45, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor ATom 1, 1 2018, 05, 06, 2018, 10, 25 0 Start_UTC, seconds, seconds since UTC midnight on day of takeoff 4 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since UTC midnight on day of takeoff Mid_UTC, seconds, seconds since UTC midnight on day of takeoff OH_ATHOS, pptv, OH mixing ratio in pptv HO2_ATHOS, pptv, HO2 mixing ratio in pptv 0 27 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom IV: Science Flight #6 -- CHC - PUQ ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 from Laser Induced Fluorescence. DATA_INFO: Units are pptv for OH and HO2. UNCERTAINTY: HOx absolute accuracy ~+/- 32% (actually a multiplicative factor of 1/1.32 to 1.32), 2 sigma confidence. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Final Data. Future modifications to the calibration are possible but unlikely. - Calibrating ATHOS with the new OH-removing inlet (OHSI) has been difficult, particularly for low pressure (high altitude). - The ATHOS HOx calibrations are pressure-dependent, changing a factor of 3-5 over the atmospheric pressure range. - The laboratory calibration uses different inlet hole sizes to simulate atmospheric pressure changes. - For 2 years, we tried various calibration approaches with the OHSI in place, but none gave repeatable results for high altitude measurements. - In the laboratory calibrations, it proved to be impossible to simulate the atmospheric airflow with the OHSI on and the smaller inlet sizes. - In the end, we found that our previous calibration method gave the most repeatable and reliable results. - In-flight diagnostics show that OH loss on the OHSI is negligible. - For details, please see Faloona et al., J. Atmos. Chem., 47, 139-167, 2004. REVISION: R1 R1: Final Data (see OTHER_COMMENTS) R0: No comments for this revision. Start_UTC, Stop_UTC, Mid_UTC, OH_ATHOS, HO2_ATHOS 73255, 73284, 73270, -9999.000, -9999.000 73285, 73314, 73300, -9999.000, -9999.000 73315, 73344, 73330, -9999.000, -9999.000 73345, 73374, 73360, -9999.000, -9999.000 73375, 73404, 73390, 0.002, 1.970 73405, 73434, 73420, 0.002, 2.919 73435, 73464, 73450, 0.004, 3.179 73465, 73494, 73480, 0.019, 2.797 73495, 73524, 73510, 0.019, 2.416 73526, 73555, 73541, 0.019, 2.522 73556, 73585, 73571, 0.019, 2.338 73586, 73615, 73601, 0.024, 2.760 73616, 73645, 73631, 0.024, 3.182 73646, 73675, 73661, 0.024, 2.952 73676, 73705, 73691, 0.019, 2.722 73706, 73735, 73721, 0.014, 2.491 73736, 73765, 73751, 0.014, 2.262 73766, 73795, 73781, 0.014, 2.301 73796, 73825, 73811, 0.048, 2.371 73826, 73855, 73841, 0.048, 2.214 73856, 73885, 73871, 0.036, 2.056 73886, 73915, 73901, 0.011, 2.510 73916, 73945, 73931, 0.011, 2.427 73946, 73975, 73961, 0.001, 2.371 73976, 74005, 73991, 0.001, 2.315 74006, 74035, 74021, 0.001, 2.316 74036, 74065, 74051, 0.012, 2.265 74066, 74095, 74081, 0.012, 1.726 74096, 74125, 74111, 0.016, 1.186 74126, 74155, 74141, 0.016, 1.500 74156, 74185, 74171, 0.026, 1.794 74186, 74215, 74201, 0.004, 1.565 74216, 74245, 74231, 0.004, 1.338 74246, 74275, 74261, 0.004, 1.632 74276, 74305, 74291, 0.020, 1.505 74307, 74336, 74322, 0.020, 1.449 74337, 74366, 74352, 0.006, 1.392 74367, 74396, 74382, 0.006, 1.466 74397, 74426, 74412, 0.003, 1.152 74427, 74456, 74442, 0.003, 1.358 74457, 74486, 74472, 0.013, 1.564 74487, 74516, 74502, 0.023, 1.097 74517, 74546, 74532, 0.023, 2.039 74547, 74576, 74562, 0.040, 2.001 74577, 74606, 74592, 0.040, 1.964 74607, 74636, 74622, 0.040, 1.768 74637, 74666, 74652, 0.021, 1.712 74667, 74696, 74682, 0.021, 1.601 74697, 74726, 74712, 0.044, 1.491 74727, 74756, 74742, 0.044, 1.806 74757, 74786, 74772, 0.029, 1.838 74787, 74816, 74802, 0.029, 1.502 74817, 74846, 74832, 0.013, 1.166 74847, 74876, 74862, 0.022, 2.062 74877, 74906, 74892, 0.022, 1.786 74907, 74936, 74922, 0.031, 1.618 74937, 74966, 74952, 0.031, 1.450 74967, 74996, 74982, 0.028, 1.715 74997, 75026, 75012, 0.028, 1.325 75027, 75056, 75042, 0.028, 1.461 75057, 75086, 75072, 0.031, 1.596 75186, 75215, 75201, 0.038, 2.433 75216, 75245, 75231, 0.038, 2.377 75246, 75275, 75261, 0.038, 2.461 75276, 75305, 75291, 0.063, 2.544 75306, 75335, 75321, 0.099, 2.860 75336, 75365, 75351, 0.099, 2.442 75366, 75395, 75381, -9999.000, 2.280 75396, 75425, 75411, -9999.000, 2.119 75426, 75455, 75441, -9999.000, 2.924 75456, 75485, 75471, -9999.000, 2.057 75486, 75515, 75501, -9999.000, 2.293 75516, 75545, 75531, -9999.000, 2.530 75546, 75575, 75561, -9999.000, 2.733 75577, 75606, 75592, -9999.000, 2.574 75607, 75636, 75622, 0.018, 2.451 75637, 75666, 75652, 0.018, 2.327 75667, 75696, 75682, 0.018, 2.547 75697, 75726, 75712, 0.035, 2.642 75727, 75756, 75742, 0.035, 2.458 75757, 75786, 75772, 0.055, 2.274 75787, 75816, 75802, 0.055, 2.052 75817, 75846, 75832, 0.053, 2.832 75847, 75876, 75862, 0.053, 2.188 75877, 75906, 75892, 0.063, 1.545 75907, 75936, 75922, 0.063, 2.081 75937, 75966, 75952, 0.085, 1.522 75967, 75996, 75982, 0.085, 1.683 75997, 76026, 76012, 0.078, 1.844 76027, 76056, 76042, 0.078, 1.859 76057, 76086, 76072, 0.097, 1.769 76087, 76116, 76102, 0.097, 1.783 76117, 76146, 76132, 0.067, 1.798 76147, 76176, 76162, 0.073, 1.884 76177, 76206, 76192, 0.073, 2.014 76207, 76236, 76222, 0.054, 1.742 76237, 76266, 76252, 0.054, 1.470 76267, 76296, 76282, 0.054, 1.402 76297, 76326, 76312, 0.062, 1.543 76328, 76357, 76343, 0.074, 1.399 76358, 76387, 76373, 0.074, 1.255 76388, 76417, 76403, 0.074, 1.693 76418, 76447, 76433, 0.048, 1.566 76448, 76477, 76463, 0.053, 1.583 76478, 76507, 76493, 0.053, 1.600 76508, 76537, 76523, 0.077, 1.917 76538, 76567, 76553, 0.077, 1.890 76568, 76597, 76583, 0.077, 1.648 76598, 76627, 76613, 0.080, 1.405 76628, 76657, 76643, 0.095, 1.828 76658, 76687, 76673, 0.095, 1.721 76688, 76717, 76703, 0.095, 1.651 76718, 76747, 76733, 0.102, 1.580 76748, 76777, 76763, 0.102, 1.748 76778, 76807, 76793, 0.097, 1.908 76808, 76837, 76823, 0.097, 1.612 76838, 76867, 76853, 0.069, 1.316 76868, 76897, 76883, 0.099, 1.655 76898, 76927, 76913, 0.099, 1.276 76928, 76957, 76943, 0.099, 1.336 76958, 76987, 76973, 0.080, 1.397 76988, 77017, 77003, 0.080, 1.798 77018, 77047, 77033, 0.046, 2.011 77048, 77077, 77063, 0.046, 1.845 77079, 77108, 77094, 0.080, 1.679 77109, 77138, 77124, 0.080, 1.856 77139, 77168, 77154, 0.051, 1.716 77169, 77198, 77184, 0.051, 1.358 77199, 77228, 77214, 0.060, 1.000 77229, 77258, 77244, 0.061, 1.563 77259, 77288, 77274, 0.061, 1.894 77289, 77318, 77304, 0.057, 1.914 77319, 77348, 77334, 0.057, 1.934 77349, 77378, 77364, 0.057, 2.373 77379, 77408, 77394, 0.033, 2.059 77409, 77438, 77424, 0.048, 1.876 77439, 77468, 77454, 0.048, 1.693 77469, 77498, 77484, 0.048, 1.769 77499, 77528, 77514, 0.019, 2.055 77529, 77558, 77544, 0.058, 1.880 77559, 77588, 77574, 0.058, 1.707 77589, 77618, 77604, 0.058, 2.226 77619, 77648, 77634, 0.042, 2.048 77649, 77678, 77664, 0.042, 1.753 77679, 77708, 77694, -0.001, 1.456 77709, 77738, 77724, 0.004, 2.238 77739, 77768, 77754, 0.004, 1.869 77769, 77798, 77784, 0.004, 1.785 77799, 77828, 77814, 0.018, 1.702 77830, 77859, 77845, -0.002, 2.379 77860, 77889, 77875, -0.002, 2.487 77890, 77919, 77905, -0.002, 2.207 77920, 77949, 77935, -9999.000, 1.927 77950, 77979, 77965, -9999.000, 1.260 77980, 78009, 77995, -9999.000, 3.000 78010, 78039, 78025, -9999.000, 2.096 78040, 78069, 78055, -9999.000, 1.196 78070, 78099, 78085, -9999.000, 3.245 78100, 78129, 78115, -9999.000, 2.086 78130, 78159, 78145, -9999.000, 1.379 78160, 78189, 78175, -9999.000, 0.674 78190, 78219, 78205, -9999.000, 1.885 78220, 78249, 78235, -9999.000, 1.634 78250, 78279, 78265, -9999.000, 1.961 78280, 78309, 78295, -9999.000, 2.289 78310, 78339, 78325, -9999.000, 1.284 78340, 78369, 78355, -9999.000, 1.972 78370, 78399, 78385, -9999.000, 1.523 78400, 78429, 78415, -9999.000, 1.074 78430, 78459, 78445, -9999.000, 2.836 78460, 78489, 78475, -9999.000, -9999.000 78490, 78519, 78505, -9999.000, 0.630 78520, 78549, 78535, -9999.000, 2.484 78550, 78579, 78565, -9999.000, 2.133 78581, 78610, 78596, -9999.000, 1.138 78611, 78640, 78626, -9999.000, 1.093 78641, 78670, 78656, -9999.000, 1.048 78671, 78700, 78686, -9999.000, 3.667 78701, 78730, 78716, -9999.000, 2.728 78731, 78760, 78746, -9999.000, 2.286 78761, 78790, 78776, -9999.000, 1.844 78791, 78820, 78806, -9999.000, -9999.000 78821, 78850, 78836, -9999.000, 1.416 78851, 78880, 78866, -9999.000, -0.324 78881, 78910, 78896, -9999.000, -9999.000 78911, 78940, 78926, 0.099, -0.242 78941, 78970, 78956, 0.099, 0.872 78971, 79000, 78986, 0.099, 1.413 79001, 79030, 79016, 0.047, 1.954 79031, 79060, 79046, 0.047, 2.076 79061, 79090, 79076, 0.056, 1.514 79091, 79120, 79106, 0.055, 1.442 79121, 79150, 79136, 0.055, 1.370 79151, 79180, 79166, 0.055, 1.676 79181, 79210, 79196, 0.100, 0.523 79211, 79240, 79226, 0.092, 0.543 79241, 79270, 79256, 0.092, 0.564 79271, 79300, 79286, 0.092, 0.806 79301, 79330, 79316, 0.111, 0.458 79331, 79360, 79346, 0.111, 0.585 79362, 79391, 79377, 0.111, 0.712 79392, 79421, 79407, 0.161, 0.870 79422, 79451, 79437, 0.161, 0.961 79452, 79481, 79467, 0.116, 1.018 79482, 79511, 79497, 0.116, 1.074 79512, 79541, 79527, 0.088, 1.556 79542, 79571, 79557, 0.088, 1.587 79572, 79601, 79587, 0.088, 1.364 79602, 79631, 79617, 0.095, 1.140 79632, 79661, 79647, 0.095, 1.541 79662, 79691, 79677, 0.088, 1.417 79692, 79721, 79707, 0.083, 1.414 79722, 79751, 79737, 0.083, 1.411 79752, 79781, 79767, 0.067, 1.897 79782, 79811, 79797, 0.067, 1.822 79812, 79841, 79827, 0.067, 1.387 79842, 79871, 79857, 0.109, 0.948 79872, 79901, 79887, 0.109, 1.697 79902, 79931, 79917, 0.075, 1.509 79932, 79961, 79947, 0.075, 1.748 79962, 79991, 79977, 0.039, 1.986 79992, 80021, 80007, 0.082, 2.029 80022, 80051, 80037, 0.082, 1.484 80052, 80081, 80067, 0.088, 1.336 80082, 80111, 80097, 0.088, 1.187 80113, 80142, 80128, 0.084, 1.412 80143, 80172, 80158, 0.084, 1.632 80173, 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