The Harvard CRDS/ICOS instrument is an absorption spectrometer that uses the relatively new and highly sensitive techniques of integrated cavity output spectroscopy (ICOS) and cavity ringdown spectroscopy (CRDS) with a high-finesse optical cavity and a cw quantum cascade laser (QCL) source. The primary spectroscopic technique employed is ICOS, in which intra-cavity absorption is measured from the steady-state output of the cavity. Light from a high power, tunable, single mode, solid-state laser source is coupled into a cavity consisting of two concave, highly reflective mirrors (R ≈ 0.9999), through which air continuously flows. The laser is scanned over a spectral region of 1–2 cm-1 containing an absorption feature, and the cavity output is detected by an LN2-cooled HgCdTe detector. The resultant output approximates an absorption spectrum with an effective pathlength of > 5 km, far greater than that of standard multipass Herriott or White cells.

The design of the newly developed total water instrument is based on the same principles as the water vapor instrument, and is intended to fly in conjunction with it. Conceptually, the total water instrument can be thought of as containing four subsystems:
1. An inlet through which liquid and/or solid water particles can be brought into an instrument duct without perturbing the ambient particle density.
2. A heater that efficiently evaporates the liquid/solid water before it reaches the detection axis.
3. Ducting through which the air flows to the detection axis without perturbing the (total) water vapor mixing ratio.
4. A water vapor detection axis that accurately and precisely measures the total water content of the ambient air.

The HyMap scanner, built by Integrated Spectronics Inc of Sydney, Australia, has four spectrometers in the interval 0.45 to 2.45 micrometers excluding the two major atmospheric water absorption windows. The bandwidths are not constant, but vary between 15 and 18 nanometers. The scanner also has an on-board bright source calibration system, which is used to monitor the stability of the signal. The signal/noise ratio measured outside the aircraft with a sun angle of 30° and a 50% reflectance standard is more than 500/1 except near the major atmospheric water absorption bands. The scanner is mounted on a hydraulically actuated Zeiss-Jena SM 2000 stabilized platform. The platform provides +/- 5 degrees of pitch and roll correction. The yaw can be offset by +/- 20 degrees with +/- 8 degrees of stabilization. The platform provides a residual error in nadir pointing of less than 1 degree and reduces aircraft motion effects by a factor ranging from 10:1 to 30:1.

The basic HyMap specifications are:

IFOV: 2.5 mr along track, 2.0 mr across track (Spatial resolution 3.5–10 m)
FOV: 62 degrees (512 pixels)

The Multiple-Angle Aerosol Spectrometer Probe (MASP) determines the size and concentration of particles from about 0.3 to 20 microns in diameter and the index of refraction for selected sizes. Size is determined by measuring the light intensity scattered by individual particles as they transit a laser beam of 0.780µm wavelength. Light scattered from particles into a cone from 30 to 60 degrees forward and 120 to 150 degrees backwards is reflected by a mangin mirror through a condensing lens to the detectors. A comparison of the signals from the open aperture detector and the masked aperture detector is used to accept only those particles passing through the center of the laser beam. The size of the particle is determined from the total scattered light. The index of refraction of particles can be estimated from the ratio of the forward to back scatter signals. A calibration diode laser is pulsed periodically during flight to ensure proper operation of the electronics. The shrouded inlet minimizes angle of attack effects and maintains isokinetic flow through the sensing volume so that volatilization of particles is eliminated.

The Multiple Aerosol Collection System contains an impactor collector which permits the collection of particles on electron microscope grids for later chemical-constituent analysis. The collector consists of a two stages. In the first stage the pressure of the sample is reduced by a factor of two without loosing particles by impaction on walls. The second stage consists of a thin plate impactor which collects efficiently even at small Reynolds numbers. The system collects particles as small as 0.02 micron at WB-57 cruise altitudes. As many as 24 samples can be collected in a flight.

IRIS is an ultra sensive laser spectrometer for in situ detection of the isotopic composition of water vapor in the higher tropopause and the lower stratosphere. The isotope signals may be used to quantify troposphere-stratosphere exchange, and to study the water chemistry in the stratosphere. IRIS is based on the technique of optical-feedback cavity enhanced absorption spectroscopy. It uses a room temperature infrared laser, needing no crygens. The instrument combines a low weight (< 50 kg) and volume (< 50 L) with a low power consumption (< 200 W), making it uniquely suitable for future deployment on an Unmanned Aerial Vehicle.

OH is detected by direct laser induced fluorescence in the (0-1) band of the 2?-2? electronic transition. A pulsed dye-laser system produces frequency tunable laser light at 282 nm. An on-board frequency reference cell is used by a computer to lock the laser to the appropriate wavelength. Measurement of the signal is then made by tuning the laser on and off resonance with the OH transition.

Stratospheric air is channeled into the instrument using a double-ducted system that both maintains laminar flow through the detection region and slows the flow from free stream velocity (200 m/s) to 40 m/s. The laser light is beam-split and directed to two detection axes where it passes through the stratospheric air in multipass White cells.

Fluorescence from OH (centered at 309 nm) is detected orthogonal to both the flow and the laser propagation using a filtered PMT assembly. Optical stability is checked periodically by exchanging the 309 nm interference filter with a filter centered at 302 nm, where Raman scattering of N2 is observed.

HO2 is measured as OH after chemical titration with nitric oxide: HO2 + NO → OH + NO2. Variation of added NO density and flow velocity as well as the use of two detection axes aid in diagnosis of the kinetics of this titration. Measurements of ozone (by uv absorption) and water vapor (by photofragment fluorescence) are made as diagnostics of potential photochemical interference from the mechanism: O3 + hv (282 nm) → O(1D) + O2, followed by: O(1D) + H2O → OH + OH

DCS is a 16-megapixel color infrared digital camera system, providing high resolution imagery for mission tracking purposes Geo-referenced image products may be generated, when used in conjunction with a POS-AV system.

The Cloud Physics Lidar, or CPL, is a backscatter lidar designed to operate simultaneously at 3 wavelengths: 1064, 532, and 355 nm. The purpose of the CPL is to provide multi-wavelength measurements of cirrus, subvisual cirrus, and aerosols with high temporal and spatial resolution. Figure 1 shows the entire CPL package in flight configuration. The CPL utilizes state-of-the-art technology with a high repetition rate, low pulse energy laser and photon-counting detection. Vertical resolution of the CPL measurements is fixed at 30 m; horizontal resolution can vary but is typically about 200 m. The CPL fundamentally measures range-resolved profiles of volume 180-degree backscatter coefficients. From the fundamental measurement, various data products are derived, including: time-height crosssection images; cloud and aerosol layer boundaries; optical depth for clouds, aerosol layers, and planetary boundary layer (PBL); and extinction profiles. The CPL was designed to fly on the NASA ER-2 aircraft but is adaptable to other platforms. Because the ER-2 typically flies at about 65,000 feet (20 km), onboard instruments are above 94% of the earth’s atmosphere, allowing ER-2 instruments to function as spaceborne instrument simulators. The ER-2 provides a unique platform for atmospheric profiling, particularly for active remote sensing instruments such as lidar, because the spatial coverage attainable by the ER-2 permits studies of aerosol properties across wide regions. Lidar profiling from the ER-2 platform is especially valuable because the cloud height structure, up to the limit of signal attenuation, is unambiguously measured.

The DLH has been successfully flown during many previous field campaigns on several aircraft, most recently ACTIVATE (Falcon); FIREX-AQ, ATom, KORUS-AQ, and SEAC4RS (DC-8); POSIDON (WB-57); CARAFE (Sherpa); CAMP2Ex and DISCOVER-AQ (P-3); and ATTREX (Global Hawk). This sensor measures water vapor (H2O(v)) via absorption by one of three strong, isolated spectral lines near 1.4 μm and is comprised of a compact laser transceiver and a sheet of high grade retroflecting road sign material to form the optical path. Optical sampling geometry is aircraft-dependent, as each DLH instrument is custom-built to conform to aircraft geometric constraints. Using differential absorption detection techniques, H2O(v) is sensed along the external path negating any potential wall or inlet effects inherent in extractive sampling techniques. A laser power normalization scheme enables the sensor to accurately measure water vapor even when flying through clouds. An algorithm calculates H2O(v) concentration based on the differential absorption signal magnitude, ambient pressure, and temperature, and spectroscopic parameters found in the literature and/or measured in the laboratory. Preliminary water vapor mixing ratio and derived relative humidities are provided in real-time to investigators.