46, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor ATom 1, 1 2017, 02, 21, 2018, 10, 25 0 Start_UTC, seconds, seconds since UTC midnight on day of takeoff 4 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since UTC midnight on day of takeoff Mid_UTC, seconds, seconds since UTC midnight on day of takeoff OH_ATHOS, pptv, OH mixing ratio in pptv HO2_ATHOS, pptv, HO2 mixing ratio in pptv 0 28 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom II: Science Flight #11 -- ANC - PMD ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 from Laser Induced Fluorescence. DATA_INFO: Units are pptv for OH and HO2. UNCERTAINTY: HOx absolute accuracy ~+/- 32% (actually a multiplicative factor of 1/1.32 to 1.32), 2 sigma confidence. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Final Data. Future modifications to the calibration are possible but unlikely. - Calibrating ATHOS with the new OH-removing inlet (OHSI) has been difficult, particularly for low pressure (high altitude). - The ATHOS HOx calibrations are pressure-dependent, changing a factor of 3-5 over the atmospheric pressure range. - The laboratory calibration uses different inlet hole sizes to simulate atmospheric pressure changes. - For 2 years, we tried various calibration approaches with the OHSI in place, but none gave repeatable results for high altitude measurements. - In the laboratory calibrations, it proved to be impossible to simulate the atmospheric airflow with the OHSI on and the smaller inlet sizes. - In the end, we found that our previous calibration method gave the most repeatable and reliable results. - In-flight diagnostics show that OH loss on the OHSI is negligible. - For details, please see Faloona et al., J. Atmos. Chem., 47, 139-167, 2004. REVISION: R2 R2: Final Data (see OTHER_COMMENTS) R1: Final Data R0: No comments for this revision. Start_UTC, Stop_UTC, Mid_UTC, OH_ATHOS, HO2_ATHOS 64856, 64875, 64866, -9999.000, -9999.000 64876, 64895, 64886, -9999.000, -9999.000 64896, 64915, 64906, -9999.000, -9999.000 64916, 64935, 64926, -9999.000, -9999.000 64936, 64955, 64946, -9999.000, -9999.000 64956, 64975, 64966, -9999.000, -9999.000 64976, 64995, 64986, 0.024, 0.935 64996, 65015, 65006, 0.024, 0.366 65016, 65035, 65026, 0.031, 0.738 65036, 65055, 65046, 0.016, 1.111 65056, 65075, 65066, 0.016, 0.972 65076, 65095, 65086, -0.010, 1.471 65096, 65115, 65106, -0.010, 1.280 65116, 65135, 65126, -0.010, 1.088 65137, 65156, 65147, -0.035, 0.531 65157, 65176, 65167, -0.007, 0.250 65177, 65196, 65187, -0.007, 0.272 65197, 65216, 65207, -0.007, 0.295 65217, 65236, 65227, 0.015, 0.361 65237, 65256, 65247, 0.015, 0.428 65257, 65276, 65267, 0.023, 0.495 65277, 65296, 65287, 0.023, 0.561 65297, 65316, 65307, 0.044, 0.629 65317, 65336, 65327, 0.044, 0.695 65337, 65356, 65347, 0.005, 0.762 65357, 65376, 65367, 0.005, 0.829 65377, 65396, 65387, 0.006, 0.896 65397, 65416, 65407, 0.013, 1.226 65417, 65436, 65427, 0.013, 1.751 65437, 65456, 65447, 0.012, 2.277 65457, 65476, 65467, 0.012, 1.282 65477, 65496, 65487, 0.012, 1.157 65497, 65516, 65507, 0.025, 1.298 65517, 65536, 65527, 0.000, 1.437 65537, 65556, 65547, 0.000, 1.577 65557, 65576, 65567, 0.000, 1.783 65577, 65596, 65587, 0.032, 1.618 65597, 65616, 65607, 0.007, 1.452 65617, 65636, 65627, 0.007, 1.372 65637, 65656, 65647, 0.007, 1.393 65657, 65676, 65667, -0.009, 1.287 65677, 65696, 65687, 0.015, 1.181 65697, 65716, 65707, 0.015, 1.075 65717, 65736, 65727, -0.006, 1.364 65737, 65756, 65747, -0.006, 1.270 65757, 65776, 65767, 0.016, 1.176 65777, 65796, 65787, 0.016, 0.942 65797, 65816, 65807, 0.016, 0.770 65817, 65836, 65827, 0.018, 0.868 65837, 65856, 65847, 0.018, 0.966 65857, 65876, 65867, -0.002, 1.064 65877, 65896, 65887, -0.002, 0.373 65898, 65917, 65908, 0.026, 0.691 65918, 65937, 65928, 0.026, 1.006 65938, 65957, 65948, 0.004, 1.247 65958, 65977, 65968, -0.008, 1.269 65978, 65997, 65988, -0.008, 1.343 65998, 66017, 66008, -0.008, 1.418 66018, 66037, 66028, 0.009, 1.493 66038, 66057, 66048, 0.009, 2.371 66058, 66077, 66068, 0.008, 2.047 66078, 66097, 66088, 0.011, 1.724 66098, 66117, 66108, 0.011, 1.444 66118, 66137, 66128, 0.011, 2.050 66138, 66157, 66148, 0.042, 1.511 66158, 66177, 66168, 0.039, 0.967 66178, 66197, 66188, 0.039, 0.428 66198, 66217, 66208, 0.044, 0.520 66218, 66237, 66228, 0.044, 0.653 66238, 66257, 66248, 0.028, 0.785 66258, 66277, 66268, 0.028, 0.481 66278, 66297, 66288, 0.028, 0.722 66298, 66317, 66308, 0.042, 0.716 66318, 66337, 66328, 0.042, 0.709 66338, 66357, 66348, 0.036, 0.703 66358, 66377, 66368, 0.037, 0.784 66378, 66397, 66388, 0.037, 0.879 66398, 66417, 66408, 0.037, 0.974 66493, 66512, 66503, 0.048, 0.996 66513, 66532, 66523, 0.026, 1.221 66533, 66552, 66543, 0.026, 1.033 66553, 66572, 66563, 0.026, 0.846 66573, 66592, 66583, 0.030, 0.657 66593, 66612, 66603, 0.035, 1.320 66613, 66632, 66623, 0.035, 1.093 66633, 66652, 66643, 0.035, 0.865 66653, 66672, 66663, 0.013, 1.285 66673, 66692, 66683, 0.013, 1.424 66693, 66712, 66703, 0.019, 1.322 66713, 66732, 66723, 0.019, 1.220 66733, 66752, 66743, 0.031, 1.118 66753, 66772, 66763, 0.031, 1.065 66773, 66792, 66783, 0.017, 1.303 66793, 66812, 66803, 0.026, 1.541 66813, 66832, 66823, 0.026, 1.119 66833, 66852, 66843, 0.026, 1.192 66853, 66872, 66863, 0.056, 1.124 66873, 66892, 66883, 0.032, 1.056 66893, 66912, 66903, 0.032, 0.988 66914, 66933, 66924, 0.045, 1.386 66934, 66953, 66944, 0.045, 1.396 66954, 66973, 66964, 0.057, 1.405 66974, 66993, 66984, 0.057, 1.248 66994, 67013, 67004, 0.057, 1.289 67014, 67033, 67024, 0.041, 1.402 67034, 67053, 67044, 0.041, 1.514 67054, 67073, 67064, 0.018, 1.628 67074, 67093, 67084, 0.018, 3.436 67094, 67113, 67104, 0.040, 3.207 67114, 67133, 67124, 0.042, 2.977 67134, 67153, 67144, 0.042, 3.307 67154, 67173, 67164, 0.042, 4.223 67174, 67193, 67184, 0.009, 3.812 67194, 67213, 67204, 0.010, 3.400 67214, 67233, 67224, 0.010, 2.990 67234, 67253, 67244, 0.010, 3.345 67254, 67273, 67264, 0.012, 3.119 67274, 67293, 67284, 0.056, 2.894 67294, 67313, 67304, 0.056, 2.639 67314, 67333, 67324, 0.056, 3.441 67334, 67353, 67344, 0.013, 3.228 67354, 67373, 67364, 0.034, 3.015 67374, 67393, 67384, 0.034, 2.803 67394, 67413, 67404, 0.034, 3.041 67414, 67433, 67424, 0.012, 2.625 67434, 67453, 67444, 0.012, 2.209 67455, 67474, 67465, 0.006, 2.118 67475, 67494, 67485, 0.007, 2.428 67495, 67514, 67505, 0.007, 2.097 67515, 67534, 67525, 0.007, 1.767 67535, 67554, 67545, 0.024, 1.436 67555, 67574, 67565, -0.019, 1.814 67575, 67594, 67585, -0.019, 1.582 67595, 67614, 67605, -0.019, 1.349 67615, 67634, 67625, 0.019, 1.621 67635, 67654, 67645, 0.019, 2.156 67655, 67674, 67665, -0.017, 1.887 67675, 67694, 67685, -0.017, 1.619 67695, 67714, 67705, 0.004, 1.350 67715, 67734, 67725, 0.004, 1.689 67735, 67754, 67745, 0.020, 2.325 67755, 67774, 67765, -0.007, 2.960 67775, 67794, 67785, -0.007, 2.361 67795, 67814, 67805, -0.007, 2.454 67815, 67834, 67825, -9999.000, 2.359 67835, 67854, 67845, -9999.000, 2.264 67855, 67874, 67865, -9999.000, 2.168 67875, 67894, 67885, -9999.000, 2.753 67895, 67914, 67905, 0.013, 2.625 67915, 67934, 67925, 0.018, 2.499 67935, 67954, 67945, 0.018, 2.069 67955, 67974, 67965, 0.018, 2.230 67975, 67994, 67985, 0.114, 2.044 67995, 68014, 68005, 0.114, 1.860 68015, 68034, 68025, 0.006, 1.675 68035, 68054, 68045, 0.006, 1.428 68150, 68169, 68160, 0.020, 1.885 68170, 68189, 68180, 0.048, 1.965 68190, 68209, 68200, 0.048, -9999.000 68211, 68230, 68221, 0.048, -9999.000 68231, 68250, 68241, 0.065, -9999.000 68251, 68270, 68261, 0.105, -9999.000 68271, 68290, 68281, 0.105, -9999.000 68291, 68310, 68301, 0.105, -9999.000 68311, 68330, 68321, -9999.000, -9999.000 68331, 68350, 68341, -9999.000, -9999.000 68351, 68370, 68361, 0.012, -9999.000 68371, 68390, 68381, -0.015, -9999.000 68391, 68410, 68401, -0.015, -9999.000 68411, 68430, 68421, -0.015, -9999.000 68431, 68450, 68441, 0.068, -9999.000 68451, 68470, 68461, 0.068, 2.299 68471, 68490, 68481, -0.004, 1.762 68491, 68510, 68501, -0.004, 1.225 68511, 68530, 68521, 0.092, 1.227 68531, 68550, 68541, 0.073, 1.481 68551, 68570, 68561, 0.073, 1.433 68571, 68590, 68581, 0.073, 1.385 68591, 68610, 68601, -9999.000, 1.337 68611, 68630, 68621, -9999.000, 1.631 68631, 68650, 68641, -9999.000, 1.359 68651, 68670, 68661, -0.010, 1.084 68671, 68690, 68681, -0.010, 1.846 68691, 68710, 68701, 0.022, 0.990 68711, 68730, 68721, 0.022, 1.298 68731, 68750, 68741, 0.022, 1.605 68751, 68770, 68761, -0.015, 1.913 68771, 68790, 68781, 0.026, 2.996 68791, 68810, 68801, 0.026, 2.693 68811, 68830, 68821, 0.026, 2.391 68831, 68850, 68841, 0.028, 2.654 68851, 68870, 68861, 0.019, 2.047 68871, 68890, 68881, 0.019, 2.030 68891, 68910, 68901, 0.019, 2.013 68911, 68930, 68921, 0.028, 1.996 68932, 68951, 68942, 0.014, 1.805 68952, 68971, 68962, 0.014, 2.376 68972, 68991, 68982, 0.014, 2.948 68992, 69011, 69002, 0.007, 2.862 69012, 69031, 69022, -0.004, 2.729 69032, 69051, 69042, -0.004, 2.852 69052, 69071, 69062, 0.010, 2.977 69072, 69091, 69082, 0.010, 3.101 69092, 69111, 69102, 0.041, 3.770 69112, 69131, 69122, 0.041, 4.603 69132, 69151, 69142, 0.041, 5.435 69152, 69171, 69162, 0.007, 4.474 69172, 69191, 69182, 0.007, 3.928 69192, 69211, 69202, 0.020, 3.923 69212, 69231, 69222, 0.017, 3.917 69232, 69251, 69242, 0.017, 3.912 69252, 69271, 69262, 0.017, 4.187 69272, 69291, 69282, 0.028, 4.152 69292, 69311, 69302, 0.028, 4.118 69312, 69331, 69322, 0.024, 4.350 69332, 69351, 69342, 0.051, 4.060 69352, 69371, 69362, 0.051, 3.993 69372, 69391, 69382, 0.003, 3.926 69392, 69411, 69402, 0.003, 3.859 69412, 69431, 69422, 0.003, 3.953 69432, 69451, 69442, 0.041, 4.205 69452, 69471, 69462, 0.024, 4.456 69472, 69491, 69482, 0.024, 3.709 69492, 69511, 69502, 0.043, 4.762 69512, 69531, 69522, 0.043, 4.695 69532, 69551, 69542, 0.043, 4.627 69552, 69571, 69562, 0.063, 4.559 69572, 69591, 69582, 0.063, 4.117 69592, 69611, 69602, 0.042, 4.244 69612, 69631, 69622, 0.055, 4.371 69632, 69651, 69642, 0.055, 4.241 69652, 69671, 69662, 0.055, 3.902 69672, 69691, 69682, 0.143, 3.735 69692, 69711, 69702, 0.147, 3.569 69712, 69731, 69722, 0.147, 3.403 69732, 69751, 69742, 0.177, 3.412 69752, 69771, 69762, 0.177, 2.838 69772, 69791, 69782, 0.177, 2.264 69792, 69811, 69802, 0.145, 2.040 69812, 69831, 69822, 0.145, 2.264 69833, 69852, 69843, 0.129, 2.205 69853, 69872, 69863, 0.129, 2.146 69873, 69892, 69883, 0.125, 2.087 69893, 69912, 69903, 0.137, 1.871 69913, 69932, 69923, 0.137, 2.403 69933, 69952, 69943, 0.137, 2.935 69953, 69972, 69963, 0.142, 2.722 69973, 69992, 69983, 0.099, 2.139 69993, 70012, 70003, 0.099, 1.840 70013, 70032, 70023, 0.105, 1.541 70033, 70052, 70043, 0.105, 1.242 70135, 70154, 70145, 0.089, 1.869 70155, 70174, 70165, 0.089, 1.667 70175, 70194, 70185, 0.099, 1.467 70195, 70214, 70205, 0.099, 1.157 70215, 70234, 70225, 0.099, 1.072 70235, 70254, 70245, 0.094, 1.230 70255, 70274, 70265, 0.094, 1.388 70275, 70294, 70285, 0.083, 1.546 70296, 70315, 70306, 0.081, 1.271 70316, 70335, 70326, 0.081, 1.551 70336, 70355, 70346, 0.084, 1.833 70356, 70375, 70366, 0.084, 1.550 70376, 70395, 70386, 0.141, 1.372 70396, 70415, 70406, 0.141, 1.748 70416, 70435, 70426, 0.141, 2.125 70436, 70455, 70446, 0.149, 2.503 70456, 70475, 70466, 0.149, 1.971 70476, 70495, 70486, 0.153, 2.308 70496, 70515, 70506, 0.161, 2.645 70516, 70535, 70526, 0.161, 2.244 70536, 70555, 70546, 0.161, 2.622 70556, 70575, 70566, 0.101, 3.093 70576, 70595, 70586, 0.025, 3.559 70596, 70615, 70606, 0.025, 4.026 70616, 70635, 70626, 0.041, 4.729 70636, 70655, 70646, 0.041, 4.860 70656, 70675, 70666, 0.043, 4.991 70676, 70695, 70686, 0.043, 4.122 70696, 70715, 70706, 0.043, 4.005 70716, 70735, 70726, 0.047, 3.695 70736, 70755, 70746, 0.039, 3.386 70756, 70775, 70766, 0.039, 3.077 70776, 70795, 70786, 0.039, 3.380 70796, 70815, 70806, -0.000, 3.949 70816, 70835, 70826, -0.000, 4.513 70836, 70855, 70846, 0.035, 3.719 70856, 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