999999.9 45454.75 -0.7 999999.9 999999.9 45489.75 6.0 999999.9 999999.9 45524.75 -0.5 999999.9 999999.9 45559.75 -1.0 999999.9 999999.9 45594.75 -3.9 999999.9 999999.9 45629.75 -3.8 999999.9 999999.9 45664.75 -3.7 999999.9 999999.9 45699.75 -1.4 999999.9 999999.9 45734.75 -3.2 999999.9 999999.9 45769.75 2.1 999999.9 999999.9 45804.75 -6.1 999999.9 -7.4 45839.75 0.6 999999.9 17.4 45874.75 -6.4 999999.9 25.4 45909.75 -3.7 999999.9 -18.5 45944.75 -0.2 999999.9 999999.9 45979.75 3.2 999999.9 999999.9 46014.75 1.4 999999.9 999999.9 46049.75 1.2 999999.9 999999.9 46084.75 -4.6 999999.9 999999.9 46119.75 -0.3 999999.9 999999.9 46154.75 4.9 999999.9 35.5 46189.75 -0.3 999999.9 4.9 46224.75 -8.8 999999.9 56.5 46259.75 -3.7 999999.9 108.7 46294.75 0.6 999999.9 999999.9 46329.75 13.1 999999.9 999999.9 46364.75 3.1 999999.9 999999.9 46399.75 6.8 999999.9 999999.9 46434.75 -0.4 999999.9 999999.9 46469.75 -2.4 999999.9 999999.9 46504.75 7.2 999999.9 999999.9 46539.75 1.3 999999.9 999999.9 46574.75 -2.8 -8.0 999999.9 46609.75 -0.4 999999.9 999999.9 46644.75 10.1 999999.9 314.0 46679.75 1.4 999999.9 286.7 46714.75 2.8 999999.9 237.5 46749.75 9.8 999999.9 999999.9 46784.75 4.8 999999.9 999999.9 46819.75 3.8 999999.9 999999.9 46854.75 999999.9 999999.9 999999.9 46889.75 4.3 999999.9 999999.9 46924.75 12.8 4.7 999999.9 46959.75 11.6 999999.9 288.7 46994.75 8.1 999999.9 254.1 47029.75 17.3 999999.9 226.1 47064.75 17.3 999999.9 282.6 47099.75 12.0 999999.9 999999.9 47134.75 18.3 999999.9 999999.9 47169.75 19.3 999999.9 999999.9 47204.75 22.2 999999.9 999999.9 47239.75 22.1 999999.9 999999.9 47274.75 7.8 -4.2 999999.9 47309.75 21.3 999999.9 368.1 47344.75 21.2 999999.9 262.5 47379.75 25.0 999999.9 340.5 47414.75 22.1 999999.9 376.3 47449.75 26.7 -18.9 999999.9 47484.75 24.9 999999.9 999999.9 47519.75 24.6 999999.9 999999.9 47554.75 25.5 999999.9 999999.9 47589.75 23.5 999999.9 999999.9 47624.75 18.9 999999.9 999999.9 47659.75 17.8 999999.9 999999.9 47694.75 23.2 999999.9 999999.9 47729.75 27.0 999999.9 999999.9 47764.75 25.5 -4.1 999999.9 47799.75 25.8 999999.9 418.1 47834.75 22.5 999999.9 304.7 47869.75 30.5 999999.9 299.3 47904.75 26.2 999999.9 247.3 47939.75 29.1 999999.9 999999.9 47974.75 35.8 999999.9 999999.9 48009.75 38.7 999999.9 999999.9 48044.75 29.7 999999.9 999999.9 48079.75 43.6 999999.9 999999.9 48114.75 34.0 -11.8 999999.9 48149.75 47.8 999999.9 450.8 48184.75 43.9 999999.9 350.6 48219.75 36.0 999999.9 349.7 48254.75 33.3 999999.9 999999.9 48289.75 33.4 999999.9 999999.9 48324.75 38.7 999999.9 999999.9 48359.75 42.0 999999.9 999999.9 48394.75 51.1 999999.9 999999.9 48429.75 39.0 999999.9 999999.9 48464.75 56.2 999999.9 999999.9 48499.75 36.1 999999.9 999999.9 48534.75 44.9 999999.9 430.4 48569.75 41.6 999999.9 303.5 48604.75 34.2 999999.9 368.7 48639.75 44.8 999999.9 999999.9 48674.75 41.4 999999.9 999999.9 48709.75 47.7 999999.9 999999.9 48744.75 45.8 999999.9 999999.9 48779.75 52.2 999999.9 999999.9 48814.75 52.6 999999.9 999999.9 48849.75 52.9 999999.9 999999.9 48884.75 55.0 999999.9 999999.9 48919.75 52.8 999999.9 999999.9 48954.75 45.7 999999.9 999999.9 48989.75 38.7 999999.9 999999.9 49024.75 36.6 -5.3 999999.9 49059.75 25.5 999999.9 357.0 49094.75 29.1 999999.9 228.4 49129.75 31.9 999999.9 195.4 49164.75 33.2 999999.9 247.0 49199.75 21.9 999999.9 999999.9 49234.75 29.1 999999.9 999999.9 49269.75 33.0 999999.9 999999.9 49304.75 38.2 999999.9 999999.9 49339.75 36.4 999999.9 999999.9 49374.75 27.5 1.5 999999.9 49409.75 44.3 999999.9 264.4 49444.75 37.3 999999.9 287.7 49479.75 41.9 999999.9 345.2 49514.75 48.5 999999.9 279.3 49549.75 47.9 999999.9 999999.9 49584.75 39.2 999999.9 999999.9 49619.75 48.9 999999.9 999999.9 49654.75 37.1 999999.9 999999.9 49689.75 32.7 999999.9 999999.9 49724.75 32.3 -4.7 999999.9 49759.75 36.6 999999.9 313.9 49794.75 45.7 999999.9 280.7 49829.75 32.9 999999.9 312.6 49864.75 45.5 999999.9 334.6 49899.75 45.3 999999.9 999999.9 49934.75 47.0 999999.9 999999.9 49969.75 41.6 999999.9 999999.9 50004.75 31.8 999999.9 999999.9 50039.75 29.0 999999.9 999999.9 50074.75 37.0 999999.9 999999.9 50109.75 28.5 999999.9 999999.9 50144.75 42.6 999999.9 999999.9 50179.75 31.2 7.7 999999.9 50214.75 29.0 999999.9 999999.9 50249.75 25.6 999999.9 224.0 50284.75 33.0 999999.9 238.3 50319.75 37.5 999999.9 245.1 50354.75 40.8 999999.9 999999.9 50389.75 38.3 999999.9 999999.9 50424.75 25.6 999999.9 999999.9 50459.75 27.7 999999.9 999999.9 50494.75 31.2 999999.9 999999.9 50529.75 29.2 0.5 999999.9 50564.75 30.3 999999.9 217.4 50599.75 21.2 999999.9 164.7 50634.75 14.5 999999.9 168.9 50669.75 25.2 999999.9 184.1 50704.75 25.7 999999.9 999999.9 50739.75 13.2 999999.9 999999.9 50774.75 23.8 999999.9 999999.9 50809.75 21.3 999999.9 999999.9 50844.75 25.6 999999.9 999999.9 50879.75 25.6 -0.0 999999.9 50914.75 27.6 999999.9 999999.9 50949.75 25.7 999999.9 170.2 50984.75 28.6 999999.9 233.6 51019.75 32.3 999999.9 242.9 51054.75 33.4 999999.9 999999.9 51089.75 31.1 999999.9 999999.9 51124.75 15.2 999999.9 999999.9 51159.75 27.9 999999.9 999999.9 51194.75 33.0 999999.9 999999.9 51229.75 19.7 999999.9 999999.9 51264.75 42.5 999999.9 999999.9 51299.75 30.8 999999.9 999999.9 51334.75 35.4 6.8 999999.9 51369.75 34.0 999999.9 999999.9 51404.75 28.8 999999.9 174.9 51439.75 32.1 999999.9 157.7 51474.75 35.7 999999.9 149.9 51509.75 28.9 999999.9 999999.9 51544.75 40.9 999999.9 999999.9 51579.75 29.8 999999.9 999999.9 51614.75 36.1 999999.9 999999.9 51649.75 27.7 999999.9 999999.9 51684.75 27.4 3.9 999999.9 51719.75 37.7 999999.9 188.2 51754.75 28.9 999999.9 150.4 51789.75 32.5 999999.9 999999.9 51824.75 26.0 999999.9 174.0 51859.75 37.2 999999.9 999999.9 51894.75 28.9 999999.9 999999.9 51929.75 26.0 999999.9 999999.9 51964.75 28.1 999999.9 999999.9 51999.75 29.8 999999.9 999999.9 52034.75 25.2 -3.3 999999.9 52069.75 27.7 999999.9 225.0 52104.75 29.2 999999.9 172.2 52139.75 36.3 999999.9 192.8 52174.75 38.9 999999.9 204.2 52209.75 37.5 999999.9 999999.9 52244.75 39.4 999999.9 999999.9 52279.75 29.4 999999.9 999999.9 52314.75 41.7 999999.9 999999.9 52349.75 36.6 999999.9 999999.9 52384.75 24.5 999999.9 999999.9 52419.75 33.3 999999.9 999999.9 52454.75 33.7 999999.9 999999.9 52489.75 34.0 999999.9 999999.9 52524.75 24.9 999999.9 999999.9 52559.75 33.0 999999.9 999999.9 52594.75 27.5 999999.9 999999.9 52629.75 29.7 -5.5 999999.9 52664.75 31.6 999999.9 230.6 52699.75 27.8 999999.9 198.3 52734.75 27.1 999999.9 202.5 52769.75 35.2 999999.9 148.0 52804.75 28.5 999999.9 999999.9 52839.75 36.8 999999.9 999999.9 52874.75 29.0 999999.9 999999.9 52909.75 32.7 999999.9 999999.9 52944.75 30.7 999999.9 999999.9 52979.75 26.0 3.2 999999.9 53014.75 24.3 999999.9 183.2 53049.75 31.7 999999.9 177.3 53084.75 22.6 999999.9 160.6 53119.75 27.8 999999.9 127.5 53154.75 27.0 7.0 999999.9 53189.75 21.2 999999.9 999999.9 53224.75 22.2 999999.9 999999.9 53259.75 19.0 999999.9 999999.9 53294.75 27.5 999999.9 999999.9 53329.75 24.0 3.1 999999.9 53364.75 27.4 999999.9 148.8 53399.75 27.0 999999.9 999999.9 53434.75 18.8 999999.9 999999.9 53469.75 20.6 999999.9 125.5 53504.75 23.1 999999.9 999999.9 53539.75 23.0 999999.9 999999.9 53574.75 31.7 999999.9 999999.9 53609.75 34.5 999999.9 999999.9 53644.75 31.7 999999.9 999999.9 53679.75 24.9 999999.9 999999.9 53714.75 24.8 999999.9 999999.9 53749.75 19.8 999999.9 999999.9 53784.75 24.7 -4.3 999999.9 53819.75 21.9 999999.9 219.1 53854.75 31.9 999999.9 167.5 53889.75 25.9 999999.9 117.7 53924.75 21.0 999999.9 149.9 53959.75 19.4 999999.9 999999.9 53994.75 30.4 999999.9 999999.9 54029.75 20.7 999999.9 999999.9 54064.75 18.3 999999.9 999999.9 54099.75 28.3 999999.9 999999.9 54134.75 23.1 2.9 999999.9 54169.75 25.5 999999.9 197.6 54204.75 31.5 999999.9 113.9 54239.75 33.8 999999.9 131.3 54274.75 19.7 999999.9 119.6 54309.75 28.5 999999.9 999999.9 54344.75 39.2 999999.9 999999.9 54379.75 28.2 999999.9 999999.9 54414.75 22.0 999999.9 999999.9 54449.75 31.8 999999.9 999999.9 54484.75 28.7 2.2 999999.9 54519.75 28.5 999999.9 999999.9 54554.75 38.3 999999.9 169.8 54589.75 27.0 999999.9 112.2 54624.75 32.0 999999.9 189.7 54659.75 33.0 999999.9 999999.9 54694.75 30.3 999999.9 999999.9 54729.75 36.8 999999.9 999999.9 54764.75 34.6 999999.9 999999.9 54799.75 40.6 999999.9 999999.9 54834.75 31.9 999999.9 999999.9 54869.75 40.2 999999.9 999999.9 54904.75 39.2 999999.9 999999.9 54939.75 28.9 11.0 999999.9 54974.75 30.4 999999.9 999999.9 55009.75 25.7 999999.9 127.3 55044.75 27.0 999999.9 162.3 55079.75 31.7 999999.9 118.9 55114.75 32.6 999999.9 999999.9 55149.75 28.3 999999.9 999999.9 55184.75 25.5 999999.9 999999.9 55219.75 32.5 999999.9 999999.9 55254.75 34.7 999999.9 999999.9 55289.75 22.9 4.3 999999.9 55324.75 29.9 999999.9 999999.9 55359.75 27.9 999999.9 127.2 55394.75 23.3 999999.9 104.1 55429.75 27.6 999999.9 116.7 55464.75 30.0 999999.9 999999.9 55499.75 22.3 999999.9 999999.9 55534.75 19.3 999999.9 999999.9 55569.75 20.7 999999.9 999999.9 55604.75 26.1 999999.9 999999.9 55639.75 26.6 10.0 999999.9 55674.75 28.7 999999.9 999999.9 55709.75 23.6 999999.9 120.0 55744.75 32.3 999999.9 127.2 55779.75 20.6 999999.9 107.5 55814.75 18.7 -11.1 999999.9 55849.75 19.7 999999.9 999999.9 55884.75 17.3 999999.9 999999.9 55919.75 26.5 999999.9 999999.9 55954.75 37.4 999999.9 999999.9 55989.75 34.8 999999.9 999999.9 56024.75 39.6 999999.9 999999.9 56059.75 36.1 999999.9 999999.9 56094.75 31.7 999999.9 999999.9 56129.75 22.2 999999.9 999999.9 56164.75 23.2 999999.9 999999.9 56199.75 22.2 13.0 999999.9 56234.75 25.8 999999.9 999999.9 56269.75 23.0 999999.9 78.7 56304.75 24.7 999999.9 999999.9 56339.75 26.2 999999.9 999999.9 56374.75 29.9 999999.9 999999.9 56409.75 20.3 999999.9 999999.9 56444.75 23.0 999999.9 999999.9 56479.75 20.0 999999.9 999999.9 56514.75 24.1 999999.9 999999.9 56549.75 25.2 8.1 999999.9 56584.75 17.2 999999.9 999999.9 56619.75 18.1 999999.9 112.5 56654.75 34.0 999999.9 98.7 56689.75 15.6 999999.9 57.2 56724.75 19.2 999999.9 999999.9 56759.75 32.6 999999.9 999999.9 56794.75 21.3 999999.9 999999.9 56829.75 18.8 999999.9 999999.9 56864.75 19.4 999999.9 999999.9 56899.75 12.8 11.5 999999.9 56934.75 15.1 999999.9 114.7 56969.75 14.4 999999.9 57.1 57004.75 13.1 999999.9 52.6 57039.75 20.0 999999.9 14.5 57074.75 14.2 999999.9 999999.9 57109.75 20.9 999999.9 999999.9 57144.75 12.1 999999.9 999999.9 57179.75 13.0 999999.9 999999.9 57214.75 23.4 999999.9 999999.9 57249.75 18.8 999999.9 999999.9 57284.75 15.7 999999.9 999999.9 57319.75 19.5 999999.9 999999.9 57354.75 13.9 999999.9 999999.9 57389.75 21.5 999999.9 999999.9 57424.75 6.1 999999.9 999999.9 57459.75 14.8 999999.9 79.6 57494.75 16.8 999999.9 51.8 57529.75 4.8 999999.9 65.7 57564.75 17.4 999999.9 999999.9 57599.75 10.4 999999.9 999999.9 57634.75 15.4 999999.9 999999.9 57669.75 15.3 999999.9 999999.9 57704.75 12.9 999999.9 999999.9 57739.75 8.7 9.3 999999.9 57774.75 17.6 999999.9 999999.9 57809.75 20.2 999999.9 76.9 57844.75 7.4 999999.9 31.6 57879.75 13.0 999999.9 70.0 57914.75 11.1 999999.9 999999.9 57949.75 13.1 999999.9 999999.9 57984.75 17.0 999999.9 999999.9 58019.75 8.2 999999.9 999999.9 58054.75 14.0 999999.9 999999.9 58089.75 4.4 12.2 999999.9 58124.75 17.6 999999.9 999999.9 58159.75 8.0 999999.9 81.4 58194.75 10.1 999999.9 76.9 58229.75 5.6 999999.9 42.8 58264.75 4.9 999999.9 999999.9 58299.75 12.3 999999.9 999999.9 58334.75 11.9 999999.9 999999.9 58369.75 8.1 999999.9 999999.9 58404.75 21.7 999999.9 999999.9 58439.75 13.1 999999.9 999999.9 58474.75 3.5 999999.9 999999.9 58509.75 2.4 999999.9 999999.9 58544.75 11.0 5.1 999999.9 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