48 1001 ELKINS, JAMES; HURST, DALE; ROMASHKIN, PAVEL; DUTTON, GEOFF U.S. DEPT OF COMMERCE, NOAA / CMDL / HALOCARBONS AND OTHER ATMOSPHERIC TRACE SPECIES GROUP ACATS SOLVE 1 1 2000 03 16 2000 12 21 0 ELAPSED TIME IN SECONDS FROM 00:00:00 GMT ON SAMPLE DATE 8 1.0 1.0 1.0 1.0 1.0 1.0 1.0 1.0 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 Mean Age of Air (years) Mean Age Error (1-sd) (years) Total Br (ppt) Total Organic Br (ppt) Total Inorganic Br (ppt) Total Cl (ppb) Total Organic Cl (ppb) Total Inorganic Cl (ppb) 25 The mean age (Age) of each sampled air mass was determined from the corresponding ACATS measurement of SF6 and the documented tropospheric trend of SF6 [Geller et al., 1997] using a variation of the mean age formula in Volk et al. [1997]. We use dG = -0.8 to account for a SF6 calibration scale change. This term no longer represents only a delay from the surface to the tropopause. The mean age error reported is solely based on the SF6 measurement precision and is thus useful in comparing ACATS ages from different flights. Absolute accuracy of the SF6 measurement and any systematic errors in the method used to calculate mean ages are not included. Organic chlorine (CCly) was calculated from ACATS in-situ measurements of CFC-11, CFC-12, CFC-113, CH3CCl3, and CCl4. Contributions to CCly from CH3Cl and HCFC-22 (measured by WAS) were calculated from their correlations with tracers measured by ACATS. Organic bromine (CBry) was calculated from ACATS in-situ measurements of halon-1211. Contributions to CBry from CH3Br, halon-2402, halon-1301, CH2Br2, and CH2BrCl (measured by WAS) were calculated from their correlations with tracers measured by ACATS using the formula in Wamsley et al. [1997]. The total chlorine (TotalCl) and total bromine (TotalBr) content of each sampled air mass was calculated from the documented tropospheric trends of chlorinated and brominated trace gases (e.g., Montzka et al. [1996]) and weighted with a mean age spectrum calculated by Hall & Plumb [1994]. Inorganic chlorine (Cly) and inorganic bromine (Bry) were calculated as TotalCl-CCly and TotalBr-CBry, respectively. Data submitted only for air masses with potential temperature greater than 380 K. 1 GMTs Age AgeERR TotalBr CBry Bry TotalCl CCly Cly 27558 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 27628 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 27698 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 27768 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 27838 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 27908 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 27978 9999.00 9999.00 9999.000 9999.000 9999.000 9999.000 9999.000 9999.000 28118 1.73 0.43 19.406 9999.000 9999.000 3.407 9999.000 9999.000 28188 1.96 0.39 19.358 13.697 5.662 3.413 2.844 0.569 28258 2.60 0.40 19.219 9999.000 9999.000 3.429 9999.000 9999.000 28328 2.28 0.40 19.292 11.541 7.751 3.421 2.610 0.811 28398 2.68 0.40 19.200 9999.000 9999.000 3.431 9999.000 9999.000 28468 2.12 0.39 19.326 12.758 6.567 3.417 2.743 0.675 28538 1.88 0.43 19.374 9999.000 9999.000 3.411 9999.000 9999.000 28678 2.08 0.39 19.334 9999.000 9999.000 3.416 9999.000 9999.000 28748 2.16 0.39 19.317 12.555 6.763 3.418 2.744 0.674 28818 2.43 0.40 19.256 9999.000 9999.000 3.425 9999.000 9999.000 28958 2.51 0.40 19.238 9999.000 9999.000 3.427 9999.000 9999.000 29028 2.84 0.41 19.159 9.722 9.437 3.435 2.434 1.001 29098 2.84 0.41 19.159 9999.000 9999.000 3.435 9999.000 9999.000 29238 3.41 0.41 19.001 9999.000 9999.000 3.446 9999.000 9999.000 29308 3.49 0.42 18.976 7.723 11.253 3.448 2.165 1.283 29378 3.45 0.42 18.989 9999.000 9999.000 3.447 9999.000 9999.000 29448 3.33 0.41 19.025 8.584 10.440 3.445 2.308 1.137 29518 2.88 0.41 19.149 9999.000 9999.000 3.436 9999.000 9999.000 29588 3.04 0.41 19.105 9.685 9.421 3.439 2.439 1.000 29658 3.20 0.41 19.060 9999.000 9999.000 3.442 9999.000 9999.000 29798 3.41 0.41 19.001 9999.000 9999.000 3.446 9999.000 9999.000 29868 3.66 0.38 18.926 7.358 11.569 3.450 2.162 1.288 29938 3.41 0.41 19.001 9999.000 9999.000 3.446 9999.000 9999.000 30008 3.75 0.38 18.901 7.861 11.040 3.452 2.237 1.215 30078 3.37 0.41 19.013 9999.000 9999.000 3.446 9999.000 9999.000 30148 3.41 0.41 19.001 6.986 12.015 3.446 2.129 1.317 30218 3.29 0.41 19.037 9999.000 9999.000 3.444 9999.000 9999.000 30358 3.62 0.38 18.939 9999.000 9999.000 3.450 9999.000 9999.000 30428 3.62 0.38 18.939 6.977 11.962 3.450 2.116 1.334 30498 3.83 0.38 18.875 9999.000 9999.000 3.453 9999.000 9999.000 30568 3.75 0.38 18.901 7.122 11.779 3.452 2.150 1.302 30638 3.58 0.42 18.952 9999.000 9999.000 3.449 9999.000 9999.000 30708 3.49 0.42 18.976 6.514 12.462 3.448 9999.000 9999.000 30778 3.75 0.38 18.901 9999.000 9999.000 3.452 9999.000 9999.000 30918 3.33 0.41 19.025 9999.000 9999.000 3.445 9999.000 9999.000 30988 3.37 0.41 19.013 7.711 11.302 3.446 2.220 1.226 31058 3.33 0.41 19.025 9999.000 9999.000 3.445 9999.000 9999.000 31128 3.37 0.41 19.013 7.456 11.557 3.446 2.183 1.263 31198 3.49 0.42 18.976 9999.000 9999.000 3.448 9999.000 9999.000 31268 3.37 0.41 19.013 7.898 11.115 3.446 2.215 1.230 31338 2.76 0.40 19.180 9999.000 9999.000 3.433 9999.000 9999.000 31478 2.88 0.41 19.149 9999.000 9999.000 3.436 9999.000 9999.000 31548 3.00 0.41 19.116 9.768 9.348 3.438 2.441 0.997 31618 3.08 0.41 19.094 9999.000 9999.000 3.440 9999.000 9999.000 31758 2.64 0.40 19.209 9999.000 9999.000 3.430 9999.000 9999.000 31828 2.68 0.40 19.200 10.204 8.996 3.431 2.492 0.939 31898 2.80 0.40 19.169 9999.000 9999.000 3.434 9999.000 9999.000 32038 2.43 0.40 19.256 9999.000 9999.000 3.425 9999.000 9999.000 32108 2.51 0.40 19.238 11.352 7.886 3.427 2.612 0.815 32178 2.72 0.40 19.190 9999.000 9999.000 3.432 9999.000 9999.000 32248 2.36 0.40 19.274 11.874 7.400 3.423 2.688 0.735 32318 2.47 0.40 19.247 9999.000 9999.000 3.426 9999.000 9999.000 32388 2.12 0.39 19.326 12.941 6.385 3.417 2.794 0.623 32458 2.32 0.40 19.283 9999.000 9999.000 3.422 9999.000 9999.000 32598 2.28 0.40 19.292 9999.000 9999.000 3.421 9999.000 9999.000 32668 2.40 0.40 19.265 12.372 6.894 3.424 2.720 0.704 32738 2.36 0.40 19.274 9999.000 9999.000 3.423 9999.000 9999.000 32878 1.84 0.43 19.382 9999.000 9999.000 3.410 9999.000 9999.000 32948 2.55 0.40 19.229 11.324 7.905 3.428 2.619 0.809 33018 2.40 0.40 19.265 9999.000 9999.000 3.424 9999.000 9999.000 33158 3.00 0.41 19.116 9999.000 9999.000 3.438 9999.000 9999.000 33228 2.51 0.40 19.238 10.380 8.858 3.427 2.487 0.940 33298 3.20 0.41 19.060 9999.000 9999.000 3.442 9999.000 9999.000 33368 2.72 0.40 19.190 8.904 10.286 3.432 2.320 1.112 33438 2.68 0.40 19.200 9999.000 9999.000 3.431 9999.000 9999.000 33508 3.33 0.41 19.025 7.130 11.895 3.445 2.095 1.350 33578 2.68 0.40 19.200 9999.000 9999.000 3.431 9999.000 9999.000 33718 3.08 0.41 19.094 9999.000 9999.000 3.440 9999.000 9999.000 33788 3.29 0.41 19.037 8.443 10.594 3.444 2.249 1.195 33858 2.80 0.40 19.169 9999.000 9999.000 3.434 9999.000 9999.000 33928 3.29 0.41 19.037 7.972 11.065 3.444 2.214 1.230 33998 3.12 0.41 19.083 9999.000 9999.000 3.441 9999.000 9999.000 34068 3.45 0.42 18.989 7.985 11.004 3.447 2.189 1.258 34138 3.49 0.42 18.976 9999.000 9999.000 3.448 9999.000 9999.000 34278 3.45 0.42 18.989 9999.000 9999.000 3.447 9999.000 9999.000 34348 3.58 0.42 18.952 7.216 11.736 3.449 2.104 1.345 34418 3.45 0.42 18.989 9999.000 9999.000 3.447 9999.000 9999.000 34558 3.41 0.41 19.001 9999.000 9999.000 3.446 9999.000 9999.000 34628 3.66 0.38 18.926 6.499 12.428 3.450 2.018 1.432 34698 4.17 0.39 18.771 9999.000 9999.000 3.457 9999.000 9999.000 34838 3.16 0.41 19.072 9999.000 9999.000 3.442 9999.000 9999.000 34908 3.62 0.38 18.939 7.216 11.723 3.450 2.106 1.343 34978 3.54 0.42 18.964 9999.000 9999.000 3.448 9999.000 9999.000 35048 3.75 0.38 18.901 6.972 11.929 3.452 2.091 1.360 35118 3.70 0.38 18.914 9999.000 9999.000 3.451 9999.000 9999.000 35188 2.96 0.41 19.127 7.758 11.369 3.437 2.189 1.248 35258 3.33 0.41 19.025 9999.000 9999.000 3.445 9999.000 9999.000 35398 3.58 0.42 18.952 9999.000 9999.000 3.449 9999.000 9999.000 35468 3.29 0.41 19.037 5.760 13.277 3.444 1.930 1.514 35538 3.83 0.38 18.875 9999.000 9999.000 3.453 9999.000 9999.000 35608 3.70 0.38 18.914 5.817 13.097 3.451 1.932 1.519 35678 3.79 0.38 18.888 9999.000 9999.000 3.452 9999.000 9999.000 35748 3.79 0.38 18.888 5.658 13.230 3.452 1.924 1.528 35818 3.66 0.38 18.926 9999.000 9999.000 3.450 9999.000 9999.000 35958 3.96 0.38 18.836 9999.000 9999.000 3.455 9999.000 9999.000 36028 4.30 0.39 18.731 4.616 14.115 3.458 1.769 1.690 36098 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 36238 3.79 0.38 18.888 9999.000 9999.000 3.452 9999.000 9999.000 36308 4.30 0.39 18.731 5.380 13.351 3.458 1.883 1.576 36378 4.43 0.39 18.691 9999.000 9999.000 3.460 9999.000 9999.000 36518 4.38 0.39 18.704 9999.000 9999.000 3.459 9999.000 9999.000 36588 4.30 0.39 18.731 5.187 13.544 3.458 1.850 1.608 36658 4.17 0.39 18.771 9999.000 9999.000 3.457 9999.000 9999.000 36728 3.91 0.38 18.849 5.410 13.440 3.454 1.878 1.576 36798 4.04 0.38 18.810 9999.000 9999.000 3.456 9999.000 9999.000 36868 4.51 0.39 18.664 5.298 13.366 3.460 1.862 1.598 36938 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 37078 3.96 0.38 18.836 9999.000 9999.000 3.455 9999.000 9999.000 37148 4.04 0.38 18.810 5.435 13.375 3.456 1.871 1.585 37218 4.30 0.39 18.731 9999.000 9999.000 3.458 9999.000 9999.000 37358 3.87 0.38 18.862 9999.000 9999.000 3.453 9999.000 9999.000 37428 4.00 0.38 18.823 5.741 13.082 3.455 1.922 1.533 37498 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 37638 3.70 0.38 18.914 9999.000 9999.000 3.451 9999.000 9999.000 37708 4.21 0.39 18.757 5.579 13.179 3.458 1.890 1.567 37778 3.66 0.38 18.926 9999.000 9999.000 3.450 9999.000 9999.000 37848 3.75 0.38 18.901 7.070 11.831 3.452 2.104 1.348 37918 3.54 0.42 18.964 9999.000 9999.000 3.448 9999.000 9999.000 37988 3.25 0.41 19.048 6.249 12.799 3.443 2.003 1.440 38058 3.96 0.38 18.836 9999.000 9999.000 3.455 9999.000 9999.000 38198 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 38268 3.75 0.38 18.901 6.003 12.898 3.452 1.953 1.499 38338 3.75 0.38 18.901 9999.000 9999.000 3.452 9999.000 9999.000 38408 3.83 0.38 18.875 5.274 13.601 3.453 1.866 1.587 38478 3.62 0.38 18.939 9999.000 9999.000 3.450 9999.000 9999.000 38548 4.00 0.38 18.823 5.602 13.222 3.455 1.911 1.545 38618 4.00 0.38 18.823 9999.000 9999.000 3.455 9999.000 9999.000 38758 3.58 0.42 18.952 9999.000 9999.000 3.449 9999.000 9999.000 38828 3.87 0.38 18.862 5.801 13.061 3.453 1.925 1.529 38898 3.87 0.38 18.862 9999.000 9999.000 3.453 9999.000 9999.000 38968 3.87 0.38 18.862 5.844 13.019 3.453 1.935 1.518 39038 3.70 0.38 18.914 9999.000 9999.000 3.451 9999.000 9999.000 39108 3.83 0.38 18.875 6.038 12.837 3.453 1.964 1.489 39178 3.62 0.38 18.939 9999.000 9999.000 3.450 9999.000 9999.000 39318 3.87 0.38 18.862 9999.000 9999.000 3.453 9999.000 9999.000 39388 3.75 0.38 18.901 6.701 12.200 3.452 2.055 1.396 39458 3.87 0.38 18.862 9999.000 9999.000 3.453 9999.000 9999.000 39528 3.49 0.42 18.976 6.790 12.186 3.448 2.076 1.372 39598 3.62 0.42 18.939 9999.000 9999.000 3.450 9999.000 9999.000 39668 3.37 0.41 19.013 7.475 11.538 3.446 2.161 1.285 39738 3.37 0.41 19.013 9999.000 9999.000 3.446 9999.000 9999.000 39878 3.58 0.42 18.952 9999.000 9999.000 3.449 9999.000 9999.000 39948 3.58 0.42 18.952 7.423 11.528 3.449 2.161 1.288 40018 3.29 0.41 19.037 9999.000 9999.000 3.444 9999.000 9999.000 40158 3.41 0.41 19.001 9999.000 9999.000 3.446 9999.000 9999.000 40228 3.20 0.41 19.060 7.829 11.231 3.442 2.215 1.228 40298 3.29 0.41 19.037 9999.000 9999.000 3.444 9999.000 9999.000 40438 3.00 0.41 19.116 9999.000 9999.000 3.438 9999.000 9999.000 40508 3.49 0.42 18.976 7.284 11.693 3.448 2.142 1.306 40578 3.79 0.38 18.888 9999.000 9999.000 3.452 9999.000 9999.000 40648 3.41 0.41 19.001 6.447 12.554 3.446 2.026 1.420 40718 3.70 0.38 18.914 9999.000 9999.000 3.451 9999.000 9999.000 40788 3.54 0.42 18.964 6.225 12.739 3.448 2.008 1.441 40858 3.49 0.42 18.976 9999.000 9999.000 3.448 9999.000 9999.000 40998 3.12 0.41 19.083 9999.000 9999.000 3.441 9999.000 9999.000 41068 3.91 0.38 18.849 6.039 12.810 3.454 1.954 1.500 41138 3.70 0.38 18.914 9999.000 9999.000 3.451 9999.000 9999.000 41208 3.58 0.42 18.952 6.292 12.660 3.449 1.997 1.452 41278 3.54 0.42 18.964 9999.000 9999.000 3.448 9999.000 9999.000 41348 3.66 0.38 18.926 7.320 11.606 3.450 2.155 1.295 41418 3.54 0.42 18.964 9999.000 9999.000 3.448 9999.000 9999.000 41558 3.96 0.38 18.836 9999.000 9999.000 3.455 9999.000 9999.000 41628 3.79 0.38 18.888 4.219 14.669 3.452 1.697 1.755 41698 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 41768 4.43 0.39 18.691 3.983 14.707 3.460 1.661 1.798 41838 4.21 0.39 18.757 9999.000 9999.000 3.458 9999.000 9999.000 41908 4.04 0.38 18.810 4.194 14.616 3.456 1.700 1.755 41978 4.21 0.39 18.757 9999.000 9999.000 3.458 9999.000 9999.000 42118 4.08 0.38 18.797 9999.000 9999.000 3.456 9999.000 9999.000 42188 4.30 0.39 18.731 3.915 14.815 3.458 1.657 1.802 42258 4.73 0.39 18.597 9999.000 9999.000 3.462 9999.000 9999.000 42328 4.47 0.39 18.677 3.090 15.587 3.460 1.534 1.926 42398 4.56 0.39 18.651 9999.000 9999.000 3.460 9999.000 9999.000 42468 4.38 0.39 18.704 3.191 15.513 3.459 1.546 1.913 42538 4.38 0.39 18.704 9999.000 9999.000 3.459 9999.000 9999.000 42678 4.08 0.38 18.797 9999.000 9999.000 3.456 9999.000 9999.000 42748 3.87 0.38 18.862 5.146 13.716 3.453 1.839 1.615 42818 3.54 0.42 18.964 9999.000 9999.000 3.448 9999.000 9999.000 42958 3.33 0.41 19.025 9999.000 9999.000 3.445 9999.000 9999.000 43028 3.87 0.38 18.862 5.685 13.178 3.453 1.918 1.536 43098 3.79 0.38 18.888 9999.000 9999.000 3.452 9999.000 9999.000 43238 3.70 0.38 18.914 9999.000 9999.000 3.451 9999.000 9999.000 43308 3.91 0.38 18.849 4.570 14.279 3.454 1.750 1.704 43378 4.13 0.38 18.784 9999.000 9999.000 3.457 9999.000 9999.000 43448 4.17 0.39 18.771 4.208 14.562 3.457 1.695 1.762 43518 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 43588 4.21 0.39 18.757 3.618 15.140 3.458 1.597 1.861 43658 4.04 0.38 18.810 9999.000 9999.000 3.456 9999.000 9999.000 43798 4.21 0.39 18.757 9999.000 9999.000 3.458 9999.000 9999.000 43868 4.43 0.39 18.691 3.307 15.384 3.460 1.554 1.906 43938 4.08 0.38 18.797 9999.000 9999.000 3.456 9999.000 9999.000 44078 2.80 0.40 19.169 9999.000 9999.000 3.434 9999.000 9999.000 44148 4.08 0.38 18.797 2.927 15.870 3.456 1.499 1.957 44218 3.62 0.42 18.939 9999.000 9999.000 3.450 9999.000 9999.000 44358 3.91 0.38 18.849 9999.000 9999.000 3.454 9999.000 9999.000 44428 4.17 0.39 18.771 2.286 16.485 3.457 1.384 2.073 44498 4.13 0.38 18.784 9999.000 9999.000 3.457 9999.000 9999.000 44568 4.60 0.39 18.637 1.816 16.821 3.461 1.286 2.175 44638 4.13 0.38 18.784 9999.000 9999.000 3.457 9999.000 9999.000 44708 4.78 0.40 18.584 1.837 16.746 3.462 1.281 2.181 44778 4.30 0.39 18.731 9999.000 9999.000 3.458 9999.000 9999.000 44918 4.26 0.39 18.744 9999.000 9999.000 3.458 9999.000 9999.000 44988 4.26 0.39 18.744 2.297 16.447 3.458 1.380 2.078 45058 4.47 0.39 18.677 9999.000 9999.000 3.460 9999.000 9999.000 45128 4.08 0.38 18.797 2.569 16.228 3.456 1.440 2.016 45198 3.96 0.38 18.836 9999.000 9999.000 3.455 9999.000 9999.000 45268 4.56 0.39 18.651 2.453 16.198 3.460 1.409 2.051 45338 4.26 0.39 18.744 9999.000 9999.000 3.458 9999.000 9999.000 45478 4.30 0.39 18.731 9999.000 9999.000 3.458 9999.000 9999.000 45548 3.91 0.38 18.849 2.660 16.190 3.454 1.465 1.989 45618 4.17 0.39 18.771 9999.000 9999.000 3.457 9999.000 9999.000 45758 4.13 0.38 18.784 9999.000 9999.000 3.457 9999.000 9999.000 45828 4.26 0.39 18.744 3.132 15.612 3.458 1.533 1.925 45898 4.13 0.38 18.784 9999.000 9999.000 3.457 9999.000 9999.000 46038 4.30 0.39 18.731 9999.000 9999.000 3.458 9999.000 9999.000 46108 4.30 0.39 18.731 3.005 15.726 3.458 1.509 1.950 46178 4.60 0.39 18.637 9999.000 9999.000 3.461 9999.000 9999.000 46248 4.13 0.38 18.784 2.946 15.838 3.457 1.502 1.954 46318 4.21 0.39 18.757 9999.000 9999.000 3.458 9999.000 9999.000 46388 4.82 0.40 18.570 2.833 15.737 3.462 1.478 1.984 46458 4.65 0.39 18.624 9999.000 9999.000 3.461 9999.000 9999.000 46598 4.65 0.39 18.624 9999.000 9999.000 3.461 9999.000 9999.000 46668 4.51 0.39 18.664 2.725 15.939 3.460 1.461 1.999 46738 4.87 0.40 18.557 9999.000 9999.000 3.462 9999.000 9999.000 46808 4.26 0.39 18.744 2.731 16.013 3.458 1.466 1.992 46878 4.34 0.39 18.717 9999.000 9999.000 3.459 9999.000 9999.000 46948 4.38 0.39 18.704 2.747 15.957 3.459 1.468 1.991 47018 4.47 0.39 18.677 9999.000 9999.000 3.460 9999.000 9999.000 47158 4.56 0.39 18.651 9999.000 9999.000 3.460 9999.000 9999.000 47228 4.56 0.39 18.651 2.801 15.849 3.460 1.465 1.995 47298 4.30 0.39 18.731 9999.000 9999.000 3.458 9999.000 9999.000 47438 4.43 0.39 18.691 9999.000 9999.000 3.460 9999.000 9999.000 47508 4.00 0.38 18.823 2.848 15.976 3.455 1.490 1.965 47578 4.51 0.39 18.664 9999.000 9999.000 3.460 9999.000 9999.000 47718 4.34 0.39 18.717 9999.000 9999.000 3.459 9999.000 9999.000 47788 4.43 0.39 18.691 2.523 16.168 3.460 1.421 2.038 47858 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