83, 1001
Jimenez, Jose Luis
CIRES and Department of Chemistry, University of Colorado Boulder
Chemically speciated submicron non-refractory particulate mass, 60 s resolution
ATom
1, 1
2016, 08, 15, 2017, 06, 05
0
AMS_Starttime_60s, seconds_past_midnight, UTC_start_time_in_seconds_from_midnight
48
1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1, 1
-9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999, -9999
AMS_Stoptime_60s, seconds_past_midnight, UTC_end_time_in_seconds_from_midnight
AMS_MidPointTime_60s, seconds_past_midnight, UTC_midpoint_time_in_seconds_from_midnight
AMS_LAT_60s, deg, Aircraft_latitude_at_time_of_sampling
AMS_LON_60s, deg, Aircraft_longitude_at_time_of_sampling
AMS_ALT_60s, m, Aircraft_GPS_altitude_at_time_of_sampling
OA_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_organic_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
OA_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_the_mass_concentration_of_organic_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
OA_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_organic_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Sulfate_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_sulfate_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Sulfate_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_mass_concentration_of_sulfate_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Sulfate_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_sulfate_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Ammonium_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_nitrate_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Ammonium_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_mass_concentration_of_nitrate_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Ammonium_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_nitrate_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Nitrate_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_ammonium_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Nitrate_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_mass_concentration_of_ammonium_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Nitrate_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_ammonium_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Chloride_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_chloride_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Chloride_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_mass_concentration_of_chloride_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Chloride_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_chloride_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Seasalt_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_seasalt_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Seasalt_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_mass_concentration_of_seasalt_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
Seasalt_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_seasalt_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
MSA_lt_1um_AMS_60s, ug sm-3, Mass_concentration_of_MSA_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
MSA_lt_1um_AMS_prec_60s, ug sm-3, 1s_precision_error_of_mass_concentration_of_MSA_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
MSA_lt_1um_AMS_DL_60s, ug sm-3, Detection_limit_for_the_mass_concentration_of_MSA_aerosol_in_air_for_particle_diameter_less_than_1um_measured_by_HRAMS
StdtoVol_AMS_60s, m3 sm-3, Conversion_factor_from_std_to_ambient_volume_and_pressure
IceFlag_AMS_60s, unitless, Datapoints_suspected_to_be_impacted_by_artifacts_due_to_ice_impaction_on_the_inlet
AmmBalance_lt_1um_AMS_60s, unitless, Ammonium_Molar_Balance_for_non_refractory_inorganic_species_less_than_1um_measured_by_HRAMS
Density_lt_1um_AMS_60s, g cm-3, Estimated_aerosol_density_assuming_internally_mixed_aerosol_for_particle_diameter_less_than_1um_measured_by_HRAMS
OADensity_lt_1um_AMS_60s, g cm-3, Estimated_density_of_the_organic_aerosol_fraction_assuming_internally_mixed_aerosol_for_particle_diameter_less_than_1um_measured_by_HRAMS
O_C_lt_1um_AMS_60s, unitless, O/C_atomic_ratio_of_the_organic_mass_fraction_of_the_aerosol_for_particle_diameter_less_than_1um_measured_by_HRAMS
H_C_lt_1um_AMS_60s, unitless, H/C_atomic_ratio_of_the_organic_mass_fraction_of_the_aerosol_for_particle_diameter_less_than_1um_measured_by_HRAMS
OA_OC_lt_1um_AMS_60s, unitless, Organic_aerosol_to_organic_carbon_ratio_of_the_organic_mass_fraction_of_the_aerosol_for_particle_diameter_less_than_1um_measured_by_HRAMS
OSc_lt_1um_AMS_60s, unitless, Estimated_average_oxidation_state_of_carbon_of_the_organic_mass_fraction_of_the_aerosol_for_particle_diameter_less_than_1um_measured_by_HRAMS
f43_lt_1um_AMS_60s, unitless, Fractional_contribution_of_m/z_43_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
f44_lt_1um_AMS_60s, unitless, Fractional_contribution_of_m/z_44_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
f57_lt_1um_AMS_60s, unitless, Fractional_contribution_of_m/z_57_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
f60_lt_1um_AMS_60s, unitless, Fractional_contribution_of_m/z_60_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
f82_lt_1um_AMS_60s, unitless, Fractional_contribution_of_m/z_82_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
f91_lt_1um_AMS_60s, unitless, Fractional_contribution_of_m/z_91_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
fC2H3O_lt_1um_AMS_60s, unitless, Fractional_contribution_of_C2H3O+_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
fCO2_lt_1um_AMS_60s, unitless, Fractional_contribution_of_CO2+_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
fC4H9_lt_1um_AMS_60s, unitless, Fractional_contribution_of_C4H9+_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
fC2H4O2_lt_1um_AMS_60s, unitless, Fractional_contribution_of_C2H4O2+_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
fC5H6O_lt_1um_AMS_60s, unitless, Fractional_contribution_of_C5H6O+_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
fC7H7_lt_1um_AMS_60s, unitless, Fractional_contribution_of_C7H7+_to_total_organic_mass_for_particle_diameter_less_than_1um_measured_by_HRAMS
OrgNitr_Fraction_lt_1um_AMS_60s, unitless, Estimated_organic_nitrate_fractional_contribution_to_total_aerosol_nitrate_mass_by_HRAMS
1
N/A
20
PI_CONTACT_INFO: Jose-Luis Jimenez, jose.jimenez@colorado.edu, Address: University of Colorado UCB 216; CIRES Bldg., Boulder, CO 80309-0216, phone +1-303-492-3557, fax +1-303-492-1149
PLATFORM: NASA DC-8 Aircraft 
LOCATION: Airports serving as home base on this deployment: PMD, ANC, KOA, PPG, CHC, PUQ, ASI, TER, THU, ANC, PMD 
ASSOCIATED_DATA: N/A
INSTRUMENT_INFO: NSTRUMENT_INFO: AMS_Type=V; Ionization_type=EI; AMS_SamplingTime: 46 s; AMS_SamplingCycle: Fast Mode, 6 s closed and 46 s open (+5 s PToF, reported under a different DataID) , 1 min synchronization clock; AMS_LensType=standard; AMS_LensPressure=1.50 Torr (actively controlled); AMS_FlowRate=92.5 sccm; AMS_PrsTempFlowCal: 273K, 1 bar; AMS_STPConversionFactor=StdtoVol_AMS; AMS_Calibrations: AN mass Calibration (400 nm particles) after every flight; Chloride and sulfate RIE, as well a PSL size calibration (100-900 nm), at regular intervals; AMS_FilEmmCurr = 1.4 mA (actively controlled); AMS_DAQType = ADQ_1600; AMS_IEOverAB=9.34e-13; AMS_RIENH4=3.65; AMS_RIESO4=1.57; AMS_RIEChl=1.96 (based on in-field calibrations); AMS_CE: Calculated using the algorithm from Middlebrook et al 2012, AS&T 46, 258–271 [https://doi.org/10.1080/02786826.2011.620041] using 1 min data; AMS_PMCut= ~1 um vacuum aerodynamic, based on in-field calibration; AMS_InletRH: < 50%; AMS_PieberCorr=0.73% (as discussed in Pieber et al 2016, ES&T 50 (19), 10494–10503 [https://doi.org/10.1021/acs.est.6b01035]; AMS_HuCorr=1.3% (as discussed in Hu et al 2017, AS&T 51 [https://doi.org/ DOI:10.1080/02786826.2017.1296104)
DATA_INFO: Only brief explanations are provided here. Please refer to http://tinyurl.com/FAQ-AMS-Data for additional topics and more detailed explanations, and contact the PIs if in doubt. Both that web page and this header are updated regularly in response to questions from data users and/or new information about the instrument and data interpretation. All concentration data is reported under STP (273 K & 1013 mb); use provided conversion factor to calculate under ambient temperature and pressure. Note that several other definitions of standard conditions are in use by others in the community, and some groups and models report under ambient and not standard conditions--check carefully before comparing!! Data was taken on a 1 min clock with 6 s background and 46 s ambient measurements, reported in 46 s increments. IMPORTANT: All reported data in this file is derived by analyzing the averaged raw spectra at 60 s resolution, it is NOT an arithmetic average of the data reported under the AMS Id. Hence it has higher S/N than the simple average and should be preferentially used for longer timescales. The remaining time was either instrument overhead or was spent taking particle size segregated data (reported in a separate data id). Time base is corrected for inlet lag (about 0.4 s in the BL). Latitude, Longitude and GPS Altitude are provided (inlet lag adjusted) from the instruments' own GPS datafeed. All reported data (including the individual f_x marker fractions) are derived from fitting individual HR ions using PIKA 1.19E, and NOT by using the unit mass resolution (UMR) signal (“Squirrel” in AMS parlance). Unlike the aerosol species concentrations (extensive properties), all the variables (intensive properties) detailing the chemical composition of the organic fraction were thresholded for the organic detection limit to avoid averaging artifacts; the thresholded data should be averaged to slower time resolutions with OA mass weighting. Reported aerosol density is estimated for non-refractory material assuming an internally mixed aerosol, following the method of Salcedo et al 2006, ACP 6, 925–946 [https://doi.org/doi:10.5194/acp-6-925-2006]; the density of the organic fraction is estimated with the expression provided in Kuwata et al 2012, ES&T 46, 787-794 [https://doi.org/10.1021/es202525q]. Only species above DL are included in the density calculation. Atomic O/C, H/C and OA/OC ratios are reported using the new calibration proposed by Canagaratna, Jimenez et al. 2015, ACP 15, 253-272 [https://doi.org/10.5194/acp-15-253-2015], which results in, on average, 28% higher O/C and 7% higher H/C ratios than using the Aiken et al 2008, ES&T 42, 4478–4485 [https://doi.org/10.1021/es703009q] method. Oxidation State of OA provided according to the approximate formula of Kroll et al 2011, Nat. Chem. 3, 133-139, 2011 [https://doi.org/10.1038/nchem.948] using the new calibration described in Canagaratna, Jimenez et al. 2015 . The molar ion balance of the inorganic species (“Ammonium Balance”) is provided as a rough proxy for aerosol acidity; we also provide a modeled pH product (reported in the final data) that is in general more meaningful. An IceFlag (based on AMS measurements of particulate water and Zinc) is included to identify periods when artifacts due to ice impaction on the inlet (not shared with the other aerosol instruments on the plane) were observed; in general, AMS data seems to be impacted to a much lesser extent by these artifacts than other instruments, but extra caution should be exercised when using data from these periods. An organic nitrate fraction is included as an experimental product (1 min resolution due to the lower signal-to-noise of this product), see Fry et al 2013, ACP 13, 8585-8605 [https://doi.org/10.5194/acp-13-8585-2013] for details; organic nitrate fraction data is not reported during elevated dust or sea salt episodes that lead to significant interferences. In some cases the measured nitrate might also include nitrite, although the presence of nitrite in submicron aerosols is very unusual in our experience (see Guo et al. 2016, JGR 121, 10355-10376 [https://doi.org/10.1002/2016JD025311]). Two new aerosol species are being reported as part of this dataset, submicron seasalt and submicron particulate MSA. Both of these data products have been calibrated with laboratory standards, and validated by comparison with the PALMS instrument, but they are still considered experimental and carry a larger uncertainty (+/-60%) than standard AMS products. Submicron seasalt is reported following the method from Ovadnevaite et al, JGR 2012, 117 (D16), 1–11 [ https://doi.org/10.1029/2011JD017379]. For this species, cloud artifacts are actually observed, and the data has hence been filtered by the AMS cloudflag variable. MSA was quantified based on the CH3SO2+ AMS ion, which is specific to MSA and was calibrated using laboratory standards, following Zorn et al ACP 2008, 8, 4711-4128 [ https://doi.org/10.5194/acp-8-4711-2008].
UNCERTAINTY: Accuracy estimate (2sdev): Inorganics +/-34%, Organics +/-38%, dominated by uncertainty in particle collection efficiency due to particle bounce, and absolute and relative ionization efficiency, as estimated in Bahreini et al. 2009, JGR 114, D00F16 (Supp. Info.)[https://doi.org/10.1029/2008JD011493]. Precision error (1sdev) for each species is provided as a separate variable. Continuous detection Limits are estimated based on the method of Drewnick et al, AMT 2, 33-46, 2009 [https://doi.org/10.5194/amt-2-33-2009] and were corrected by comparison with frequent, periodic blanks. 
ULOD_FLAG: -7777
ULOD_VALUE: N/A
LLOD_FLAG: -8888
LLOD_VALUE: -9999, -9999, -9999, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888, -8888
DM_CONTACT_INFO: Pedro Campuzano Jost, Pedro.CampuzanoJost-1@colorado.edu, Address: University of Colorado UCB 216; CIRES Bldg., Boulder, CO 80309-0216, phone +1-303-492-9599, fax +1-303-492-1149
PROJECT_INFO: NASA ATom-1 Mission, July-August 2016 
STIPULATIONS_ON_USE: Final data. Data users are encouraged to consult with the PI for proper data interpretation.
OTHER_COMMENTS: N/A 
REVISION: R2
R2: Fixed Header errors.
R1: Final Data. 
R0: Preliminary Data
AMS_Starttime_60s, AMS_Stoptime_60s, AMS_MidPointTime_60s, AMS_LAT_60s, AMS_LON_60s, AMS_ALT_60s, OA_lt_1um_AMS_60s, OA_lt_1um_AMS_prec_60s, OA_lt_1um_AMS_DL_60s, Sulfate_lt_1um_AMS_60s, Sulfate_lt_1um_AMS_prec_60s, Sulfate_lt_1um_AMS_DL_60s, Ammonium_lt_1um_AMS_60s, Ammonium_lt_1um_AMS_prec_60s, Ammonium_lt_1um_AMS_DL_60s, Nitrate_lt_1um_AMS_60s, Nitrate_lt_1um_AMS_prec_60s, Nitrate_lt_1um_AMS_DL_60s, Chloride_lt_1um_AMS_60s, Chloride_lt_1um_AMS_prec_60s, Chloride_lt_1um_AMS_DL_60s, Seasalt_lt_1um_AMS_60s, Seasalt_lt_1um_AMS_prec_60s, Seasalt_lt_1um_AMS_DL_60s, MSA_lt_1um_AMS_60s, MSA_lt_1um_AMS_prec_60s, MSA_lt_1um_AMS_DL_60s, StdtoVol_AMS_60s, IceFlag_AMS_60s, AmmBalance_lt_1um_AMS_60s, Density_lt_1um_AMS_60s, OADensity_lt_1um_AMS_60s, O_C_lt_1um_AMS_60s, H_C_lt_1um_AMS_60s, OA_OC_lt_1um_AMS_60s, OSc_lt_1um_AMS_60s, f43_lt_1um_AMS_60s, f44_lt_1um_AMS_60s, f57_lt_1um_AMS_60s, f60_lt_1um_AMS_60s, f82_lt_1um_AMS_60s, f91_lt_1um_AMS_60s, fC2H3O_lt_1um_AMS_60s, fCO2_lt_1um_AMS_60s, fC4H9_lt_1um_AMS_60s, fC2H4O2_lt_1um_AMS_60s, fC5H6O_lt_1um_AMS_60s, fC7H7_lt_1um_AMS_60s, OrgNitr_Fraction_lt_1um_AMS_60s
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37920.00,37980.00,37950.00,-53.0455,-70.7809,1741.5,-0.0563,0.0476,0.0935,0.0689,0.0054,0.0112,0.0027,0.0014,0.0013,-0.0024,0.0049,0.0060,-0.0032,0.0043,0.0087,0.0051,0.0133,0.0384,0.0004,0.0003,0.0009,1.27188,0,0.114,1.750,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888
37980.00,38040.00,38010.00,-53.0108,-70.6631,2235.6,-0.0548,0.0472,0.0927,0.0723,0.0056,0.0116,0.0027,0.0014,0.0013,-0.0006,0.0051,0.0064,-0.0030,0.0043,0.0086,0.0017,0.0050,0.0095,0.0003,0.0003,0.0007,1.34507,0,0.107,1.750,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888
38048.78,38094.78,38071.78,-52.9735,-70.5342,2807.5,-0.0229,0.0459,0.0899,0.0200,0.0053,0.0116,0.0010,0.0014,0.0013,0.0047,0.0047,0.0056,0.0075,0.0040,0.0079,-0.0005,0.0074,0.0171,0.0004,0.0002,0.0006,1.42886,0,0.082,1.692,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,-8888,1.00
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